US11584736B2ActiveUtilityA1

Heterocyclic P2Y14 receptor antagonists

67
Assignee: US HEALTHPriority: Feb 9, 2018Filed: Feb 11, 2019Granted: Feb 21, 2023
Est. expiryFeb 9, 2038(~11.6 yrs left)· nominal 20-yr term from priority
C07D 211/70A61P 11/06A61P 29/00C07D 409/10C07D 235/18C07D 211/18C07D 471/08C07D 209/10C07D 249/06C07D 209/20C07D 401/10A61P 13/12C07D 401/14C07D 211/34C07C 235/84C07D 403/04
67
PatentIndex Score
1
Cited by
46
References
25
Claims

Abstract

Disclosed are compounds of formulas (I)-(IX) for treating or preventing a disease or disorder responsive to antagonism of a P2Y14R receptor agonist in a mammal in need thereof, wherein R1-R8, X, Y, Z, X′, Y′, Z′, and A are as defined herein, that are useful in treating an inflammatory such as asthma, cystic fibrosis, and sterile inflammation of the kidney.

Claims

exact text as granted — not AI-modified
The invention claimed is: 
     
       1. A compound of formula (I): 
       
         
           
           
               
               
           
         
         wherein (i) X is N, Y is CH, and Z is CH, (ii) X is CH, Y is N, and Z is CH, (iii) X is CH, Y is CH, and Z is N, or (iv) X, Y, and Z are all CH, 
         R 1  is trifluoromethylphenyl, 
         R 2  is COOH, CN, CONH 2 , or 
       
       
         
           
           
               
               
           
         
         A is selected from the group consisting of 
       
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         wherein R 3  is at each occurrence H, C 1 -C 10  alkyl, C 3 -C 10  alkynyl, benzyl, C 1 -C 6  alkoxycarbonyl, CO((CH 2 ) 2 O) 6 (CH 2 ) 2 Q wherein Q is NH 2 , NHCOCH 3 , or NHCO(CH 3 ) 3 , or CO((CH 2 ) 2 O) 6 CH 3 , and wherein R 4  and R 5  are each H or F, 
         with the proviso that the compound is not 4-[4-(4-piperidinyl)phenyl]-7-[4-(trifluoromethyl)phenyl]-2-naphthalene-carboxylic acid, 
         or a pharmacologically acceptable salt thereof. 
       
     
     
       2. The compound or salt of  claim 1 , wherein X, Y, and Z are all CH. 
     
     
       3. The compound or salt of  claim 1 , wherein A is 
       
         
           
           
               
               
           
         
       
     
     
       4. The compound or salt of  claim 3 , wherein the compound is selected from the group consisting of: 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
       
     
     
       5. A pharmaceutical composition comprising a compound or salt of  claim 1  and a pharmaceutically acceptable carrier. 
     
     
       6. A method for antagonizing a P2Y 14 R receptor in a mammal in need thereof, comprising administering to the mammal an effective amount of a compound or salt of  claim 1 . 
     
     
       7. A method for treating an inflammatory condition in a mammal in need thereof, comprising administering to the mammal an effective amount of a compound or salt of  claim 1 . 
     
     
       8. The method of  claim 7 , wherein the inflammatory condition is selected from the group consisting of asthma, cystic fibrosis, and sterile inflammation of the kidney. 
     
     
       9. A compound of formula (III), (IV), or (V): 
       
         
           
           
               
               
           
         
         wherein R 6  is selected from the group consisting of 
       
       
         
           
           
               
               
           
         
         R 7  is COOH, CONH 2 , CN 
       
       
         
           
           
               
               
           
         
       
       or COCH 2 NMe 2 ,
 R 8  is selected from the group consisting of C 1 -C 10  alkyl, —CONHR 12 R 13 , —CONH(CH 2 ) m —NHR 14 R 15 , 
 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         R 10  is halo or CF 3 , 
         R 11  is halo, OH, or C 1 -C 6  alkoxy, 
         R 12  and R 13  are independently H or C 1 -C 6  alkyl, 
         R 14  and R 15  are independently H or C 1 -C 6  alkyl, 
         R 16  is H, C 1 -C 10  alkyl, or C 3 -C 10  alkynyl, 
         R 17  and R 18  are both H or both F, and 
         m is an integer of from 1 to about 10, 
         (i) X is N, Y is CH, and Z is CH, (ii) X is CH, Y is N, and Z is CH, (iii) X is CH, Y is CH, and Z is N, or X, Y, and Z are all H, 
         X′ and Y′ are C or N, and 
         Z′ is N or CR 9  wherein R 9  is H or C 1 -C 6  alkyl, 
         or a pharmaceutically acceptable salt thereof; 
         with the proviso that, in the compound of formula (III), when X=N and Y and Z are 
         CH, R 7  is CN, and R 6  is 
       
       
         
           
           
               
               
           
         
       
       wherein R 10  is CF 3 , then R 8  is not C 6  alkyl. 
     
     
       10. The compound or salt of  claim 9 , wherein R 7  is COOH. 
     
     
       11. The compound or salt of  claim 9 , wherein the compound is 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
       
     
     
       12. The compound or salt of  claim 9 , wherein the compound is 
       
         
           
           
               
               
           
         
       
     
     
       13. The compound or salt of  claim 9 , wherein the compound is 
       
         
           
           
               
               
           
         
       
       or 
       
         
           
           
               
               
           
         
       
     
     
       14. A pharmaceutical composition comprising a compound or salt of  claim 9  and a pharmaceutically acceptable carrier. 
     
     
       15. A method for antagonizing a P2Y 14 R receptor in a mammal in need thereof, comprising administering to the mammal an effective amount of a compound or salt of  claim 9 . 
     
     
       16. A method for treating an inflammatory condition in a mammal in need thereof, comprising administering to the mammal an effective amount of a compound or salt of  claim 9 . 
     
     
       17. The method of  claim 16 , wherein the inflammatory condition is selected from the group consisting of asthma, cystic fibrosis, and sterile inflammation of the kidney. 
     
     
       18. A compound of formula (II): 
       
         
           
           
               
               
           
         
         wherein R 6  is selected from the group consisting of 
       
       
         
           
           
               
               
           
         
         R 7  is COOH, CONH 2 , CN 
       
       
         
           
           
               
               
           
         
       
       or COCH 2 NMe 2 ,
 R 8  is selected from the group consisting of C 2 -C 10  alkyl, —CONHR 12 R 13 , —CONH(CH 2 ) m —NHR 14 R 15 , 
 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         wherein: 
         R 10  is halo or CF 3 , 
         R 11  is halo, OH, or C 1 -C 6  alkoxy, 
         R 12  and R 13  are independently H or C 1 -C 6  alkyl, 
         R 14  and R 15  are independently H or C 1 -C 6  alkyl, 
         R 16  is H, C 1 -C 10  alkyl, or C 3 -C 10  alkynyl, 
         R 17  and R 18  are both H or both F, 
         m is an integer of from 1 to about 10, 
         X′ and Y′ are C or N, and 
         Z′ is N or CR 9  wherein R 9  is H or C 1 -C 6  alkyl, 
         with the proviso that when R 6  is 4-chlorophenyl, R 7  is COOH, and R 9  is CH, then R 8  is not alkyl; 
         or a pharmaceutically acceptable salt thereof. 
       
     
     
       19. A pharmaceutical composition comprising a compound or salt of  claim 18  and a pharmaceutically acceptable carrier. 
     
     
       20. A method for antagonizing a P2Y 14 R receptor in a mammal in need thereof, comprising administering to the mammal an effective amount of a compound or salt of  claim 18 . 
     
     
       21. The compound or salt of  claim 9 , wherein the compound is a compound of formula (III) and wherein R 7  is COOH, CONH 2   
       
         
           
           
               
               
           
         
       
       or COCH 2 NMe 2 . 
     
     
       22. A pharmaceutical composition comprising a compound or salt of  claim 21  and a pharmaceutically acceptable carrier. 
     
     
       23. A method for antagonizing a P2Y 14 R receptor in a mammal in need thereof, comprising administering to the mammal an effective amount of a compound or salt of  claim 21 . 
     
     
       24. A method for treating an inflammatory condition in a mammal in need thereof, comprising administering to the mammal an effective amount of a compound or salt of  claim 21 . 
     
     
       25. The method of  claim 24 , wherein the inflammatory condition is selected from the group consisting of asthma, cystic fibrosis, and sterile inflammation of the kidney.

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