P
US12150378B2ActiveUtilityPatentIndex 51

Luminescence device and polycyclic compound for luminescence device

Assignee: SAMSUNG DISPLAY CO LTDPriority: Oct 7, 2019Filed: Oct 5, 2020Granted: Nov 19, 2024
Est. expiryOct 7, 2039(~13.3 yrs left)· nominal 20-yr term from priority
Inventors:JIN XIULAN
H10K 85/6576H10K 85/6574H10K 85/657H10K 50/15C07D 495/04C07D 491/048H10K 85/615H10K 85/631H10K 85/636H10K 85/6572H10K 85/633H10K 85/626C07B 2200/05C09K 2211/1029C09K 2211/1092C09K 2211/1088C09K 2211/1037C09K 2211/1033C09K 2211/1022C09K 2211/1014C09K 2211/1011C07B 59/002C09K 11/06
51
PatentIndex Score
0
Cited by
25
References
18
Claims

Abstract

The present disclosure herein relates to a luminescence device including a polycyclic compound represented by Formula 1 in at least one functional layer and achieving a low driving voltage, high efficiency, and long life, and a polycyclic compound represented by Formula 1 below.

Claims

exact text as granted — not AI-modified
What is claimed is: 
     
       1. A luminescence device, comprising:
 a first electrode; 
 a second electrode disposed on the first electrode; and 
 at least one functional layer disposed between the first electrode and the second electrode, 
 wherein the at least one functional layer comprises a polycyclic compound represented by Formula 1: 
 
       
         
           
           
               
               
           
         
       
       wherein in Formula 1,
 X is O, or S, 
 R 1  and R 2  are each independently a hydrogen atom, a deuterium atom, a halogen atom, a substituted or unsubstituted alkyl group of 1 to 20 carbon atoms, a substituted or unsubstituted aryl group of 6 to 30 ring carbon atoms, or a substituted or unsubstituted heteroaryl group of 2 to 30 ring carbon atoms, 
 Ar 1  and Ar 2  are each independently represented by Formula 2:
   *—(Ar 11 ) p —Ar 12   Formula 2
 
 
 
       wherein in Formula 2,
 Ar 11  is a substituted or unsubstituted phenylene group, a substituted or unsubstituted divalent biphenyl group, a substituted or unsubstituted divalent terphenyl group, a substituted or unsubstituted phenanthrylene group, a substituted or unsubstituted fluorenylene group, a substituted or unsubstituted naphthylene group, a substituted or unsubstituted carbazolylene group, a substituted or unsubstituted dibenzofuranylene group, or a substituted or unsubstituted dibenzothiophenylene group, 
 Ar 12  is a substituted or unsubstituted phenyl group, a substituted or unsubstituted biphenyl group, a substituted or unsubstituted terphenyl group, a substituted or unsubstituted phenanthryl group, a substituted or unsubstituted fluorenyl group, a substituted or unsubstituted naphthyl group, a substituted or unsubstituted carbazolyl group, a substituted or unsubstituted dibenzofuranyl group, or a substituted or unsubstituted dibenzothiophenyl group, and 
 p is 0 or 1, 
 provided that i) when n is 1 and *—(Ar 11 ) p Ar 12  of Ar 1  is an unsubstituted biphenylene group, then *—(Ar 11 ) p Ar 12  of Ar 2  is not an unsubstituted dibenzothiophenylene group, and ii) when n is 1 and *—(Ar 11 ) p Ar 12  of Ar 2  is an unsubstituted biphenylene group, then *—(Ar 11 ) p Ar 12  of Ar 1  is not an unsubstituted dibenzothiophenylene group, 
 wherein in Formula 1, 
 Ar 3  is a substituted or unsubstituted aryl group of 6 to 30 ring carbon atoms, or a substituted or unsubstituted heteroaryl group of 2 to 30 ring carbon atoms, 
 L is a direct linkage, a substituted or unsubstituted arylene group of 6 to 30 ring carbon atoms, or a substituted or unsubstituted heteroarylene group of 2 to 30 ring carbon atoms, 
 l is an integer of 0 to 3, 
 m is an integer of 0 to 4, and 
 n is an integer of 0 to 3. 
 
     
     
       2. The luminescence device of  claim 1 , wherein the at least one functional layer comprises:
 a hole transport region disposed on the first electrode; 
 an emission layer disposed on the hole transport region; and 
 an electron transport region disposed on the emission layer, 
 wherein the hole transport region comprises the polycyclic compound. 
 
     
     
       3. The luminescence device of  claim 2 , wherein the hole transport region comprises:
 a hole injection layer disposed on the first electrode; and 
 a hole transport layer disposed between the hole injection layer and the emission layer, 
 wherein the hole transport layer comprises the polycyclic compound. 
 
     
     
       4. The luminescence device of  claim 1 , wherein the polycyclic compound comprises one acyclic amine. 
     
     
       5. The luminescence device of  claim 1 , wherein Formula 1 is represented by Formula 1-1 or Formula 1-2: 
       
         
           
           
               
               
           
         
       
       wherein in Formula 1-1 and Formula 1-2,
 Ar 21 , Ar 22 , Ar 31 , and Ar 32  are each independently represented by Formula 2, 
 Ar 23  and Ar 33  are each independently a substituted or unsubstituted aryl group of 6 to 30 ring carbon atoms, or a substituted or unsubstituted heteroaryl group of 2 to 30 ring carbon atoms, 
 L 11 , and L 12  are each independently a direct linkage, a substituted or unsubstituted arylene group of 6 to 30 ring carbon atoms, or a substituted or unsubstituted heteroarylene group of 2 to 30 ring carbon atoms, and 
 n11, and n12 are each independently an integer of 0 to 3. 
 
     
     
       6. The luminescence device of  claim 1 , wherein Formula 1 is represented by Formula 1-3: 
       
         
           
           
               
               
           
         
       
       wherein in Formula 1-3,
 X, R 1 , R 2 , Ar 1 , Ar 2 , L, and I to n are the same as defined in Formula 1. 
 
     
     
       7. The luminescence device of  claim 1 , wherein Formula 1 is represented by Formula 1-4: 
       
         
           
           
               
               
           
         
       
       wherein in Formula 1-4,
 n1 is 0 or 1, and 
 X, R 1 , R 2 , Ar 1  to Ar 3 , 1, and m are the same as defined in Formula 1. 
 
     
     
       8. The luminescence device of  claim 1 , wherein Ar 1  and Ar 2  are each independently represented by Formulae 1-1 to 1-10: 
       
         
           
           
               
               
           
         
       
       wherein in Formulae 1-1 to 1-10,
 R 11  to R 27  are each independently a hydrogen atom, a deuterium atom, a halogen atom, a substituted or unsubstituted alkyl group of 1 to 20 carbon atoms, a substituted or unsubstituted aryl group of 6 to 30 ring carbon atoms, or a substituted or unsubstituted heteroaryl group of 2 to 30 ring carbon atoms, 
 r1, r2, and r5 are each independently an integer of 0 to 4, 
 r3 is an integer of 0 to 5, 
 r4, r6, r8, and r10 to r12 are each independently an integer of 0 to 7, 
 r7 is an integer of 0 to 9, 
 r9 and r13 are each independently an integer of 0 to 8, and 
 q1 and q2 are each independently 0 or 1. 
 
     
     
       9. The luminescence device of  claim 1 , wherein Formula 1 is represented by Formula 1-5: 
       
         
           
           
               
               
           
         
       
       wherein in Formula 1-5,
 n1 is 0 or 1, and 
 X, Ar 1 , and Ar 2  are the same as defined in Formula 1. 
 
     
     
       10. A luminescence device, comprising:
 a first electrode; 
 a second electrode disposed on the first electrode; and 
 at least one functional layer disposed between the first electrode and the second electrode, 
 wherein the at least one functional layer comprises a polycyclic compound comprising at least one among Compound Group 1 and Compound Group 2: 
 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
       
     
     
       11. A polycyclic compound represented by the following Formula 1: 
       
         
           
           
               
               
           
         
         in Formula 1, 
         X is O, or S, 
         R 1  and R 2  are each independently a hydrogen atom, a deuterium atom, a halogen atom, a substituted or unsubstituted alkyl group of 1 to 20 carbon atoms, a substituted or unsubstituted aryl group of 6 to 30 ring carbon atoms, or a substituted or unsubstituted heteroaryl group of 2 to 30 ring carbon atoms, 
         Ar 1  and Ar 2  are each independently represented by Formula 2:
   *—(Ar 11 ) p —Ar 12   Formula 2
 
 
       
       wherein in Formula 2,
 Ar 11  is a substituted or unsubstituted phenylene group, a substituted or unsubstituted divalent biphenyl group, a substituted or unsubstituted divalent terphenyl group, a substituted or unsubstituted phenanthrylene group, a substituted or unsubstituted fluorenylene group, a substituted or unsubstituted naphthylene group, a substituted or unsubstituted carbazolylene group, a substituted or unsubstituted dibenzofuranylene group, or a substituted or unsubstituted dibenzothiophenylene group, 
 Ar 12  is a substituted or unsubstituted phenyl group, a substituted or unsubstituted biphenyl group, a substituted or unsubstituted terphenyl group, a substituted or unsubstituted phenanthryl group, a substituted or unsubstituted fluorenyl group, a substituted or unsubstituted naphthyl group, a substituted or unsubstituted carbazolyl group, a substituted or unsubstituted dibenzofuranyl group, or a substituted or unsubstituted dibenzothiophenyl group, and 
 p is 0 or 1, 
 provided that i) when n is 1 and *—(Ar 11 ) p Ar 12  of Ar 1  is an unsubstituted biphenylene group, then *—(Ar 11 ) p Ar 12  of Ar 2  is not an unsubstituted dibenzothiophenylene group, and ii) when n is 1 and *—(Ar 11 ) p Ar 12  of Ar 2  is an unsubstituted biphenylene group, then *—(Ar 11 ) p Ar 12  of Ar 1  is not an unsubstituted dibenzothiophenylene group, 
 wherein in Formula 1, 
 Ar 3  is a substituted or unsubstituted aryl group of 6 to 30 ring carbon atoms, or a substituted or unsubstituted heteroaryl group of 2 to 30 ring carbon atoms, 
 L is a direct linkage, a substituted or unsubstituted arylene group of 6 to 30 ring carbon atoms, or a substituted or unsubstituted heteroarylene group of 2 to 30 ring carbon atoms, 
 l is an integer of 0 to 3, 
 m is an integer of 0 to 4, and 
 n is an integer of 0 to 3. 
 
     
     
       12. The polycyclic compound of  claim 11 , wherein the polycyclic compound comprises one acyclic amine. 
     
     
       13. The polycyclic compound of  claim 11 , wherein Formula 1 is represented by the following Formula 1-1 or Formula 1-2: 
       
         
           
           
               
               
           
         
         in Formula 1-1 and Formula 1-2, 
         Ar 21 , Ar 22 , Ar 31 , and Ar 32  are each independently represented by Formula 2, 
         Ar 23  and Ar 33  are each independently a substituted or unsubstituted aryl group of 6 to 30 ring carbon atoms, or a substituted or unsubstituted heteroaryl group of 2 to 30 ring carbon atoms, 
         L 11 , and L 12  are each independently a direct linkage, a substituted or unsubstituted arylene group of 6 to 30 ring carbon atoms, or a substituted or unsubstituted heteroarylene group of 2 to 30 ring carbon atoms, and 
         n11, and n12 are each independently an integer of 0 to 3. 
       
     
     
       14. The polycyclic compound of  claim 11 , wherein Formula 1 is represented by the following Formula 1-3: 
       
         
           
           
               
               
           
         
       
       wherein in Formula 1-3,
 X, R 1 , R 2 , Ar 1 , Ar 2 , L, and I to n are the same as defined in Formula 1. 
 
     
     
       15. The polycyclic compound of  claim 11 , wherein Formula 1 is represented by the following Formula 1-4: 
       
         
           
           
               
               
           
         
       
       wherein in Formula 1-4,
 n1 is 0 or 1, and 
 X, R 1 , R 2 , Ar 1  to Ar 3 , 1, and m are the same as defined in Formula 1. 
 
     
     
       16. The polycyclic compound of  claim 11 , wherein Ar 1  and Ar 2  are each independently represented by the following 1-1 to 1-10: 
       
         
           
           
               
               
           
         
       
       wherein in 1-1 to 1-10,
 R 11  to R 27  are each independently a hydrogen atom, a deuterium atom, a halogen atom, a substituted or unsubstituted alkyl group of 1 to 20 carbon atoms, a substituted or unsubstituted aryl group of 6 to 30 ring carbon atoms, or a substituted or unsubstituted heteroaryl group of 2 to 30 ring carbon atoms, 
 r1, r2, and r5 are each independently an integer of 0 to 4, 
 r3 is an integer of 0 to 5, 
 r4, r6, r8, and r10 to r12 are each independently an integer of 0 to 7, 
 r7 is an integer of 0 to 9, 
 r9 and r13 are each independently an integer of 0 to 8, and 
 q1 and q2 are each independently 0 or 1. 
 
     
     
       17. The polycyclic compound of  claim 11 , wherein Formula 1 is represented by the following Formula 1-5: 
       
         
           
           
               
               
           
         
         in Formula 1-5, 
         n1 is 0 or 1, and 
         X, Ar 1 , and Ar 2  are the same as defined in Formula 1. 
       
     
     
       18. A polycyclic compound selected from Compound Group 1 or Compound Group 2:

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