US2004068062A1PendingUtilityA1

Hydroxyaliphatic functional epoxy resins

Priority: Aug 3, 1999Filed: Jun 24, 2003Published: Apr 8, 2004
Est. expiryAug 3, 2019(expired)· nominal 20-yr term from priority
C08G 59/1466C08F 290/064C08F 22/1006C07D 303/24C08F 290/061C08G 59/245C08F 290/06
45
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Claims

Abstract

The present invention concerns hydroxyaliphatic functional diglycidyl ethers of bisphenols (epoxy resins); curable (thermosettable) mixtures of at least one hydroxyaliphatic functional epoxy resin and at least one curing agent and/or catalyst therefor, as well as cured (thermoset) compositions prepared therefrom; and derivatives prepared therefrom. The bisphenol precursor to the diglycidyl ether contains a hydroxyaliphatic group linkage between the two aromatic rings of the bisphenol.

Claims

exact text as granted — not AI-modified
What is claimed is:  
     
         1 . A resin having the structural Formula I  
       
         
           
           
               
               
           
         
       
       wherein each R is independently selected from the group consisting of hydrogen, a hydrocarbyl or hydrocarbyloxy group having from one to about 10 carbon atoms, a halogen atom, a nitro group, a nitrile group and a —CO—R 2  group; each E is independently selected from the group consisting of  
       
         
           
           
               
               
           
         
       
       each R 1  is independently selected from the group consisting of hydrogen and a hydrocarbyl group having from one to about 10 carbon atoms; X is independently selected from the group consisting of  
       
         
           
           
               
               
           
         
       
       each R 2  is independently selected from the group consisting of hydrogen and a hydrocarbyl group having from one to about 10 carbon atoms; R 3  is a hydrocarbyl group having from one to about 10 carbon atoms; and n has a value of from one to about 10.  
     
     
         2 . A resin of  claim 1  wherein E is  
       
         
           
           
               
               
           
         
       
     
     
         3 . A resin of  claim 1  wherein E is  
       
         
           
           
               
               
           
         
       
     
     
         4 . A resin of  claim 1  wherein each R is hydrogen.  
     
     
         5 . A resin of  claim 1  wherein R 1  is hydrogen.  
     
     
         6 . A resin of  claim 1  wherein X is  
       
         
           
           
               
               
           
         
       
     
     
         7 . A resin of  claim 1  wherein X is  
       
         
           
           
               
               
           
         
       
     
     
         8 . A resin of  claim 1  wherein X is  
       
         
           
           
               
               
           
         
       
     
     
         9 . A resin prepared by advancing a resin of Formula I wherein E is  
       
         
           
           
               
               
           
         
       
     
     
         10 . A resin having the structural Formula II  
       
         
           
           
               
               
           
         
       
       wherein each R is independently selected from the group consisting of hydrogen, a hydrocarbyl or hydrocarbyloxy group having from one to about 10 carbon atoms, a halogen atom, a nitro group, a nitrile group and a —CO—R 2  group; each E is independently selected from the group consisting of  
       
         
           
           
               
               
           
         
       
       each R 1  is independently selected from the group consisting of hydrogen and a hydrocarbyl group having from one to about 10 carbon atoms; each R 2  is independently selected from the group consisting of hydrogen and a hydrocarbyl group having from one to about 10 carbon atoms; R 3  is a hydrocarbyl group having from one to about 10 carbon atoms; n has a value of from one to about 10; and X 1  is selected from the group consisting of  
       
         
           
           
               
               
           
         
       
       E 1  is a moiety containing a polymerizable ethylenically unsaturated group wherein the oxygen atom attached to E 1  is part of an ester or a urethane linkage.  
     
     
         11 . A resin of  claim 10  wherein E is  
       
         
           
           
               
               
           
         
       
     
     
         12 . A resin of  claim 10  wherein E is  
       
         
           
           
               
               
           
         
       
     
     
         13 . A resin of  claim 10  wherein each R is hydrogen.  
     
     
         14 . A resin of  claim 10  wherein R 1  is hydrogen.  
     
     
         15 . A resin of  claim 10  wherein X 1  is  
       
         
           
           
               
               
           
         
       
     
     
         16 . A resin of  claim 10  wherein X 1  is  
       
         
           
           
               
               
           
         
       
     
     
         17 . A resin of  claim 10  wherein X 1  is  
       
         
           
           
               
               
           
         
       
     
     
         18 . A composition comprising a resin of Formula and a resin of Formula II.  
     
     
         19 . A polymer modified epoxy resin prepared by polymerizing an epoxy resin of the composition of  claim 18  with one or more polymerizable ethylenically unsaturated monomers.  
     
     
         20 . A polymer modified vinyl ester resin prepared from the resin of  claim 19 .  
     
     
         21 . A resin having the structural Formula III  
       
         
           
           
               
               
           
         
       
       wherein each R is independently selected from the group consisting of hydrogen, a hydrocarbyl or hydrocarbyloxy group having from one to about 10 carbon atoms, a halogen atom, a nitro group, a nitrile group and a —CO—R 2  group; each E is independently selected from the group consisting of  
       
         
           
           
               
               
           
         
       
       each R 1  is independently selected from the group consisting of hydrogen and a hydrocarbyl group having from one to about 10 carbon atoms; each R 2  is independently selected from the group consisting of hydrogen and a hydrocarbyl group having from one to about 10 carbon atoms; R 3  is a hydrocarbyl group having from one to about 10 carbon atoms; n has a value of from one to about 10; E 3  is a direct bond or a hydrocarbyl group having from one to about 30 carbon atoms; and X 2  is selected from the group consisting of  
       
         
           
           
               
               
           
         
       
     
     
         22 . A resin of  claim 21  wherein E is  
       
         
           
           
               
               
           
         
       
     
     
         23 . A resin of  claim 21  wherein E is  
       
         
           
           
               
               
           
         
       
     
     
         24 . A resin of  claim 21  wherein each R is hydrogen.  
     
     
         25 . A resin of  claim 21  wherein R 1  is hydrogen.  
     
     
         26 . A resin of  claim 21  wherein X 2  is  
       
         
           
           
               
               
           
         
       
     
     
         27 . A resin of  claim 21  wherein X 2  is  
       
         
           
           
               
               
           
         
       
     
     
         28 . A resin of  claim 21  wherein X 2  is  
       
         
           
           
               
               
           
         
       
     
     
         29 . A resin of  claim 21  wherein E 3  is —(CH 2 ) 4 —.  
     
     
         30 . A resin having the structural Formula IV  
       
         
           
           
               
               
           
         
       
       wherein each R is independently selected from the group consisting of hydrogen, a hydrocarbyl or hydrocarbyloxy group having from one to about 10 carbon atoms, a halogen atom, a nitro group, a nitrile group and a —CO—R 2  group; each E is independently selected from the group consisting of  
       
         
           
           
               
               
           
         
       
       each R 1  is independently selected from the group consisting of hydrogen and a hydrocarbyl group having from one to about 10 carbon atoms; each R 2  is independently selected from the group consisting of hydrogen and a hydrocarbyl group having from one to about 10 carbon atoms; R 3  is a hydrocarbyl group having from one to about 10 carbon atoms; n has a value of from one to about 10; E 4  is a hydrocarbyl group having from about 4 to about 35 carbon atoms; X 2  is selected from the group consisting of  
       
         
           
           
               
               
           
         
       
     
     
         31 . A resin of  claim 30  wherein E is  
       
         
           
           
               
               
           
         
       
     
     
         32 . A resin of  claim 30  wherein E is  
       
         
           
           
               
               
           
         
       
     
     
         33 . A resin of  claim 30  wherein each R is hydrogen.  
     
     
         34 . A resin of  claim 30  wherein R 1  is hydrogen.  
     
     
         35 . A resin of  claim 30  wherein X 2  is  
       
         
           
           
               
               
           
         
       
     
     
         36 . A resin of  claim 30  wherein X 2  is  
       
         
           
           
               
               
           
         
       
     
     
         37 . A resin of  claim 30  wherein X 2  is  
       
         
           
           
               
               
           
         
       
     
     
         38 . A resin of  claim 30  wherein E 4  is  
       -p-C 6 H 4 —CH 2 —P—C 6 H 4 —.  
     
     
         39 . A polymer modified epoxy resin prepared by polymerizing an epoxy resin of Formula II with one or more polymerizable ethylenically unsaturated monomers.  
     
     
         40 . A polymer modified vinyl ester resin prepared from the resin of  claim 39.

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