US2007135489A1PendingUtilityA1

Vegfr-2 and vegfr-3 inhibitory anthranilamide pyridones

56
Assignee: HUTH ANDREASPriority: Jun 13, 2003Filed: Jan 18, 2007Published: Jun 14, 2007
Est. expiryJun 13, 2023(expired)· nominal 20-yr term from priority
C07D 213/64
56
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Claims

Abstract

Novel VEGFR-2 and VEGFR-3 inhibitory anthranilamide pyridones and their use as pharmaceutical agents for treating diseases that are triggered by persistent angiogenesis are selected.

Claims

exact text as granted — not AI-modified
1 - 11 . (canceled)  
     
     
         12 . A method for treating a tumor or metastasis growth, psoriasis, Kaposi's sarcoma, restenosis, stent-induced restenosis, endometriosis, Crohn's disease, Hodgkin's disease, leukemia, arthritis, rheumatoid arthritis, hemangioma, angiofibroma, an eye disease, diabetic retinopathy, neovascular glaucoma, a renal disease, glomerulonephritis, diabetic nephropathy, malignant nephrosclerosis, thrombic microangiopathic syndrome, a transplant rejection, glomerulopathy, a fibrotic disease, cirrhosis of the liver, a mesangial cell proliferative disease, arteriosclerosis, an injury to nerve tissue, senile keratosis or contact dermatitis; a method for inhibiting the reocclusion of a vessel after balloon catheter treatment, vascular prosthetics or use of a mechanical device to keep vessels open, or use of a stent; a method for immunosuppression or supporting scar-free healing; or 
 a method for inhibiting tyrosine kinases selected from KDR, FLT-1 and FLT-4 or inhibiting VEGFR kinase 3 of lymphangiogenesis    comprising administering to a patient in need thereof an effective amount of a pharmaceutical composition comprising a pharmaceutically acceptable carrier and a compound of formula I                          in which    A stands for an aryl or heteroaryl,    X stands for hydrogen or fluorine,    R 1  and R 2 , independently of one another, stand for hydrogen, halogen, C 1 -C 12 -alkyl, C 1 -C 12 -alkoxy-C 1 -C 10 -alkylene, halo-C 1 -C 10 -alkyl, C 3 -C 10 -cycloalkyl or halo-C 3 -C 10 -cycloalkyl, and    Y stands for a bond or for oxygen or for the group —S—, —S(O)— or —SO 2 —,    or a salt thereof.    
     
     
         13 . A method according to  claim 12 , which is for treating a tumor or metastasis growth, psoriasis, Kaposi's sarcoma, restenosis, stent-induced restenosis, endometriosis, Crohn's disease, Hodgkin's disease, leukemia, arthritis, rheumatoid arthritis, hemangioma, angiofibroma, an eye disease, diabetic retinopathy, neovascular glaucoma, a renal disease, glomerulonephritis, diabetic nephropathy, malignant nephrosclerosis, thrombic microangiopathic syndrome, a transplant rejection, glomerulopathy, a fibrotic disease, cirrhosis of the liver, a mesangial cell proliferative disease, arteriosclerosis, an injury to nerve tissue, senile keratosis or contact dermatitis; a method for inhibiting the reocclusion of a vessel after balloon catheter treatment, vascular prosthetics or use of a mechanical device to keep vessels open, or use of a stent; a method for immunosuppression or supporting scar-free healing.  
     
     
         14 . A method according to  claim 12 , which is for inhibiting tyrosine kinases selected from KDR, FLT-1 and FLT-4.  
     
     
         15 . A method according to  claim 12 , which is for inhibiting VEGFR kinase 3 of lymphangiogenesis.  
     
     
         16 . A method according to  claim 12 , which is for treating psoriasis, Kaposi's sarcoma, stent-induced restenosis, endometriosis, Crohn's disease, Hodgkin's disease, leukemia, rheumatoid arthritis, hemangioma, angiofibroma, diabetic retinopathy, neovascular glaucoma, glomerulonephritis, diabetic nephropathy, malignant nephrosclerosis, thrombic microangiopathic syndrome, a transplant rejection, glomerulopathy, cirrhosis of the liver, arteriosclerosis; or a method for inhibiting the reocclusion of a vessel after balloon catheter treatment, vascular prosthetics or use of a mechanical device to keep vessels open, or use of a stent; or a method for supporting scar-free healing.  
     
     
         17 . A method according to  claim 12 , wherein at least one of the Y groups is oxygen, —S—, —S(O)— or —SO 2 —.  
     
     
         18 . A method according to  claim 12 , wherein at least one of the Y groups is oxygen or —S—.  
     
     
         19 . A method according to  claim 12 , wherein A stands for: cyclopropenyl, cyclopentadienyl, phenyl, tropyl, cyclooctadienyl, indenyl, naphthyl, azulenyl, biphenyl, fluorenyl, anthracenyl, thienyl, furanyl, pyrrolyl, oxazolyl, thiazolyl, imidazolyl, pyrazolyl, isoxazolyl, isothiazolyl, oxadiazolyl, triazolyl, thiadiazolyl, benzofuranyl, benzothienyl, benzoxazolyl, benzimidazolyl, indolyl, isoindolyl, pyridyl, pyridazinyl, pyrimidinyl, pyrazinyl, triazinyl, quinolyl, isoquinolyl, azocinyl, indolizinyl, purinyl, quinolinyl, isoquinolinyl, cinnolinyl, phthalazinyl, quinazolinyl, quinoxalinyl, naphthyridinyl, pteridinyl, carbazolyl, acridinyl, phenazinyl, phenothiazinyl, phenoxazinyl, xanthenyl, or oxepinyl.  
     
     
         20 . A method according to  claim 12 , wherein R 1  or R 2  is —OCF 3 , —OMe, -OiProp, —OEt, -OnBu, —OCH 2 CF 3 , —OH, —SCF 3 , —OCH 2 CH 2 OMe, —OCHF 2 , —OCH 2 CH 2 CF 3 , —OCH 2 CF 2 CF 3 , —OCH(CF 3 ) 2 , —OCH(CF 3 ) 2 CH 3 , —Cl, or —OCH 2 CH(CH 3 ) 2 .  
     
     
         21 . A method according to  claim 12 , wherein 
 A stands for a phenyl or pyridyl,    X stands for hydrogen or fluorine,    R 1  and R 2 , independently of one another, stand for hydrogen, halogen, C 1 -C 12 -alkyl, C 1 -C 12 -alkoxy-C 1 -C 10 -alkylene, C 3 -C 10 -cycloalkyl or halo-C 3 -C 10 -cycloalkyl and    Y stands for a bond or for oxygen or for the group —S—, —S(O)— or —SO 2 —,    or a salt thereof.    
     
     
         22 . A method according to  claim 12 , wherein 
 A stands for a phenyl,    X stands for hydrogen or fluorine,    R 1  and R 2 , independently of one another, stand for hydrogen, halogen, C 1 -C 2 -alkyl, C 1 -C 12 -alkoxy-C 1 -C 10 -alkylene, halo-C 1 -C 10 -alkyl, C 3 -C 10 -cycloalkyl or halo-C 3 -C 10 -cycloalkyl, and    Y stands for a bond or for oxygen or for the group —S—, —S(O)— or —SO 2 —,    or a salt thereof.    
     
     
         23 . A method according to  claim 12 , wherein 
 A stands for a phenyl,    X stands for hydrogen,    R 1  and R 2 , independently of one another, stand for hydrogen, halogen, C 1 -C 12 -alkyl, C 1 -C 12 -alkoxy-C 1 -C 10 -alkylene, C 3 -C 10 -cycloalkyl or halo-C 3 -C 10 -cycloalkyl, and    Y stands for a bond or for oxygen or for the group —S—, —S(O)— or —SO 2 —,    or a salt thereof.    
     
     
         24 . A method according to  claim 12 , wherein 
 A stands for an aryl or heteroaryl, wherein the heteroaryl is not an indazole group,    X stands for hydrogen or fluorine,    R 1  and R 2 , independently of one another, stand for hydrogen, halogen, C 1 -C 12 -alkyl, C 1 -C 12 -alkoxy-C 1 -C 10 -alkylene, C 3 -C 10 -cycloalkyl or halo-C 3 -C 10 -cycloalkyl, and    Y stands for a bond or for oxygen or for the group —S—, —S(O)— or —SO 2 —,    or a salt thereof.    
     
     
         25 . A method according to  claim 12 , wherein the compound of formula I is an isomer, enantiomer, or diastereomer of said compound.  
     
     
         26 . A method according to  claim 12 , wherein the administration is selected from enteral, parenteral and oral administration.  
     
     
         27 . A method according to  claim 12 , wherein the compound of formula I is  
       
         
           
                 
               
                     
                 
                     
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                     
                 
             
                
                
                
                
                
                
                
                
                
               
               
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
               
            
           
         
       
     
     
         28 . A method according to  claim 12 , wherein the compound of formula I is  
       
         
           
           
               
               
           
         
       
     
     
         29 . A method according to  claim 12 , wherein A stands for an aryl or unsubstituted heteroaryl moiety.  
     
     
         30 . A method according to  claim 24 , wherein A stands for an aryl or unsubstituted heteroaryl moiety.

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