US2007178134A1PendingUtilityA1

Pyridines and uses thereof

Assignee: CELL THERAPEUTICS INCPriority: Apr 4, 2003Filed: Mar 14, 2007Published: Aug 2, 2007
Est. expiryApr 4, 2023(expired)· nominal 20-yr term from priority
A61L 31/10A61L 27/34C07D 213/74C07D 213/75
61
PatentIndex Score
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Claims

Abstract

The invention relates to pyridines and uses thereof, including to inhibit lysophosphatidic acid acyltransferase β (LPAAT-β) activity and/or proliferation of cells such as tumor cells.

Claims

exact text as granted — not AI-modified
1 . A compound or physiologically acceptable salt thereof, wherein the compound has the formula:  
       
         
           
           
               
               
           
         
       
       wherein: 
 X, Y and Z are N, CH or CR where R is alkyl, alkoxy, Cl, Br, NH 2 , NHR′ or NR′R″ where R′ and R″ independently are alkyl;  
 Q is NR, RN—(CH 2 ) n , (CH 2 ) n —NR, O, O—(CH 2 ) n , (CH 2 ) n —O, S, S—(CH 2 ) n , or (CH 2 ) n —S, where n is 1-10 and R is H or alkyl;  
 R 1  is H, OH, alkyl, alkoxy, Cl, F, Br, CR 3  where R 3  is Cl 3 , F 3  or Br 3 , NH 2 , NHR or NRR′ where R and R′ independently are alkyl;  
 R 2  is H, OH, alkyl, alkoxy, Cl, F, Br or CR 3  where R 3  is Cl 3 , F 3  or Br 3 ;  
 R 3  is H, alkyl, alkoxy, Cl, CCl 3 , NH 2 , NHR or NRR′ where R and R′ independently are alkyl or acyl;  
 R 4 , R 5 , and R are independently H, OH, alkyl, alkenyl, alkynyl, alkoxy, (CH 2 ) n —OR where R is H or alkyl and n is 1-10, Cl, F, Br, CR 3  where R 3  is Cl 3 , F 3  or Br 3  heterocycle, N + (═O)O − , C≡N, N 3 , SH, SR or S(═O) 2 R where R is alkyl, NH 2 , NHR or NRR′ where R and R′ independently are alkyl, or R 4  and R 5  or R 5  and R 6  are taken together with the benzene ring to form a heterocycle;  
 and with the proviso that one of X, Y and Z is N.  
 
     
     
         2 . The compound or salt thereof of  claim 1  wherein X or Y of the compound or salt thereof is N.  
     
     
         3 . The compound or salt thereof of  claim 1  wherein Q of the compound or salt thereof is NH.  
     
     
         4 . The compound or salt thereof of  claim 1  wherein R 4  or R 5  of the compound or salt thereof is acyl.  
     
     
         5 . The compound or salt thereof of  claim 1  wherein R 1  of the compound or salt thereof is alkyl, alkoxy or Cl.  
     
     
         6 . The compound or salt thereof of  claim 1  wherein R 2  of the compound or salt thereof is Cl or Br.  
     
     
         7 . The compound or salt thereof of  claim 1  wherein R 3  of the compound or salt thereof is alkyl or NH 2 .  
     
     
         8 . The compound or salt thereof of  claim 1  wherein R 4  or R 5  of the compound or salt thereof is alkyl, Cl, Br, CF 3 , CH 2 —OH, (CH 2 ) 2 —OH, N + (═O)O − , C≡N, or C(═O)R wherein R is alkyl or alkoxy, or R 4  and R 5  are taken together with the benzene ring to form indazole.  
     
     
         9 . The compound or salt thereof of  claim 1  wherein the compound is any one of compounds 1-14 of Table 1, or physiologically acceptable salts thereof.  
     
     
         10 . A pharmaceutical composition comprising a compound or salt thereof according to  claim 1  in combination with a pharmaceutically acceptable carrier or diluent.  
     
     
         11 . The pharmaceutical composition of  claim 10  wherein X or Y of the compound or salt thereof is N.  
     
     
         12 . The pharmaceutical composition of  claim 10  wherein Q of the compound or salt thereof is NH.  
     
     
         13 . The pharmaceutical composition of  claim 10  wherein R 4  or R 5  of the compound or salt thereof is acyl.  
     
     
         14 . The pharmaceutical composition of  claim 10  wherein R 1  of the compound or salt thereof is alkyl, alkoxy or Cl.  
     
     
         15 . The pharmaceutical composition of  claim 10  wherein R 2  of the compound or salt thereof is Cl or Br.  
     
     
         16 . The pharmaceutical composition of  claim 10  wherein R 3  of the compound or salt thereof is alkyl or NH 2 .  
     
     
         17 . The pharmaceutical composition of  claim 10  wherein R 4  or R 5  of the compound or salt thereof is alkyl, Cl, Br, CF 3 , CH 2 —OH, (CH 2 ) 2 —OH, N + (═O)O − , C≡N, or C(═O)R wherein R is alkyl or alkoxy, or R 4  and R 5  are taken together with the benzene ring to form indazole.  
     
     
         18 . The pharmaceutical composition of  claim 10  wherein the compound is any one of compounds 1-14 of Table 1, or physiologically acceptable salts thereof.  
     
     
         19 . A method for reducing the activity of lysophosphatidic acid acyltransferase β (LPAAT-β) comprising contacting LPAAT-β with a compound or salt thereof according to  claim 1  or a composition according to  claim 10  in an amount effective to reduce LPAAT-β activity.  
     
     
         20 . The method of  claim 19  wherein the LPAAT-β resides in an animal.  
     
     
         21 . The method of  claim 20  wherein the animal is a mammal.  
     
     
         22 . The method of  claim 19  wherein X or Y of the compound or salt thereof is N.  
     
     
         23 . The method of  claim 19  wherein Q of the compound or salt thereof is NH.  
     
     
         24 . The method of  claim 19  wherein R 4  or R 5  of the compound or salt thereof is acyl.  
     
     
         25 . The method of  claim 19  wherein R 1  of the compound or salt thereof is alkyl, alkoxy or Cl.  
     
     
         26 . The method of  claim 19  wherein R 2  of the compound or salt thereof is Cl or Br.  
     
     
         27 . The method of  claim 19  wherein R 3  of the compound or salt thereof is alkyl or NH 2 .  
     
     
         28 . The method of  claim 19  wherein R 4  or R 5  of the compound or salt thereof is alkyl, Cl, Br, CF 3 , CH 2 —OH, (CH 2 ) 2 —OH, N + (═O)O − , C≡N, or C(═O)R wherein R is alkyl or alkoxy, or R 4  and R 5  are taken together with the benzene ring to form indazole.  
     
     
         29 . The method of  claim 19  wherein the compound is any one of compounds 1-14 of Table 1, or physiologically acceptable salts thereof.  
     
     
         30 . A method for inhibiting the proliferation of a cell in which the activity of lysophosphatidic acid acyltransferase β (LPAAT-β) is required for the proliferation of the cell comprising contacting the cell with a compound or salt thereof according to  claim 1  or a composition according to  claim 10  in an amount effective to inhibit the proliferation of the cell.  
     
     
         31 . The method of  claim 30  wherein the cell resides in an animal.  
     
     
         32 . The method of  claim 31  wherein the animal is a mammal.  
     
     
         33 . The method of  claim 30  wherein X or Y of the compound or salt thereof is N.  
     
     
         34 . The method of  claim 30  wherein Q of the compound or salt thereof is NH.  
     
     
         35 . The method of  claim 30  wherein R 4  or R 5  of the compound or salt thereof is acyl.  
     
     
         36 . The method of  claim 30  wherein R 1  of the compound or salt thereof is alkyl, alkoxy or Cl.  
     
     
         37 . The method of  claim 30  wherein R 2  of the compound or salt thereof is Cl or Br.  
     
     
         38 . The method of  claim 30  wherein R 3  of the compound or salt thereof is alkyl or NH 2 .  
     
     
         39 . The method of  claim 30  wherein R 4  or R 5  of the compound or salt thereof is alkyl, Cl, Br, CF 3 , CH 2 —OH, (CH 2 ) 2 —OH, N + (═O)O − , C≡N, or C(═O)R wherein R is alkyl or alkoxy, or R 4  and R 5  are taken together with the benzene ring to form indazole.  
     
     
         40 . The method of  claim 30  wherein the compound is any one of compounds 1-14 of Table I, or physiologically acceptable salts thereof.  
     
     
         41 . A method for treating a cancer in which lysophosphatidic acid acyltransferase β (LPAAT-β) activity is associated comprising administering to an animal in need, a compound or salt thereof according to  claim 1  or a composition according to  claim 10  in an amount effective to treat the cancer.  
     
     
         42 . The method of  claim 41  wherein the animal is a mammal.  
     
     
         43 . The method of  claim 41  wherein X or Y of the compound or salt thereof is N.  
     
     
         44 . The method of  claim 41  wherein Q of the compound or salt thereof is NH.  
     
     
         45 . The method of  claim 41  wherein R 4  or R 5  of the compound or salt thereof is acyl.  
     
     
         46 . The method of  claim 41  wherein R 1  of the compound or salt thereof is alkyl, alkoxy or Cl.  
     
     
         47 . The method of  claim 41  wherein R 2  of the compound or salt thereof is Cl or Br.  
     
     
         48 . The method of  claim 41  wherein R 3  of the compound or salt thereof is alkyl or NH 2 .  
     
     
         49 . The method of  claim 41  wherein R 4  or R 5  of the compound or salt thereof is alkyl, Cl, Br, CF 3 , CH 2 —OH, (CH 2 ) 2 —OH, N + (═O)O − , C≡N, or C(═O)R wherein R is alkyl or alkoxy, or R 4  and R 5  are taken together with the benzene ring to form indazole.  
     
     
         50 . The method of  claim 41  wherein the compound is any one of compounds 1-14 of Table 1, or physiologically acceptable salts thereof.  
     
     
         51 . A coated medical device for inhibiting the proliferation of a cell in which the activity of lysophosphatidic acid acyltransferase β (LPAAT-β) is required for the proliferation of the cell comprising a medical device coated with a compound or salt thereof according to  claim 1  or a composition according to  claim 10 .  
     
     
         52 . The device of  claim 51  wherein X or Y of the compound or salt thereof is N.  
     
     
         53 . The device of  claim 51  wherein Q of the compound or salt thereof is NH.  
     
     
         54 . The device of  claim 51  wherein R 4  or R 5  of the compound or salt thereof is acyl.  
     
     
         55 . The device of  claim 51  wherein R 1  of the compound or salt thereof is alkyl, alkoxy or Cl.  
     
     
         56 . The device of  claim 51  wherein R 2  of the compound or salt thereof is Cl or Br.  
     
     
         57 . The device of  claim 51  wherein R 3  of the compound or salt thereof is alkyl or NH 2 .  
     
     
         58 . The device of  claim 51  wherein R 4  or R 5  of the compound or salt thereof is alkyl, Cl, Br, CF 3 , CH 2 —OH, (CH 2 ) 2 —OH, N + (═O)O − , C≡N, or C(═O)R wherein R is alkyl or alkoxy, or R 4  and R 5  are taken together with the benzene ring to form indazole.  
     
     
         59 . The device of  claim 51  wherein the compound is any one of compounds 1-14 of Table 1, or physiologically acceptable salts thereof.

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