US2012009142A1PendingUtilityA1

Methods for treating hepatitis c

43
Assignee: KARP GARY MITCHELLPriority: Jul 14, 2004Filed: Jun 13, 2011Published: Jan 12, 2012
Est. expiryJul 14, 2024(expired)· nominal 20-yr term from priority
A61P 31/14A61P 31/20A61K 31/4439A61K 31/405A61K 31/404A61P 1/16Y02A50/30
43
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Claims

Abstract

In accordance with the present invention, compounds that inhibit viral replication, preferably Hepatitis C Virus (HCV) replication, have been identified, and methods for their use provided. In one aspect of the invention, compounds useful in the treatment or prevention of a viral infection are provided. In another aspect of the invention, compounds useful in the treatment or prevention of HCV infection are provided.

Claims

exact text as granted — not AI-modified
1 .- 41 . (canceled) 
     
     
         42 . A compound of Formula (I): 
       
         
           
           
               
               
           
         
       
       wherein: 
       X is: -cyano; 
       Y is: 
       amino optionally substituted with one or more C 1  to C 6  alkyl substituents; 
       —NHCOR e , where R e  is:
 —C 1  to C 6  alkyl; 
 cyclopropyl; 
 cyclobutyl; 
 cyclopentyl; 
 cyclohexyl; or 
 aryl optionally substituted with:
 —C 1  to C 6  alkyl, 
 —C 1  to C 6  alkoxy, 
 cyano, 
 nitro, or 
 halogen; 
 
 
       —NHCOOR x , where R x  is C 1  to C 6  alkyl; 
       —CH 2 O—R f , where R f  is aryl; 
       —NR g R h , where R g  is C 1  to C 6  alkyl or hydrogen and R h  is aryl optionally substituted with C 1  to C 6  alkoxy; 
       
         
           
           
               
               
           
         
       
       where R cc  is:
 naphthalene, 
 5 or 6 membered heteroaryl, 
 
       
         
           
           
               
               
           
         
         aryl, optionally substituted with one or more of the following:
 —C 1  to C 6  alkoxy, 
 hydroxy, 
 halogen, 
 —C 1  to C 6  alkyl, optionally substituted with cyano, 
 amino optionally substituted with one or more C 1  to C 6  alkyl substituents, 
 —NHPO(R x ) 2 , where R x  is as defined above, 
 —NR ee CONR ff , where R ee  is hydrogen or C 1  to C 6  alkyl, optionally substituted with halogen, and R ff  is:
 hydrogen, 
 —C 1  to C 6  haloalkyl, 
 —C 1  to C 6  haloalkoxy, 
 —C 1  to C 6  alkyl, or 
 —COR x , where R x  is as defined above, 
 
 —NR gg COR hh , where R hh  is:
 hydrogen, 
 —C 1  to C 6  alkyl optionally substituted with:
 —C 1  to C 6  alkoxy, 
 halogen, or 
 amino optionally substituted with one or more C 1  to C 6  alkyl substituents, 
 
 amino optionally substituted with one or more C 1  to C 6  alkyl substituents, where alkyl is optionally substituted with halogen, 
 5 or 6 membered heterocycle, 
 5 or 6 membered heteroaryl, 
 cyclopropyl, 
 cyclobutyl, 
 cyclopentyl, or 
 cyclohexyl, 
 
 and R gg  is:
 hydrogen, 
 —C 1  to C 6  alkyl, 
 —C 1  to C 6  haloalkyl, 
 —C 1  to C 6  haloalkoxy, or 
 —COR x , where R x  is as defined above, 
 —C 1  to C 6  haloalkyl, 
 5 or 6 membered heterocycle optionally substituted with carboxy or oxo, 
 amino optionally substituted with one or more C 1  to C 6  alkyl substituents, 
 —NR ii SO 2 R x , where R x  is as defined above, and R ii  is:
 hydrogen, 
 —C 1  to C 6  alkyl, 
 —C 1  to C 6  haloalkyl, 
 —C 1  to C 6  haloalkoxy, 
 —COR x , where R x  is as defined above; 
 
 
 
       
       Z is: 
       hydrogen; 
       —C 1  to C 6  alkyl optionally substituted with:
 —C 1  to C 6  alkoxy, 
 one or more halogen substituents, or 
 aryl; 
 
       aryl optionally substituted with C 1  to C 6  alkoxy or one or more C 1  to C 6  alkyl substituents; 
       R is hydrogen, halogen or C 1  to C 6  alkoxy; 
       R 1  is: 
       hydrogen; 
       hydroxy; 
       halogen; 
       —C 1  to C 6  haloalkyl; 
       nitro; 
       5 or 6 membered heteroaryl; 
       5 or 6 membered heterocycle; 
       —C 1  to C 6  alkoxy optionally substituted with:
 one or more halogen substituents, 
 aryl, or 
 5 or 6 membered heterocycle; 
 
       aryl optionally substituted with C 1  to C 6  alkoxy; 
       —COR x , where R x  is as defined above; 
       —C 1  to C 6  alkyl optionally substituted with di-C 1  to C 6  alkyl-amino or 5 or 6 membered heterocycle; or 
       R 1  joins together with R 2  to form: 
       
         
           
           
               
               
           
         
       
       R 2  is: 
       nitro; 
       hydrogen; 
       halogen; 
       hydroxy; 
       —C 1  to C 6  alkyl, optionally substituted with one or more halogen substituents; 
       amino; 
       —C 1  to C 6  alkoxy optionally substituted with:
 one or more halogen substituents, 
 —OCOR x , where R x  is as defined above, 
 di-C 1  to C 6  alkyl-amino optionally substituted with C 1  to C 6  alkoxy, 
 5 or 6 membered heterocycle optionally substituted with C 1  to C 6  alkyl, 
 5 or 6 membered heteroaryl, or 
 aryl; 
 
       —COOR x , where R x  is as defined above; 
       —C 1  to C 6  haloalkyl; 
       amide optionally substituted with:
 hydroxy, or 
 aryl; 
 
       5 or 6 membered heteroaryl; 
       —OCOR x , where R x  is as defined above; 
       —NHCOR jj , where R jj  is:
 —C 1  to C 6  alkoxy, or 
 amino optionally substituted with one or more C 1  to C 6  alkyl substituents; 
 
       —OR kk , where R kk  is 5 to 6 membered heteroaryl; 
       —NHSO 2 R x , where R x  is as defined above; or 
       R 2  joins together with R 1  to form: 
       
         
           
           
               
               
           
         
       
       and, 
       R 3  is: 
       hydrogen; or 
       —CH 2 OCOR x , and R x  is as defined above; 
       or a pharmaceutically acceptable salt thereof. 
     
     
         43 . The compound of  claim 42 , wherein Y is selected from the group consisting of the following compounds: 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
       
     
     
         44 . The compound of  claim 42 , wherein Z is selected from the group consisting of -hydrogen; —C 1  to C 6  alkyl optionally substituted with: —C 1  to C 6  alkoxy, -one or more halogen substituents, or -aryl; and -aryl optionally substituted with C 1  to C 6  alkoxy. 
     
     
         45 . The compound of  claim 42 , wherein Z is selected from the group consisting of -hydrogen; —C 1  to C 6  alkyl; and -aryl optionally substituted with C 1  to C 6  alkoxy. 
     
     
         46 . The compound of  claim 42 , wherein R is hydrogen. 
     
     
         47 . The compound of  claim 42 , wherein R 1  is selected from the group consisting of -hydrogen; -halogen; —C 1  to C 6  haloalkyl; -nitro; -5 or 6 membered heterocycle; —C 1  to C 6  alkoxy; -aryl optionally substituted with C 1  to C 6  alkoxy. 
     
     
         48 . The compound of  claim 42 , wherein R 2  is selected from the group consisting of -nitro; -hydrogen; -halogen; -hydroxy; —C 1  to C 6  alkyl, optionally substituted with one or more halogen substituents; C 1  to C 6  alkoxy optionally substituted with: -one or more halogen substituents, —OCOR x , where R x  is as defined above, -di-C 1  to C 6  alkyl-amino optionally substituted with C 1  to C 6  alkoxy, -5 or 6 membered heterocycle optionally substituted with C 1  to C 6  alkyl, or -5 or 6 membered heteroaryl; -amide; and —NHSO 2 R x , where R x  is as defined above. 
     
     
         49 . The compound of  claim 42 , wherein R 2  is selected from the group consisting of -nitro; -hydroxy; —C 1  to C 6  alkyl, optionally substituted with one or more halogen substituents; C 1  to C 6  alkoxy optionally substituted with: -one or more halogen substituents, or -amide. 
     
     
         50 . The compound of  claim 42 , wherein R 3  is hydrogen. 
     
     
         51 . A compound selected from the group consisting of: 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
       
       or a pharmaceutically acceptable salt thereof. 
     
     
         52 . A pharmaceutical composition comprising the compound of  claim 42  or pharmaceutically acceptable salt thereof and one or more pharmaceutically acceptable excipients. 
     
     
         53 . The pharmaceutical composition of  claim 52 , further comprising one or more additional anti-viral agent selected from the group consisting of pegylated interferon, un-pegylated interferon, ribavirin or prodrugs or derivatives thereof, a glucosidase inhibitor, a protease inhibitor, a polymerase inhibitor, p7 inhibitors, an entry inhibitor, a fusion inhibitor, an anti-fibrotic, a caspase inhibitor, an inosine monophosphate dehydrogenase inhibitor, synthetic thymosin alpha 1, therapeutic vaccines, immunomodulators, a helicase inhibitor, a glycosidase inhibitor, a Toll-like receptor agonist and combinations thereof. 
     
     
         54 . A method for treating a viral infection in a subject in need thereof comprising administering an effective amount of the compound of  claim 42  or pharmaceutically acceptable salt thereof to the subject. 
     
     
         55 . The method of  claim 54 , wherein said viral infection is a Hepatitis C viral infection. 
     
     
         56 . A pharmaceutical composition comprising the compound of  claim 51  or pharmaceutically acceptable salt thereof and one or more pharmaceutically acceptable excipients. 
     
     
         57 . The pharmaceutical composition of  claim 56 , further comprising one or more additional anti-viral agent selected from the group consisting of pegylated interferon, un-pegylated interferon, ribavirin or prodrugs or derivatives thereof, a glucosidase inhibitor, a protease inhibitor, a polymerase inhibitor, p7 inhibitors, an entry inhibitor, a fusion inhibitor, an anti-fibrotic, a caspase inhibitor, an inosine monophosphate dehydrogenase inhibitor, synthetic thymosin alpha 1, therapeutic vaccines, immunomodulators, a helicase inhibitor, a glycosidase inhibitor, a Toll-like receptor agonist and combinations thereof. 
     
     
         58 . A method for treating a viral infection in a subject in need thereof comprising administering an effective amount of the compound of  claim 51  or pharmaceutically acceptable salt thereof to the subject. 
     
     
         59 . The method of  claim 58 , wherein said viral infection is a Hepatitis C viral infection.

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