US2022048922A1PendingUtilityA1

Compounds targeting prmt5

Assignee: ALIGOS THERAPEUTICS INCPriority: Apr 2, 2019Filed: Oct 28, 2021Published: Feb 17, 2022
Est. expiryApr 2, 2039(~12.7 yrs left)· nominal 20-yr term from priority
C07D 495/04C07D 513/04C07D 471/04C07D 473/26A61P 35/00A61K 31/53A61K 31/52C07D 519/00A61K 45/06C07D 487/04A61K 31/437A61K 31/519A61K 31/522C07D 473/30C07K 16/22C07D 498/04C07D 473/34
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Claims

Abstract

Provided herein are compounds of Formula (I), or pharmaceutically acceptable salts thereof, pharmaceutical compositions that include a compound described herein (including pharmaceutically acceptable salts of a compound described herein) and methods of synthesizing the same. Also provided herein are methods of treating diseases and/or conditions with a compound of Formula (I), or a pharmaceutically acceptable salt thereof.

Claims

exact text as granted — not AI-modified
1 . A compound of Formula (I), or a pharmaceutically acceptable salt thereof, having the structure: 
       
         
           
           
               
               
           
         
         wherein: 
         B 1  is an optionally substituted 
       
       
         
           
           
               
               
           
         
         , 
         wherein X 1  is CR C1 ; X 2  is CR C2 ; X 3  is CR C3 ; and R C1 , R C2 , R C3 , R C4  and R C5  are independently hydrogen or halogen or an unsubstituted C 1-4  alkyl; 
         R 1B  is hydrogen, halogen, hydroxy, an unsubstituted C 1-4  alkyl, an unsubstituted C 2-4  alkenyl, an unsubstituted C 3 -C 6  cycloalkyl, an unsubstituted C 1-4  alkoxy or NR A1 R A2 ; and 
         R A1  and R A2  are each hydrogen; 
         R 1  is hydrogen; 
         R 2A  is hydrogen; 
         R 2B  is OH or —O—C(═O)—C 1-4  alkyl; 
         R 3A  is hydrogen; 
         R 3B  is OH or —O—C(═O)—C 1-4  alkyl; 
         R 4A  is —(CR D1 R E1 )(CR D2 R E2 )n-R F1 ; 
         wherein R D1 , R E1 , R D2  and R E2  are independently selected from the group consisting of hydrogen, halogen, hydroxy and an unsubstituted C 1-3  alkyl; n is 1; and R F1  is an unsubstituted or a substituted aryl, an unsubstituted or a substituted heteroaryl or an unsubstituted or a substituted heterocyclyl; 
         R 4B  is an unsubstituted C 1-4  alkyl, 
         Z 1  is CR 5A R 5B;    
         R 5A  and R 5B  are each hydrogen. 
       
     
     
         2 .- 18 . (canceled) 
     
     
         19 . The compound of  claim 1 , wherein R 2B  is OH. 
     
     
         20 . The compound of  claim 1 , wherein R 2B  is —O—C(═O)—C 1-4  alkyl. 
     
     
         21 .- 31 . (canceled) 
     
     
         32 . The compound of  claim 1 , wherein R 3B  is OH. 
     
     
         33 . The compound of  claim 1 , wherein R 3B  is —O—C(═O)—C 1-4  alkyl. 
     
     
         34 .- 45 . (canceled) 
     
     
         46 . The compound of  claim 1 , wherein R D1 , R E1 , R D2  and R E2  are each hydrogen. 
     
     
         47 .- 56 . (canceled) 
     
     
         57 . The compound of  claim 1 , wherein R F1  is an unsubstituted or a substituted heteroaryl. 
     
     
         58 . (canceled) 
     
     
         59 . The compound of  claim 57 , wherein R F1  is pyridinyl. 
     
     
         60 . (canceled) 
     
     
         61 . The compound of  claim 59 , wherein R F1  is substituted with one, two or three substituents independently selected from the group consisting of halogen, cyano, an unsubstituted C 1-4  alkyl, an unsubstituted C 1-4  haloalkyl, an unsubstituted monocyclic C 3-6  cycloalkyl, an optionally substituted C-carboxy, an optionally substituted N-amido, amino, a mono-substituted amine, a di-substituted amine, —NH—C(═O)-unsubstituted C 1-8  alkyl, —NH—C(═O)—O-unsubstituted C 1-8  alkyl, —NH—C(═O)-unsubstituted C 3-6  cycloalkyl and —NH—C(═O)—O-unsubstituted C 3-6  cycloalkyl. 
     
     
         62 . The compound of  claim 1 , wherein R F1  is selected from the group consisting of: 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
       
     
     
         63 .- 105 . (canceled) 
     
     
         106 . The compound of  claim 1 , wherein R 4B  is CH 3 . 
     
     
         107 .- 134 . (canceled) 
     
     
         135 . The compound of  claim 1 , wherein R 1B  is NR A1 R A2 , wherein R A1  and R A2  are each hydrogen. 
     
     
         136 .- 142 . (canceled) 
     
     
         143 . The compound of  claim 1 , wherein B 1  is 
       
         
           
           
               
               
           
         
       
     
     
         144 .- 147 . (canceled) 
     
     
         148 . The compound of  claim 1 , wherein the compound is 
       
         
           
           
               
               
           
         
       
       or a pharmaceutically acceptable salt thereof. 
     
     
         149 .- 154 . (canceled) 
     
     
         155 . The compound of  claim 148 , wherein B 1  is 
       
         
           
           
               
               
           
         
       
     
     
         156 . (canceled) 
     
     
         157 . (canceled) 
     
     
         158 . The compound of  claim 148 , wherein R F1  is pyridinyl. 
     
     
         159 . (canceled) 
     
     
         160 . The compound of  claim 158 , wherein R F1  is substituted with one, two or three substituents independently selected from the group consisting of halogen, cyano, an unsubstituted C 1-4  alkyl, an unsubstituted C 1-4  haloalkyl, an unsubstituted monocyclic C 3-6  cycloalkyl, an optionally substituted C-carboxy, an optionally substituted N-amido, amino, a mono-substituted amine, a di-substituted amine, —NH—C(═O)-unsubstituted C 1-8  alkyl, —NH—C(═O)—O-unsubstituted C 1-8  alkyl, —NH—C(═O)-unsubstituted C 3-6  cycloalkyl and —NH—C(═O)—O-unsubstituted C 3-6  cycloalkyl. 
     
     
         161 . The compound of  claim 1 , wherein the compound is selected from the group consisting of: 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
       
       or a pharmaceutically acceptable salt of any of the foregoing. 
     
     
         162 . A pharmaceutical composition comprising an effective amount of a compound of  claim 1 , or a pharmaceutically acceptable salt thereof, and excipient. 
     
     
         163 - 174 . (canceled) 
     
     
         175 . A method for treating a cancer comprising administering an effective amount of a compound of  claim 1 , or a pharmaceutically acceptable salt thereof, to a subject in need thereof. 
     
     
         176 . (canceled) 
     
     
         177 . A method for modulating PRMT5 comprising contacting the PRMT5 enzyme with an effective amount of a compound of  claim 1 , or a pharmaceutically acceptable salt thereof. 
     
     
         178 . A method for inhibiting PRMT5 comprising contacting the PRMT5 enzyme Use of a compound of  claim 1 , or a pharmaceutically acceptable salt thereof. 
     
     
         179 . The method of  claim 175 , further comprises the use of an additional agent selected from the group consisting of a kinase inhibitor, a checkpoint inhibitor/modulator and an anti-VEGF antibody. 
     
     
         180 . (canceled)

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