US2023135173A1PendingUtilityA1

Novel substituted quinoline-8-carbonitrile derivatives having androgen receptor degradation activity and uses thereof

Assignee: ACCUTAR BIOTECHNOLOGY INCPriority: Sep 23, 2019Filed: Oct 24, 2022Published: May 4, 2023
Est. expirySep 23, 2039(~13.2 yrs left)· nominal 20-yr term from priority
C07D 403/14A61P 35/00C07D 401/14A61K 31/506A61K 31/4709A61K 31/496A61K 31/501
75
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Claims

Abstract

The present disclosure relates to novel compounds, pharmaceutical compositions containing such compounds, and their use in prevention and treatment of cancer and related diseases and conditions. In some embodiments, the compounds disclosed herein exhibit androgen receptor degradation activity.

Claims

exact text as granted — not AI-modified
What is claimed is: 
     
         1 . A compound of Formula (1) or a pharmaceutically acceptable salt thereof: 
       
         
           
           
               
               
           
         
       
       wherein:
 X 1  is CR 1  or N; 
 X 2  is CR 2  or N; 
 X 3  is CR 3  or N; 
 X 4  is CR 4  or N; 
 each of R 1 , R 2 , R 3 , and R 4  is independently selected from hydrogen, halogen, C 1 -C 3 alkoxy, and C 1 -C 3 haloalkyl, each of which is substituted with 0, 1, 2, or 3 R S ; 
 each R 5  is independently selected from halogen, hydroxyl, C 1 -C 3 alkyl, C 1 -C 3 alkoxy, C 1 -C 3 haloalkyl, —N(R 9 ) 2 , and —CN, each of which is substituted with 0, 1, 2, or 3 R S ; 
 each R 6  is independently selected from hydrogen, halogen, C 1 -C 3 alkyl, and C 1 -C 3 haloalkyl, each of which is substituted with 0, 1, 2, or 3 R S , or two R 6  groups are taken together to form an oxo; 
 each R 7  is independently selected from halogen, hydroxyl, C 1 -C 3 alkyl, C 1 -C 3 alkoxy, C 1 -C 3 haloalkyl, —N(R 9 ) 2 , and —CN, each of which is substituted with 0, 1, 2, or 3 R S ; 
 each R 8  is independently selected from hydrogen, hydroxyl, C 1 -C 3 alkyl, and C 1 -C 3 haloalkyl, each of which is substituted with 0, 1, 2, or 3 R S , or two R 8  groups are taken together to form an oxo; 
 each R 9  is independently selected from hydrogen, C 1 -C 3 alkyl, —C(═O)—(C 1 -C 3 alkyl), —C(═O)—O—(C 1 -C 3 alkyl), and —C(═O)—NH—(C 1 -C 3 alkyl), each of which is substituted with 0, 1, 2, or 3 R S , or two R 9  groups are taken together to form a 3- to 6-membered heterocycle or heteroaryl; 
 each R S  is independently selected from halogen, hydroxyl, C 1 -C 3 alkyl, C 1 -C 3 alkoxy, C 1 -C 3 haloalkyl, —N(R 9 ) 2 , and —CN; 
 L is a linker of 1 to 16 carbon atoms in length, wherein one or more carbon atoms are optionally replaced by C(O), O, N(R 9 ), S, C 2 -alkenyl, C 2 -alkynyl, cycloalkyl, aryl, heterocycle, or heteroaryl, wherein the R 9 , C 2 -alkenyl, cycloalkyl, aryl, heterocycle, and heteroaryl are each independently substituted with 0, 1, 2, or 3 R S ; 
 m is 0, 1, or 2; 
 n is 0, 1, 2, or 3; and 
 o is 0, 1, 2, or 3, 
 wherein each hydrogen atom is independently and optionally replaced by a deuterium atom. 
 
     
     
         2 . The compound or pharmaceutically acceptable salt thereof according to  claim 1 , wherein X 1  is N. 
     
     
         3 . The compound or pharmaceutically acceptable salt thereof according to  claim 1  or  2 , wherein X 2  is N. 
     
     
         4 . The compound or pharmaceutically acceptable salt thereof according to  claim 1 , wherein X 1  and X 2  are each N. 
     
     
         5 . The compound or pharmaceutically acceptable salt thereof according to  claim 1  or  2 , wherein X 2  is CR 2 , X 3  is CR 3 , and X 4  is CR 4 . 
     
     
         6 . The compound or pharmaceutically acceptable salt thereof according to  claim 5 , wherein R 2 , R 3 , and R 4  are each independently selected from H and F. 
     
     
         7 . The compound or pharmaceutically acceptable salt thereof according to  claim 1 , wherein X 1  is CR 1 , X 2  is CR 2 , X 3  is CR 3 , and X 4  is CR 4 . 
     
     
         8 . The compound or pharmaceutically acceptable salt thereof according to  claim 7 , wherein R 1 , R 2 , R 3 , and R 4  are each independently selected from H and F. 
     
     
         9 . The compound or pharmaceutically acceptable salt thereof according to  claim 7  or  8 , wherein R 1  is F. 
     
     
         10 . The compound or pharmaceutically acceptable salt thereof according to  claim 7  or  8 , wherein R 2  is F. 
     
     
         11 . The compound or pharmaceutically acceptable salt thereof according to  claim 7  or  8 , wherein R 3  is F. 
     
     
         12 . The compound or pharmaceutically acceptable salt thereof according to  claim 7  or  8 , wherein R 4  is F. 
     
     
         13 . The compound or pharmaceutically acceptable salt thereof according to  claim 7  or  8 , wherein R 1  and R 3  are each F. 
     
     
         14 . The compound or pharmaceutically acceptable salt thereof according to  claim 7  or  8 , wherein R 3  and R 4  are each F. 
     
     
         15 . The compound or pharmaceutically acceptable salt thereof according to  claim 9 , wherein R 2 , R 3 , and R 4  are each H. 
     
     
         16 . The compound or pharmaceutically acceptable salt thereof according to  claim 10 , wherein R 1 , R 3 , and R 4  are each H. 
     
     
         17 . The compound or pharmaceutically acceptable salt thereof according to  claim 11 , wherein R 1 , R 2 , and R 4  are each H. 
     
     
         18 . The compound or pharmaceutically acceptable salt thereof according to  claim 12 , wherein R 1 , R 2 , and R 3  are each H. 
     
     
         19 . The compound or pharmaceutically acceptable salt thereof according to  claim 13 , wherein R 2  and R 4  are each H. 
     
     
         20 . The compound or pharmaceutically acceptable salt thereof according to  claim 14 , wherein R 1  and R 2  are each H. 
     
     
         21 . The compound or pharmaceutically acceptable salt thereof according to  claim 1 , wherein the 
       
         
           
           
               
               
           
         
       
       group is selected from 
       
         
           
           
               
               
           
         
       
     
     
         22 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  21 , wherein each R 5  is independently selected from halogen, C 1 -C 3 alkoxy, and C 1 -C 3 haloalkyl. 
     
     
         23 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  22 , wherein each R 5  is independently selected from —Cl, —OCH 3 , and —CF 3 . 
     
     
         24 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  23 , wherein m is 0 or 1. 
     
     
         25 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  24 , wherein m is 0. 
     
     
         26 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  25 , wherein m is 1. 
     
     
         27 . The compound or pharmaceutically acceptable salt according to any one of  claims 1  to  26 , wherein o is 0. 
     
     
         28 . The compound or pharmaceutically acceptable salt according to any one of  claims 1  to  26 , wherein o is 1. 
     
     
         29 . The compound or pharmaceutically acceptable salt according to any one of  claims 1  to  23 , wherein m and o are each 0. 
     
     
         30 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  29 , wherein each R 6  is independently selected from H and C 1 -C 3 alkyl. 
     
     
         31 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  30 , wherein each R 6  is independently selected from H and —CH 3 . 
     
     
         32 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  31 , wherein the two R 6  groups attached to the same carbon are identical. 
     
     
         33 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  31 , wherein each R 6  is identical. 
     
     
         34 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  31 , wherein each R 6  is different. 
     
     
         35 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  34 , wherein the 
       
         
           
           
               
               
           
         
       
       group is selected from 
       
         
           
           
               
               
           
         
       
     
     
         36 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  34 , wherein the 
       
         
           
           
               
               
           
         
       
       group is selected from 
       
         
           
           
               
               
           
         
       
     
     
         37 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  36 , wherein each R 7  is independently selected from halogen, hydroxyl, C 1 -C 3 alkyl, and C 1 -C 3 haloalkyl. 
     
     
         38 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  37 , wherein each R 7  is independently selected from halogen, hydroxyl, —CH 3 , and —CF 3 . 
     
     
         39 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  38 , wherein each R 7  is independently selected from F, hydroxyl, —CH 3 , and —CF 3 . 
     
     
         40 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  39 , wherein each R 7  is independently F. 
     
     
         41 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  37 , wherein n is 0. 
     
     
         42 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  37 , wherein n is 1. 
     
     
         43 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  42 , wherein each R 8  is hydrogen or two R 8  groups are taken together to form an oxo. 
     
     
         44 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  42 , wherein each R 8  is hydrogen. 
     
     
         45 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  42 , wherein two R 8  groups are taken together to form an oxo. 
     
     
         46 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  45 , wherein each R 9  is independently selected from hydrogen, C 1 -C 3 alkyl, and —C(═O)—C 1 -C 3 alkyl. 
     
     
         47 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  46 , wherein each R 9  is independently selected from hydrogen and C 1 -C 3 alkyl. 
     
     
         48 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  47 , wherein each R 9  is independently selected from hydrogen, —CH 3 , —CH 2 CH 3 , and —CH(CH 3 ) 2 . 
     
     
         49 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  36 , wherein the 
       
         
           
           
               
               
           
         
       
       group is selected from 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
       
     
     
         50 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  49 , wherein L is a linker of 1 to 12 carbon atoms in length, wherein one or more carbon atoms are optionally replaced by C(═O), O, N(R 9 ), S, C 2 -alkenyl, C 2 -alkynyl, cycloalkyl, aryl, heterocycle, or heteroaryl, wherein the R 9 , C 2 -alkenyl, cycloalkyl, aryl, heterocycle, and heteroaryl are each independently substituted with 0, 1, 2, or 3 R S . 
     
     
         51 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  50 , wherein L is a linker of 1 to 10 carbon atoms in length, wherein one or more carbon atoms are optionally replaced by C(═O), O, N(R 9 ), S, C 2 -alkenyl, C 2 -alkynyl, cycloalkyl, aryl, heterocycle, or heteroaryl, wherein the R 9 , C 2 -alkenyl, cycloalkyl, aryl, heterocycle, and heteroaryl are each independently substituted with 0, 1, 2, or 3 R S . 
     
     
         52 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  51 , wherein L is a linker of 1 to 8 carbon atoms in length, wherein one or more carbon atoms are optionally replaced by C(═O), O, N(R 9 ), S, C 2 -alkenyl, C 2 -alkynyl, cycloalkyl, aryl, heterocycle, or heteroaryl, wherein the R 9 , C 2 -alkenyl, cycloalkyl, aryl, heterocycle, and heteroaryl are each independently substituted with 0, 1, 2, or 3 R S . 
     
     
         53 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  52 , wherein L is a linker of 1 to 6 carbon atoms in length, wherein one or more carbon atoms are optionally replaced by C(═O), O, N(R 9 ), S, C 2 -alkenyl, C 2 -alkynyl, cycloalkyl, aryl, heterocycle, or heteroaryl, wherein the R 9 , C 2 -alkenyl, cycloalkyl, aryl, heterocycle, and heteroaryl are each independently substituted with 0, 1, 2, or 3 R S . 
     
     
         54 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  53 , wherein one or more carbon atoms of linker L are optionally replaced by C(═O), O, N(R 9 ), S, cycloalkyl, aryl, heterocycle, or heteroaryl, wherein the R 9 , C 2 -alkenyl, cycloalkyl, aryl, heterocycle, and heteroaryl are each independently substituted with 0, 1, 2, or 3 R S . 
     
     
         55 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  54 , wherein one or more carbon atoms of linker L are optionally replaced by O, N(R 9 ), cycloalkyl, or heterocycle, wherein the R 9 , cycloalkyl, and heterocycle are each independently substituted with 0, 1, 2, or 3 R S . 
     
     
         56 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  55 , wherein at least one carbon atom of linker L is replaced by a heterocycle, which is substituted with 0, 1, 2, or 3 R S . 
     
     
         57 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  55 , wherein at least two carbon atoms of linker L are replaced by a heterocycle, each of which is substituted with 0, 1, 2, or 3 R S . 
     
     
         58 . The compound or pharmaceutically acceptable salt thereof according to  claim 56  or  57 , wherein the heterocycle is selected from piperidine and piperazine, each of which is substituted with 0, 1, 2, or 3 R S . 
     
     
         59 . The compound or pharmaceutically acceptable salt thereof according to  claim 56  or  57 , wherein the heterocycle is selected from 
       
         
           
           
               
               
           
         
       
     
     
         60 . The compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  49 , wherein L is selected from: 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
       
     
     
         61 . The compound according to  claim 1 , wherein the compound is chosen from: 
       
         
           
                 
                 
               
                     
                 
                    1 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-((5- 
                 
                     
                   ((2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl) 
                 
                     
                   oxy)pentyl)oxy)benzamide; 
                 
                    2 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-(3- 
                 
                     
                   (3-((2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl) 
                 
                     
                   oxy)propoxy)propoxy)benzamide; 
                 
                    3 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-(2- 
                 
                     
                   (4-(2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   ethoxy)benzamide 
                 
                    4 
                   N-((1r,3r)-3-((8-oyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-(3- 
                 
                     
                   (4-(2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   propoxy)benzamide 
                 
                    5 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-(4- 
                 
                     
                   (4-(2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   butoxy)benzamide 
                 
                    6 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-((5- 
                 
                     
                   (4-(2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   pentyl)oxy)benzamide 
                 
                    7 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-6-(4- 
                 
                     
                   (2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   nicotinamide 
                 
                    8 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-(4- 
                 
                     
                   (((1r,3r)-3-((2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl) 
                 
                     
                   oxy)cyclobutyl)(methyl)amino)butoxy)benzamide 
                 
                    9 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-6-(4- 
                 
                     
                   ((((1r,3r)-3-((2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl) 
                 
                     
                   oxy)cyclobutyl)(methyl)amino)methyl)piperidin-1-yl)nicotinamide 
                 
                   10 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-6-(4- 
                 
                     
                   ((((1r,3r)-3-((2-(2,6-dioxopiperidin-3-yl)-,3-dioxoisoindolin-5-yl) 
                 
                     
                   oxy)cyclobutyl)(ethyl)amino)methyl)piperidin-1-yl)nicotinamide 
                 
                   11 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-6-(4- 
                 
                     
                   ((((1r,3r)-3-((2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl) 
                 
                     
                   oxy)cyclobutyl)(isopropyl)amino)methyl)piperidin-1-yl)nicotinamide 
                 
                   12 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-6-(4- 
                 
                     
                   ((((1s,3s)-3-((2-(2,6-dioxopipendin-3-yl)-1,3-dioxoisoindolin-5-yl) 
                 
                     
                   oxy)cyclobutyl)(isopropyl)amino)methyl)piperidin-1-yl)nicotinamide 
                 
                   13 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-6-(4- 
                 
                     
                   ((4-(2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)nicotinamide 
                 
                   14 
                   N-((1S,3S)-3-((8-cyanoquinolin-5-yl)oxy)-2,2-dimethylcyclobutyl)-6-(4-((4-(2- 
                 
                     
                   (2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)nicotinamide 
                 
                   15 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)cyclobutyl)-6-(4-((4-(2-(2,6- 
                 
                     
                   dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)piperazin-1-yl)methyl)piperidin-1-yl) 
                 
                     
                   nicotinamide 
                 
                   16 
                   N-((1s,3s)-3-((8-cyanoquinolin-5-yl)oxy)cyclobutyl)-6-(4-((4-(2-(2,6- 
                 
                     
                   dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)piperazin-1-yl)methyl)piperidin-1-yl) 
                 
                     
                   nicotinamide 
                 
                   17 
                   N-((1S,3R)-3-((8-cyanoquinolin-5-yl)oxy)-2,2-dimethylcyclobutyl)-6-(4-((4-(2- 
                 
                     
                   (2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)nicotinamide 
                 
                   18 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-2-(4- 
                 
                     
                   ((4-(2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)pyrimidine-5-carboxamide 
                 
                   19 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-6-(4- 
                 
                     
                   ((4-(2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)pyridazine-3-carboxamide 
                 
                   20 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-5-(4- 
                 
                     
                   ((4-(2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)pyrazine-2-carboxamide 
                 
                   21 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-(4- 
                 
                     
                   ((4-(2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)benzamide 
                 
                   22 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-(4- 
                 
                     
                   ((4-(2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)-3-fluorobenzamide 
                 
                   23 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-(4- 
                 
                     
                   (2-(4-(2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   ethyl)piperazin-1-yl)-3-fluorobenzamide 
                 
                   24 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-(4- 
                 
                     
                   (2-(4-(2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   ethyl)piperidin-1-yl)-3-fluorobenzamide 
                 
                   25 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-6-(4- 
                 
                     
                   (2-(4-(2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   ethyl)piperidin-1-yl)nicotinamide 
                 
                   26 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-2-(4- 
                 
                     
                   (2-(4-(2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   ethyl)piperidin-1-yl)pyrimidine-5-carboxamide 
                 
                   27 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-6-(4- 
                 
                     
                   (2-(4-(2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   ethyl)piperidin-1-yl)pyridazine-3-carboxamide 
                 
                   28 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-6-(4- 
                 
                     
                   (2-(4-(2-(2,6-dioxopipendin-3-yl)-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   ethyl)piperidin-1-yl)-5-fluoronicotinamide 
                 
                   29 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-6-(4- 
                 
                     
                   ((4-(2-((S)-2,6-dioxopiperidin-3-yl)-1-oxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)nicotinamide 
                 
                   30 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-2-(4- 
                 
                     
                   ((4-(2-((S)-2,6-dioxopipendin-3-yl)-1-oxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)pyrimidine-5-carboxamide 
                 
                   31 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-6-(4- 
                 
                     
                   ((4-(2-((S)-2,6-dioxopipendin-3-yl)-1-oxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)pyridazine-3-carboxamide 
                 
                   32 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-(4- 
                 
                     
                   ((4-(2-((S)-2,6-dioxopipendin-3-yl)-1-oxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)-3-fluorobenzamide 
                 
                   33 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-6-(4- 
                 
                     
                   ((4-(2-((S)-2,6-dioxopipendin-3-yl)-6-fluoro-1-oxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)nicotinamide 
                 
                   34 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-6-(4- 
                 
                     
                   ((4-(2-((S)-2,6-dioxopiperidin-3-yl)-6-fluoro-1-oxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)pyridazine-3-carboxamide 
                 
                   35 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-6-(4- 
                 
                     
                   ((4-(2-(2,6-dioxopiperidin-3-yl)-6-fluoro-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)pyridazine-3-carboxamide 
                 
                   36 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-6-(4- 
                 
                     
                   ((4-(2-(2,6-dioxopiperidin-3-yl)-6-fluoro-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)nicotinamide 
                 
                   37 
                   N-((1r,3S)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-6-(4- 
                 
                     
                   (((2S)-4-(2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)-2- 
                 
                     
                   methylpiperazin-1-yl)methyl)piperidin-1-yl)nicotinamide 
                 
                   38 
                   N-((1r,3R)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-6-(4- 
                 
                     
                   (((2R)-4-(2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)-2- 
                 
                     
                   methylpiperazin-1-yl)methyl)piperidin-1-yl)nicotinamide 
                 
                   39 
                   N-((1r,3S)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-(4- 
                 
                     
                   (((2S)-4-(2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)-2- 
                 
                     
                   methylpiperazin-1-yl)methyl)piperidin-1-yl)benzamide 
                 
                   40 
                   N-((1r,3R)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-(4- 
                 
                     
                   (((2R)-4-(2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)-2- 
                 
                     
                   methylpiperazin-1-yl)methyl)piperidin-1-yl)benzamide 
                 
                   41 
                   N-((1r,3R)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-(4- 
                 
                     
                   (((2R)-4-(2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)-2- 
                 
                     
                   methylpiperazin-1-yl)methyl)piperidin-1-yl)benzamide 
                 
                   42 
                   N-((1r,3R)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-(4- 
                 
                     
                   (((2R)-2-((dimethylamino)methyl)-4-(2-(2,6-dioxopiperidin-3-yl)-1,3- 
                 
                     
                   dioxoisoindolin-5-yl)piperazin-1-yl)methyl)piperidin-1-yl)-3-fluorobenzamide 
                 
                   43 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-(4- 
                 
                     
                   (2-(4-(2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   ethyl)piperidin-1-yl)benzamide 
                 
                   44 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-6-(4- 
                 
                     
                   ((((1r,3r)-3-((2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl) 
                 
                     
                   oxy)cyclobutyl)(isopropyl)amino)methyl)piperidin-1-yl)pyridazine-3- 
                 
                     
                   carboxamide 
                 
                   45 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-(4- 
                 
                     
                   (((2-(dimethylamino)ethyl)((1r,3r)-3-((2-(2,6-dioxopiperidin-3-yl)-1,3- 
                 
                     
                   dioxoisoindolin-5-yl)oxy)cyclobutyl)amino)methyl)piperidin-1-yl)-3- 
                 
                     
                   fluorobenzamide 
                 
                   46 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-6-(4- 
                 
                     
                   ((4-(2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)-5-fluoronicotinamide 
                 
                   47 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-(4- 
                 
                     
                   ((4-(2-(2,6-dioxopiperidin-3-yl)-6-fluoro-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)benzamide 
                 
                   48 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-(4- 
                 
                     
                   ((4-(2-(2,6-dioxopiperidin-3-yl)-6-fluoro-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)-3-fluorobenzamide 
                 
                   49 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-(4- 
                 
                     
                   ((4-(2-((S)-2,6-dioxopiperidin-3-yl)-1-oxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)benzamide 
                 
                   50 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-2-(4- 
                 
                     
                   ((4-(2-(2,6-dioxopiperidin-3-yl)-6-fluoro-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)pyrimidine-5-carboxamide 
                 
                   51 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-(4- 
                 
                     
                   ((4-(2-(2,6-dioxopiperidin-3-yl)-1-oxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)-3-fluorobenzamide 
                 
                   52 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-6-(4- 
                 
                     
                   ((4-(2-(2,6-dioxopiperidin-3-yl)-6-fluoro-1,3-dioxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)-5-fluoronicotinamide 
                 
                   53 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-(4- 
                 
                     
                   ((4-(2-((S)-2,6-dioxopiperidin-3-yl)-6-fluoro-1-oxoisoindolin-5-yl)piperazin-1-yl) 
                 
                     
                   methyl)piperidin-1-yl)-3-fluorobenzamide 
                 
                   54 
                   N-((1r,3r)-3-((8-cyanoquinolin-5-yl)oxy)-2,2,4,4-tetramethylcyclobutyl)-4-(4- 
                 
                     
                   ((((1r,3r)-3-((2-(2,6-dioxopiperidin-3-yl)-1,3-dioxoisoindolin-5-yl) 
                 
                     
                   oxy)cyclobutyl)(ethyl)amino)methyl)piperidin-1-yl)benzamide 
                 
                     
                 
             
                
               
               
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
               
            
           
         
       
       or a pharmaceutically acceptable salt thereof, wherein each hydrogen is independently and optionally replaced by a deuterium. 
     
     
         62 . A pharmaceutical composition comprising at least one compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  61  and a pharmaceutically acceptable carrier. 
     
     
         63 . The pharmaceutical composition according to  claim 62 , wherein the compound or pharmaceutically acceptable salt thereof is present in a therapeutically effective amount. 
     
     
         64 . A method of treating cancer in a subject in need thereof, comprising administering to said subject a compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  61  or a pharmaceutical composition according to  claim 62  or  63 . 
     
     
         65 . The method according to  claim 64 , wherein the cancer is selected from prostate cancer, head and neck cancer, skin cancer, sarcoma, renal cell carcinoma, adrenocortical carcinoma, bladder cancer, lung cancer, gastric carcinoma, esophageal carcinoma, pancreatic adenocarcinoma, colorectal cancer, connective tissue cancer, glioblastoma multiforme, cervical cancer, uterine cancer, ovarian cancer, and breast cancer. 
     
     
         66 . The method according to  claim 64  or  65 , wherein the cancer is prostate cancer. 
     
     
         67 . The method according to any one of  claims 64  to  66 , wherein the cancer is androgen receptor positive. 
     
     
         68 . The method according to any one of  claims 64  to  67 , wherein the subject has been previously treated with an anti-cancer agent. 
     
     
         69 . The method according to  claim 68 , wherein the anti-cancer agent is enzalutamide, apalutamide, bicalutamide, darolutamide, flutamide, abiraterone, or a combination of any of the foregoing. 
     
     
         70 . The method according to  claim 69 , wherein the anti-cancer agent is enzalutamide. 
     
     
         71 . A use of a compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  61  or a pharmaceutical composition according to  claim 62  or  63  for treating cancer. 
     
     
         72 . The use according to  claim 71 , wherein the cancer is selected from prostate cancer, head and neck cancer, skin cancer, sarcoma, renal cell carcinoma, adrenocortical carcinoma, bladder cancer, lung cancer, gastric carcinoma, esophageal carcinoma, pancreatic adenocarcinoma, colorectal cancer, connective tissue cancer, glioblastoma multiforme, cervical cancer, uterine cancer, ovarian cancer, and breast cancer. 
     
     
         73 . The method according to  claim 71  or  72 , wherein the cancer is prostate cancer. 
     
     
         74 . The method according to any one of  claims 71  to  73 , wherein the cancer is androgen receptor positive. 
     
     
         75 . A use of a compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  61  or a pharmaceutical composition according to  claim 62  or  63  in the manufacture of a medicament. 
     
     
         76 . The use according to  claim 75 , wherein the medicament is for the treatment of a cancer selected from prostate cancer, head and neck cancer, skin cancer, sarcoma, renal cell carcinoma, adrenocortical carcinoma, bladder cancer, lung cancer, gastric carcinoma, esophageal carcinoma, pancreatic adenocarcinoma, colorectal cancer, connective tissue cancer, glioblastoma multiforme, cervical cancer, uterine cancer, ovarian cancer, and breast cancer. 
     
     
         77 . The use according to  claim 76 , wherein the cancer is prostate cancer. 
     
     
         78 . The use according to  claim 76  or  77 , wherein the cancer is androgen receptor positive. 
     
     
         79 . A method of inhibiting cell growth, comprising contacting a cell with a compound or pharmaceutically acceptable salt thereof according to any one of  claims 1  to  61  or a pharmaceutical composition according to  claim 62  or  63 . 
     
     
         80 . The method according to  claim 79 , wherein the cell is a cancer cell. 
     
     
         81 . The method according to  claim 80 , wherein the cancer cell is a prostate cancer cell. 
     
     
         82 . The method according to any one of  claims 79  to  81 , wherein the cell is androgen receptor positive. 
     
     
         83 . The compound of Formula (1) according to  claim 1 , wherein the compound is a compound of Formula (1A)

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