US2024002388A1PendingUtilityA1

Pyrimidinone compounds and uses thereof

Assignee: HUTCHISON MEDIPHARMA LTDPriority: Aug 18, 2020Filed: Aug 17, 2021Published: Jan 4, 2024
Est. expiryAug 18, 2040(~14.1 yrs left)· nominal 20-yr term from priority
A61P 37/00A61P 35/00A61P 25/00A61P 19/02C07D 487/04A61K 45/06C07D 471/04C07D 413/12C07D 239/47C07D 403/12A61K 31/513Y02P20/55C07D 239/36A61K 31/519A61P 29/00
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Claims

Abstract

It relates to pyrimidinone compounds and uses thereof. In particular, it relates to pyrimidinone compounds of formula (I), and the pharmaceutical compositions, the preparing methods and the uses thereof, wherein the variables are as defined in the description.

Claims

exact text as granted — not AI-modified
1 . A compound of formula (I): 
       
         
           
           
               
               
           
         
         or a pharmaceutically acceptable salt thereof, or a solvate, a racemic mixture, an enantiomer, a diastereomer or a tautomer thereof, wherein 
         R 1  is hydrogen, C 1-6  alkyl, C 1-6  haloalkyl, cyano-substituted C 1-6  alkyl, —(C 1-6  alkylene) n -C 3-6  cycloalkyl, —(C 1-6  alkylene) n -phenyl, —(C 1-6  alkylene) n -4-6 membered heterocyclyl or —(C 1-6  alkylene) n -5-6 membered heteroaryl; wherein the C 3-6  cycloalkyl, phenyl, 4-6 membered heterocyclyl and 5-6 membered heteroaryl are each optionally substituted with one or more groups independently chosen from: halogen, —CN, —OH, —NH 2 , C 1-6  alkyl, C 2-6  alkenyl, C 2-6  alkynyl, C 1-6  haloalkyl, —O(C 1-6  alkyl), —O(C 1-6  haloalkyl), —NH(C 1-6  alkyl) and —N(C 1-6  alkyl) 2 ; 
         R 2  is hydrogen, halogen, —CN, —NH 2 , C 1-6  alkyl, C 1-6  haloalkyl, —O(C 1-6  alkyl), —O(C 1-6  haloalkyl), —NH(C 1-6  alkyl) or —N(C 1-6  alkyl) 2 ; 
         Z is O, NR 3  or CR 4 R 5 ; 
         R 3  is hydrogen or C 1-6  alkyl; 
         R 4  and R 5  are each independently chosen from: hydrogen, halogen, —CN, —OH, C 1-6  alkyl, C 1-6  haloalkyl, —O(C 1-6  alkyl), —O(C 1-6  haloalkyl) and C 3-6  cycloalkyl; 
       
       
         
           
           
               
               
           
         
         is phenyl or 5-6 membered heteroaryl, each of which is optionally substituted with one or more groups independently chosen from: halogen, —CN, —OH, —NH 2 , C 1-6  alkyl, C 2-6  alkenyl, C 2-6  alkynyl, C 1-6  haloalkyl, —O(C 1-6  alkyl), —O(C 1-6  haloalkyl), —NH(C 1-6  alkyl) and —N(C 1-6  alkyl) 2 ; 
       
       
         
           
           
               
               
           
         
         is 5-12 membered heteroaryl, which is optionally substituted with one or more groups independently chosen from: halogen, —CN, —OH, oxo, —NH 2 , C 1-6  alkyl, C 1-6  haloalkyl, C 2-6  alkenyl, C 2-6  alkynyl, —O(C 1-6  alkyl), —O(C 1-6  haloalkyl), —NH(C 1-6  alkyl), —N(C 1-6  alkyl) 2 , —(C 1-6  alkylene) n -C 3-6  cycloalkyl, —(C 1-6  alkylene) n -phenyl, —(C 1-6  alkylene) n -4-6 membered heterocyclyl and —(C 1-6  alkylene) n -5-6 membered heteroaryl; wherein the phenyl, C 3-6  cycloalkyl, 4-6 membered heterocyclyl and 5-6 membered heteroaryl are each optionally substituted with one or more groups independently chosen from: halogen, —CN, —OH, —NH 2 , C 1-6  alkyl, C 2-6  alkenyl, C 2-6  alkynyl, C 1-6  haloalkyl, —O(C 1-6  alkyl), —O(C 1-6  haloalkyl), —NH(C 1-6  alkyl), —N(C 1-6  alkyl) 2  and C 3-6  cycloalkyl; 
         n is 0 or 1; 
         and p is 0 or 1. 
       
     
     
         2 . (canceled) 
     
     
         3 . The compound of formula (I), or a pharmaceutically acceptable salt thereof, or a solvate, a racemic mixture, an enantiomer, a diastereomer or a tautomer thereof according to  claim 1 , wherein R 1  is C 1-6  alkyl, C 1-6  haloalkyl, cyano-substituted C 1-6  alkyl, —(C 1-6  alkylene) n -C 3-6  cycloalkyl or —(C 1-6  alkylene) n -4-6 membered heterocyclyl; wherein the C 3-6  cycloalkyl and 4-6 membered heterocyclyl are each optionally substituted with one or more groups independently chosen from: halogen and C 1-6  alkyl. 
     
     
         4 . The compound of formula (I), or a pharmaceutically acceptable salt thereof, or a solvate, a racemic mixture, an enantiomer, a diastereomer or a tautomer thereof according to  claim 3 , wherein R 1  is C 1-6  alkyl. 
     
     
         5 . The compound of formula (I), or a pharmaceutically acceptable salt thereof, or a solvate, a racemic mixture, an enantiomer, a diastereomer or a tautomer thereof according to  claim 3 , wherein R 1  is —(C 1-6  alkylene) n -C 3-6  cycloalkyl, wherein the C 3-6  cycloalkyl is optionally substituted with one or more halogen, and n is 0 or 1; or R 1  is 4-6 membered heterocyclyl, wherein the 4-6 membered heterocyclyl is oxetanyl, tetrahydrofuranyl or tetrahydropyranyl. 
     
     
         6 . The compound of formula (I), or a pharmaceutically acceptable salt thereof, or a solvate, a racemic mixture, an enantiomer, a diastereomer or a tautomer thereof according to  claim 1 , wherein R 2  is hydrogen, —NH 2  or C 1-6  alkyl. 
     
     
         7 . The compound of formula (I), or a pharmaceutically acceptable salt thereof, or a solvate, a racemic mixture, an enantiomer, a diastereomer or a tautomer thereof according to  claim 1 , wherein p is 0, and Z is CH 2 . 
     
     
         8 . The compound of formula (I), or a pharmaceutically acceptable salt thereof, or a solvate, a racemic mixture, an enantiomer, a diastereomer or a tautomer thereof according to  claim 1 , wherein 
       
         
           
           
               
               
           
         
       
       is phenyl or pyridyl, each of which is optionally substituted with one or more groups independently chosen from: halogen, C 1-6  alkyl, and C 1-6  haloalkyl. 
     
     
         9 . The compound of formula (I), or a pharmaceutically acceptable salt thereof, or a solvate, a racemic mixture, an enantiomer, a diastereomer or a tautomer thereof according to  claim 1 , wherein 
       
         
           
           
               
               
           
         
       
       is 5-9 membered heteroaryl, which is optionally substituted with one or more groups independently chosen from: halogen, C 1-6  alkyl, —(C 1-6  alkylene) n -C 3-6  cycloalkyl, —(C 1-6  alkylene) n -phenyl, —(C 1-6  alkylene) n -4-6 membered heterocyclyl and —(C 1-6  alkylene) n -5-6 membered heteroaryl; and wherein the phenyl, C 3-6  cycloalkyl, 4-6 membered heterocyclyl and 5-6 membered heteroaryl are each optionally substituted with one or more halogen. 
     
     
         10 . The compound of formula (I), or a pharmaceutically acceptable salt thereof, or a solvate, a racemic mixture, an enantiomer, a diastereomer or a tautomer thereof according to  claim 1 , wherein the compound of formula (I) is the compound of formula (I-1): 
       
         
           
           
               
               
           
         
         wherein 
         R 1  is C 1-6  alkyl, C 1-6  haloalkyl, cyano-substituted C 1-6  alkyl, —(C 1-6  alkylene) n -C 3-6  cycloalkyl or —(C 1-6  alkylene) n -4-6 membered heterocyclyl; wherein the C 3-6  cycloalkyl and 4-6 membered heterocyclyl are each optionally substituted with one or more groups independently chosen from: halogen and C 1-6  alkyl; 
         R 2  is hydrogen, —NH 2  or C 1-6  alkyl; 
       
       
         
           
           
               
               
           
         
         is 5-9 membered heteroaryl, which is optionally substituted with one or more groups independently chosen from: halogen, C 1-6  alkyl, —(C 1-6  alkylene) n -C 3-6  cycloalkyl, —(C 1-6  alkylene) n -phenyl, —(C 1-6  alkylene) n -4-6 membered heterocyclyl and —(C 1-6  alkylene) n -5-6 membered heteroaryl; wherein the phenyl, C 3-6  cycloalkyl, 4-6 membered heterocyclyl and 5-6 membered heteroaryl are each optionally substituted with one or more halogen; 
         and n is 0 or 1. 
       
     
     
         11 . The compound of formula (I), or a pharmaceutically acceptable salt thereof, or a solvate, a racemic mixture, an enantiomer, a diastereomer or a tautomer thereof according to  claim 1 , wherein 
       
         
           
           
               
               
           
         
       
       is triazolyl, oxazolyl, isoxazolyl, oxadiazolyl, pyrimidyl, pyrazolopyrimidyl, pyrazolopyridyl or dihydropyrrolotriazolyl, each of which is optionally substituted with one or more groups independently chosen from: halogen, C 1-6  alkyl, —(C 1-6  alkylene) n -C 3-6  cycloalkyl, —(C 1-6  alkylene) n -phenyl, —(C 1-6  alkylene) n -4-6 membered heterocyclyl and —(C 1-6  alkylene) n -5-6 membered heteroaryl; wherein the phenyl, C 3-6  cycloalkyl, 4-6 membered heterocyclyl and 5-6 membered heteroaryl are each optionally substituted with one or more halogen. 
     
     
         12 . The compound of formula (I), or a pharmaceutically acceptable salt thereof, or a solvate, a racemic mixture, an enantiomer, a diastereomer or a tautomer thereof according to  claim 11 , wherein 
       
         
           
           
               
               
           
         
         is chosen from 
       
       
         
           
           
               
               
           
         
         each of which is optionally substituted with one or more groups independently chosen from: halogen, C 1-6  alkyl, —(C 1-6  alkylene) n -C 3-6  cycloalkyl, —(C 1-6  alkylene) n -phenyl, —(C 1-6  alkylene) n -4-6 membered heterocyclyl and —(C 1-6  alkylene) n -5-6 membered heteroaryl; wherein the phenyl, C 3-6  cycloalkyl, 4-6 membered heterocyclyl and 5-6 membered heteroaryl are each optionally substituted with one or more halogen. 
       
     
     
         13 . The compound of formula (I), or a pharmaceutically acceptable salt thereof, or a solvate, a racemic mixture, an enantiomer, a diastereomer or a tautomer thereof according to  claim 12 , wherein 
       
         
           
           
               
               
           
         
       
       which is optionally substituted with one or more groups independently chosen from: C 1-6  alkyl, —(C 1-6  alkylene) n -C 3-6  cycloalkyl, —(C 1-6  alkylene) n -phenyl, —(C 1-6  alkylene) n -4-6 membered heterocyclyl and —(C 1-6  alkylene) n -5-6 membered heteroaryl; and wherein the C 3-6  cycloalkyl, 4-6 membered heterocyclyl and 5-6 membered heteroaryl are each optionally substituted with one or more halogen, and n is 0 or 1. 
     
     
         14 . The compound of formula (I), or a pharmaceutically acceptable salt thereof, or a solvate, a racemic mixture, an enantiomer, a diastereomer or a tautomer thereof according to  claim 13 , wherein 
       
         
           
           
               
               
           
         
         which is optionally substituted with one or more groups independently chosen from: C 1-6  alkyl; 
         or 
       
       
         
           
           
               
               
           
         
         which is optionally substituted with one or more groups independently chosen from: —(C 1-6  alkylene) n -C 3-6  cycloalkyl, wherein n is 0 or 1; wherein the C 3-6  cycloalkyl is optionally substituted with one or more halogen; 
         or 
       
       
         
           
           
               
               
           
         
         which is optionally substituted with one or more groups independently chosen from: —(C 1-6  alkylene) n -phenyl, wherein n is 0 or 1; 
         or 
       
       
         
           
           
               
               
           
         
         which is optionally substituted with one or more groups independently chosen from: 4-6 membered heterocyclyl; wherein the 4-6 membered heterocyclyl is oxetanyl; 
         or 
       
       
         
           
           
               
               
           
         
         which is optionally substituted with one or more groups independently chosen from: 5-6 membered heteroaryl; wherein the 5-6 membered heteroaryl is pyridyl. 
       
     
     
         15 . The compound of formula (I), or a pharmaceutically acceptable salt thereof according to  claim 1 , wherein the compound of formula (I) is chosen from Compounds 1-19, 22-48 and 53-95: 
       
         
           
                 
                 
               
                     
                 
                   Compound 
                     
                 
                   No. 
                   Structure 
                 
                     
                 
                    1 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                    2 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                    3 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                    4 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                    5 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                    6 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                    7 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                    8 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                    9 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   10 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   11 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   12 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   13 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   14 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   15 and 16 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                     
                   and 
                 
                     
                 
                     
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   17 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   18 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   19 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   22 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   23 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   24 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   25 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   26 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   27 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   28 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   29 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   30 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   31 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   32 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   33 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   34 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   35 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   36 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   37 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   38 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   39 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   40 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   41 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   42 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   43 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   44 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   45 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   46 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   47 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   48 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   53 and 54 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                     
                   and 
                 
                     
                 
                     
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   55 and 56 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                     
                   and 
                 
                     
                 
                     
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   57 and 58 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                     
                   and 
                 
                     
                 
                     
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   59 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   60 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   61 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   62 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   63 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   64 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   65 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   66 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   67 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   68 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   69 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   70 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   71 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   72 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   73 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   74 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   75 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   76 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   77 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   78 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   79 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   80 and 81 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                     
                   and 
                 
                     
                 
                     
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   82 and 83 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                     
                   and 
                 
                     
                 
                     
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   84 and 85 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                     
                   and 
                 
                     
                 
                     
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   86 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   87 and 88 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                     
                   and 
                 
                     
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                   89 and 90 
                     
                 
                     
                   and 
                 
                     
                 
                   91 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   92 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   93 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   94 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
                   95 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                 
                     
                 
             
                
                
                
                
               
               
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
               
            
           
         
       
     
     
         16 . A pharmaceutical composition, comprising the compound or a pharmaceutically acceptable salt thereof according to  claim 1 , and optionally comprising a pharmaceutically acceptable carrier. 
     
     
         17 . A method of in vivo or in vitro inhibiting the activity of RIPK1, comprising contacting RIPK1 with an effective amount of the compound or a pharmaceutically acceptable salt thereof according to  claim 1 . 
     
     
         18 . A method of treating a disease partially or completely mediated by RIPK1 in a subject, comprising administering to the subject an effective amount of the compound or a pharmaceutically acceptable salt thereof according to  claim 1 , wherein the disease is chosen from an autoimmune disease, an inflammatory disease, a neurodegenerative disease, and cancer. 
     
     
         19 . (canceled) 
     
     
         20 . (canceled) 
     
     
         21 . (canceled) 
     
     
         22 . (canceled) 
     
     
         23 . (canceled) 
     
     
         24 . (canceled) 
     
     
         25 . A pharmaceutical combination, comprising the compound or a pharmaceutically acceptable salt thereof according to  claim 1 , and at least one additional therapeutic agent. 
     
     
         26 . The pharmaceutical combination according to  claim 25 , wherein the therapeutic agent is an anti-inflammatory agent or an anti-neoplastic agent; and the anti-neoplastic agent is chosen from a radiotherapeutic agent, a chemotherapeutic agent, an immunotherapeutic agent and a targeted therapeutic agent.

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