US2024043414A1PendingUtilityA1

Compounds for the Treatment of Kinase-Dependent Disorders

Assignee: EXELIXIS INCPriority: Jan 26, 2018Filed: Nov 17, 2022Published: Feb 8, 2024
Est. expiryJan 26, 2038(~11.5 yrs left)· nominal 20-yr term from priority
C07D 215/48C07F 9/60Y02P20/55A61P 35/02C07D 413/12C07D 215/22C07D 401/12C07D 405/12C07D 413/10C07D 498/04A61K 31/47A61K 31/4709C07D 401/04C07D 401/06C07D 405/04C07D 413/04A61P 35/00
70
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Claims

Abstract

Disclosed herein are compounds of formula I. Compounds of formula I inhibit, regulate and/or modulate kinase receptor, particularly Axl and Mer signal transduction pathways related to the changes in cellular activities as mentioned above, compositions which contain these compounds, and methods of using them to treat kinase-dependent diseases and conditions. The present invention also provides methods for making compounds as mentioned above, and compositions which contain these compounds.

Claims

exact text as granted — not AI-modified
1 - 93 . (canceled) 
     
     
         94 . A compound of formula B-1 
       
         
           
           
               
               
           
         
       
       or a pharmaceutically acceptable salt thereof,
 R a1  is optionally substituted (C 1 -C 6 ) alkyl; 
 R 1  is 
 
       
         
           
           
               
               
           
         
          wherein “ ” indicates the point of attachment, wherein:
 Y 1  is absent; 
 Y 2  is absent or is —O—, —NH—, —NHO—, —NH—NH—, or —N—(C 1 -C 6 ) alkyl-; or 
 Y 2  is optionally substituted 
 
       
       
         
           
           
               
               
           
         
         
            wherein ring A is a 3, 4, 5, 6, or 7-membered ring, wherein “ ” indicates points of attachment, 
           Z 1  is O, NH, N—(C 1 -C 6 ) alkyl, NHO, or NO—(C 1 -C 6 ) alkyl; and
 R a  is —H, —(C 1 -C 6 ) alkyl, 4-6-membered heterocycloalkyl, 3-6-membered cycloalkyl, —(C 2 -C 6 ) alkylene-OH, —CH 2 CHOH—(C 2 -C 6 ) alkylene-OH, —(C 2 -C 6 ) alkylene-NH 2 , —(C 2 -C 6 ) alkylene-NH(C 1 -C 6 ), —(C 2 -C 6 ) alkylene-N(C 1 -C 6 ) 2 , or —(C 2 -C 6 ) alkylene-(4-6-membered heterocycloalkyl), wherein heterocycloalkyl is optionally substituted; 
 
         
         R 3  is —H or halo; 
         R 4  is —H or halo; 
         R 14  is —H or halo; 
         Y is —O—; 
         the subscript n is an integer of 1, 2, 3, or 4; 
         the subscript m is an integer of 1, 2, 3, 4, or 5; and 
         the subscript p is an integer of 0, 1, 2, 3, or 4, 
       
       wherein at each occurrence, “optionally substituted” means optionally substituted with 1, 2, 3, 4, or 5 independently selected R b  substituents;
 each R b  is independently selected from the group consisting of halo, oxo, (C 1 -C 6 ) alkyl, (C 2 -C 6 ) alkenyl, (C 2 -C 6 ) alkynyl, (C 1 -C 6 ) haloalkyl, (C 1 -C 6 ) haloalkoxy, (C 6 -C 10 ) aryl, (C 3 -C 10 ) cycloalkyl, 5-10 membered heteroaryl, 4-10 membered heterocycloalkyl, (C 6 -C 10 ) aryl-(C 1 -C 4 ) alkylene-, (C 3 -C 10 ) cycloalkyl-(C 1 -C 4 ) alkylene-, (5-10 membered heteroaryl)-(C 1 -C 4 ) alkylene-, (4-10 membered heterocycloalkyl)-(C 1 -C 4 ) alkylene-, —CN, —OH, —NH 2 , —NO 2 , —NHOR c , —OR c , —SR c , —C(O)R c , —C(O)NR c R c , —C(O)OR c , —C(O)NR c S(O) 2 R c , —OC(O)R c , —OC(O)NR c R c , —C(═NOH)R c , —C(═NOH)NR c , —C(═NCN)NR c R c , —NR c C(═NCN)NR c R c , —C(═NR c )NR c R c , —NR c C(═NR c )NR c R c , —NHR c , —NR c R c , —NR c C(O)R c , —NR c C(═NR c )R c , —NR c C(O)OR c , —NR c C(O)NR c R c , —NR c S(O)R c , —NR c S(O) 2 R c , —NR c S(O) 2 NR c R c , —S(O)R c , —S(O)NR c R c , —S(O) 2 R c , —S(O) 2 NR c C(O)R c , —Si(R c ) 3 , —P(O)R c R c , —P(O)(OR c )(OR c ), —B(OH) 2 , —B(OR c ) 2 , and —S(O) 2 NR c R c , wherein the (C 1 -C 6 ) alkyl, (C 1 -C 6 ) haloalkyl, (C 1 -C 6 ) haloalkoxy, (C 2 -C 6 ) alkenyl, (C 2 -C 6 ) alkynyl, (C 6 -C 10 ) aryl, (C 3 -C 10 ) cycloalkyl, 5-10 membered heteroaryl, 4-10 membered heterocycloalkyl, (C 6 -C 10 ) aryl-(C 1 -C 4 ) alkylene-, (C 3 -C 10 ) cycloalky-(C 1 -C 4 ) alkylene-, (5-10 membered heteroaryl)-(C 1 -C 4 ) alkylene-, and (4-10 membered heterocycloalkyl)-(C 1 -C 4 ) alkylene- of R b  are each further optionally substituted with 1, 2, or 3 independently selected R d  substituents; 
 each R c  is independently selected from the group consisting of —H, (C 1 -C 6 ) alkyl, (C 1 -C 6 ) haloalkyl, (C 2 -C 6 ) alkenyl, (C 2 -C 6 ) alkynyl, (C 6 -C 10 ) aryl, (C 3 -C 10 ) cycloalkyl, 5-10 membered heteroaryl, 4-10 membered heterocycloalkyl, (C 6 -C 10 ) aryl-(C 1 -C 4 ) alkylene-, (C 3 -C 10 ) cycloalkyl-(C 1 -C 4 ) alkylene-, (5-10 membered heteroaryl)-(C 1 -C 4 ) alkylene-, and (4-10 membered heterocycloalkyl)-(C 1 -C 4 ) alkylene-, wherein the (C 1 -C 6 ) alkyl, (C 2 -C 6 ) alkenyl, (C 2 -C 6 ) alkynyl, (C 6 -C 10 ) aryl, (C 3 -C 10 ) cycloalkyl, 5-10 membered heteroaryl, 4-10 membered heterocycloalkyl, (C 6 -C 10 ) aryl-(C 1 -C 4 ) alkylene-, (C 3 -C 10 ) cycloalkyl-(C 1 -C 4 ) alkylene-, (5-10 membered heteroaryl)-(C 1 -C 4 ) alkylene-, and (4-10 membered heterocycloalkyl)-(C 1 -C 4 ) alkylene- of R e  are each optionally substituted with 1, 2, 3, 4, or 5 independently selected R f  substituents; 
 each R d  is independently selected from the group consisting of (C 1 -C 6 ) alkyl, (C 1 -C 6 ) haloalkyl, halo, (C 6 -C 10 ) aryl, 5-10 membered heteroaryl, (C 3 -C 10 ) cycloalkyl, 4-10 membered heterocycloalkyl, (C 6 -C 10 ) aryl-(C 1 -C 4 ) alkylene-, (C 3 -C 10 ) cycloalkyl-(C 1 -C 4 ) alkylene-, (5-10 membered heteroaryl)-(C 1 -C 4 ) alkylene-, (4-10 membered heterocycloalkyl)-(C 1 -C 4 ) alkylene-, —CN, —NH 2 , —NHOR e , —OR e , —SR e , —C(O)R e , —C(O)NR e R e , —C(O)OR e , —OC(O)R e , —OC(O)NR e R e , —NHR e , —NR e R e , —NR e C(O)R e , —NR e C(O)NR e R e , —NR e C(O)OR e , —C(═NR e )NR e R e , —NR e C(═NR e )NR e R e , —NR e C(═NOH)NR e R e , —NR e C(═NCN)NR e R e , —S(O)R e , —S(O)NR e R e , —S(O) 2 R e , —NR e S(O) 2 R e , —NR e S(O) 2 NR e R e , and —S(O) 2 NR e R e , wherein the (C 1 -C 6 ) alkyl, (C 1 -C 6 ) haloalkyl, (C 6 -C 10 ) aryl, 5-10 membered heteroaryl, (C 3 -C 10 ) cycloalkyl, 4-10 membered heterocycloalkyl, (C 6 -C 10 ) aryl-(C 1 -C 4 ) alkylene-, (C 3 -C 10 ) cycloalkyl-(C 1 -C 4 ) alkylene-, (5-10 membered heteroaryl)-(C 1 -C 4 ) alkylene-, and (4-10 membered heterocycloalkyl)-(C 1 -C 4 ) alkylene- of R d  are each optionally substituted with 1, 2, or 3 independently selected R f  substituents; 
 each R e  is independently selected from the group consisting of —H, (C 1 -C 6 ) alkyl, (C 3 -C 6 ) cycloalkyl, (C 3 -C 6 ) cycloalkyl-(C 1 -C 4 ) alkylene-, (C 6 -C 10 ) aryl, (C 6 -C 10 ) aryl-(C 1 -C 4 ) alkylene-, 5- or 6-membered heteroaryl, (5- or 6-membered heteroaryl)-(C 1 -C 4 ) alkylene-, 4-7-membered heterocycloalkyl, (4-7-membered heterocycloalkyl)-(C 1 -C 4 ) alkylene-, (C 1 -C 6 ) haloalkyl, (C 1 -C 6 ) haloalkoxy, (C 2 -C 4 ) alkenyl, and (C 2 -C 4 ) alkynyl, wherein the (C 1 -C 4 ) alkyl, (C 3 -C 6 ) cycloalkyl, (C 6 -C 10 ) aryl, 5 or 6-membered heteroaryl, 4-7-membered heterocycloalkyl, (C 6 -C 10 ) aryl-(C 1 -C 4 ) alkylene-, (5- or 6-membered heteroaryl)-(C 1 -C 4 ) alkylene-, (4-7-membered heterocycloalkyl)-(C 1 -C 4 ) alkylene-, (C 2 -C 4 ) alkenyl, and (C 2 -C 4 ) alkynyl of R e  are each optionally substituted with 1, 2, or 3 R f  substituents, 
 each R f  is independently selected from the group consisting of halo, —OH, —CN, —COOH, —NH 2 , —NH—(C 1 -C 6 ) alkyl, —N((C 1 -C 6 ) alky) 2 , (C 1 -C 6 ) alkyl, (C 1 -C 6 ) alkoxy, (C 1 -C 6 ) alkylthio, (C 1 -C 6 )haloalkyl, (C 1 -C 6 )haloalkoxy, phenyl, 5-6 membered heteroaryl, 4-6 membered heterocycloalkyl, and (C 3 -C 6 ) cycloalkyl, wherein the (C 1 -C 6 ) alkyl, phenyl, (C 3 -C 6 ) cycloalkyl, 4-6 membered heterocycloalkyl, and 5-6 membered heteroaryl of R f  are each optionally substituted with 1, 2, or 3 substituents selected from the group consisting of halo, —OH, —CN, —COOH, —NH 2 , (C 1 -C 4 ) alkyl, (C 1 -C 4 ) alkoxy, (C 1 -C 4 ) haloalkyl, (C 1 -C 4 ) haloalkoxy, phenyl, (C 3 -C 10 ) cycloalkyl, 5-6 membered heteroaryl, and 4-6 membered heterocycloalkyl; 
 
       wherein heteroaryl and heterocycloalkyl each contain 1, 2, or 3 heteroatoms independently selected from the group consisting of nitrogen, sulfur, and oxygen. 
     
     
         95 . The compound of  claim 94  or a pharmaceutically acceptable salt thereof, wherein:
 R a1  is (C 1 -C 6 ) alkyl; 
 Y 1  is absent; 
 Y 2  is O, NH, NHO, NH—NH, or N—(C 1 -C 6 ) alkyl; or 
 Y 2  is optionally substituted azetidinyl; 
 Z is O, NH, or N—(C 1 -C 6 ) alkyl; and
 R a  is H, (C 1 -C 6 ) alkyl, —(C 2 -C 6 ) alkylene-OH, —CH 2 CHOH—(C 2 -C 6 ) alkylene-OH, —(C 2 -C 6 ) alkylene-NH 2 , —(C 2 -C 6 ) alkylene-NH(C 1 -C 6 ) alkyl, —(C 2 -C 6 ) alkylene-N((C 1 -C 6 ) alkyl) 2 , —(C 2 -C 6 ) alkylene-heterocycloalkyl), and 4-6 membered heterocycloalkyl, wherein heterocycloalkyl is optionally substituted. 
 
 
     
     
         96 . The compound of  claim 94  or a pharmaceutically acceptable salt thereof, wherein —OR a1  is methoxy. 
     
     
         97 . The compound of  claim 94 , which is a compound of formula C: 
       
         
           
           
               
               
           
         
       
       or a pharmaceutically acceptable salt thereof, wherein:
 Y 1  is absent; 
 Y 2  is O, NH, NHO, NH—NH, or N—(C 1 -C 6 ) alkyl; or 
 Y 2  is optionally substituted azetidinyl; 
 Z 1  is O, NH, NO—(C 1 -C 6 ) alkyl, or N—(C 1 -C 6 ) alkyl; 
 R a  is H, (C 1 -C 6 ) alkyl, —(C 2 -C 6 ) alkylene-OH, —CH 2 CHOH—(C 2 -C 6 ) alkylene-OH, —(C 2 -C 6 ) alkylene-NH 2 , —(C 2 -C 6 ) alkylene-NH(C 1 -C 6 ) alkyl, —(C 2 -C 6 ) alkylene-N((C 1 -C 6 ) alkyl) 2 , —(C 2 -C 6 ) alkylene-optionally substituted 4-6 membered heterocycloalkyl, or optionally substituted 4-6 membered heterocycloalkyl; 
 R 2  is (C 1 -C 6 )alkoxy; and 
 n and m are each independently integers of 0 to 3. 
 
     
     
         98 . The compound of  claim 97  or a pharmaceutically acceptable salt thereof, wherein:
 Y 1  is absent; 
 Y 2  is O, NH, NHO, NH—NH, or N—(C 1 -C 6 ) alkyl; or 
 Y 2  is optionally substituted azetidinyl; 
 Z 1  is O, NH, NO—(C 1 -C 6 ) alkyl, or N—(C 1 -C 6 ) alkyl; 
 R a  is H, methyl, ethyl, —(C 2 -C 6 ) alkylene-OH, —CH 2 CHOH—(C 2 -C 6 ) alkylene-OH, —(C 2 -C 6 ) alkylene-NH 2 , —(C 2 -C 6 ) alkylene-NHMe, —(C 2 -C 6 ) alkylene-N(Me) 2 , —(C 1 -C 6 ) alkylene-morpholinyl, —(C 1 -C 6 ) alkylene-piperidinyl, (C 1 -C 6 )alkylene-(optionally substituted pyrrolidinyl), optionally substituted azetidinyl, or optionally substituted oxetanyl; 
 and n and m or each 0 or 1. 
 
     
     
         99 . The compound of  claim 97 , which is a compound of formula C-1. 
       
         
           
           
               
               
           
         
       
       or a pharmaceutically acceptable salt thereof, wherein:
 Y 2  is O, NH, NHO, NH—NH, or N—(C 1 -C 6 ) alkyl; or 
 Y 2  is optionally substituted azetidinyl, 
 Z 1  is O, NH, NO—(C 1 -C 6 ) alkyl, or N—(C 1 -C 6 ) alkyl; 
 R a  is H, methyl, ethyl, —(C 2 -C 6 ) alkylene-OH, —CH 2 CHOH—(C 2 -C 6 ) alkylene-OH, —(C 2 -C 6 ) alkylene-NH 2 , —(C 2 -C 6 ) alkylene-NHMe, —(C 2 -C 6 ) alkylene-N(Me) 2 , —(C 1 -C 6 ) alkylene-morpholinyl, —(C 1 -C 6 ) alkylene-piperidinyl, (C 1 -C 6 )alkylene-(optionally substituted pyrrolidinyl), optionally substituted azetidinyl, or optionally substituted oxetanyl. 
 
     
     
         100 . The compound of  claim 94 , which is a compound of formula F: 
       
         
           
           
               
               
           
         
       
       or a pharmaceutically acceptable salt thereof. 
     
     
         101 . The compound of  claim 100  or a pharmaceutically acceptable salt thereof, wherein:
 R a1  is methyl; and 
 R 1  is 
 
       
         
           
           
               
               
           
         
          wherein:
 Y 1  is absent; 
 Y 2  is —O—, —NH—, —NHO—, —NH—NH—, or N—(C 1 -C 6 ) alkyl; or 
 Y 2  is optionally substituted azetidinyl; 
 Z 1  is O, NH, or N—(C 1 -C 6 ) alkyl; and 
 R a  is H, (C 1 -C 6 ) alkyl, —(C 2 -C 6 ) alkylene-OH, —CH 2 CHOH—(C 2 -C 6 ) alkylene-OH, —(C 2 -C 6 ) alkylene-NH 2 , —(C 2 -C 6 ) alkylene-NH(C 1 -C 6 ) alkyl, —(C 2 -C 6 ) alkylene-N((C 1 -C 6 ) alkyl) 2 , —(C 2 -C 6 ) alkylene-heterocycloalkyl), and 4-6 membered heterocycloalkyl, wherein heterocycloalkyl is optionally substituted. 
 
       
     
     
         102 . The compound of  claim 94  or a pharmaceutically acceptable salt thereof, wherein R 1  is selected from the group consisting of: 
       
         
           
           
               
               
           
         
       
     
     
         103 . The compound of  claim 94  or a pharmaceutically acceptable salt thereof, wherein R 1  is selected from the group consisting of: 
       
         
           
           
               
               
           
         
       
     
     
         104 . The compound of  claim 94  which is selected from: 
       
         
           
                 
                 
                 
               
                   TABLE 1 
                 
                     
                 
                   No. 
                   Structure 
                   Name 
                 
                     
                 
                     
                 
                 
                 
                 
               
                   5 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   methyl 4-[4-[[1-[(4- fluorophenyl)carbamoyl] cyclopropanecarbonyl]amino] phenoxy]-7- methoxyquinoline-6- carboxylate 
                 
                     
                 
                   6 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   4-[4-[[1-[(4- fluorophenyl)carbamoyl] cyclopropanecarbonyl]amino] phenoxy]-7- methoxyquinoline-6- carboxylic acid 
                 
                     
                 
                   7 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N-[4-(6-carbamoyl-7- methoxyquinolin-4- yl)oxyphenyl]-1-N′-(4- fluorophenyl)cyclopropane-1,1- dicarboxamide 
                 
                     
                 
                   9 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N-[4-[6-(ethylcarbamoyl)-7- methoxyquinolin-4- yl]oxyphenyl]-1-N′-(4- fluorophenyl)cyclopropane-1,1- dicarboxamide 
                 
                     
                 
                   10 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N-[4-[6-[2- (dimethylamino)ethylcarbamoyl] 7-methoxyquinolin-4- yl]oxyphenyl]-1-N′-(4- fluorophenyl)cyclopropane-1,1- dicarboxamide 
                 
                     
                 
                   11 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N′-(4-fluorophenyl)-N-[4-[7- methoxy-6-(2-piperidin-1- ylethylcarbamoyl)quinolin-4- yl]oxyphenyl]cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   12 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N′-(4-fluorophenyl)-1-N- [4-[7-methoxy-6-(2-morpholin- 4-ylethylcarbamoyl)quinolin- 4-yl]oxyphenyl]cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   13 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N′-(4-fluorophenyl)-1-N- [4-[7-methoxy-6-(oxetan-3- ylcarbamoyl)quinolin-4- yl]oxyphenyl]cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   14 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N′-(4-fluorophenyl)-1-N- [4-[7-methoxy-6- [(1-methylazetidin-3- yl)carbamoyl]quinolin-4- yl]oxyphenyl]cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   15 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N-[4-[6-(azetidine-1- carbonyl)-7-methoxyquinolin- 4-yl]oxyphenyl]-1-N′-(4- fluorophenyl)cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   16 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N′-(4-fluorophenyl)-1-N- [4-[6-(3-hydroxyazetidine- 1-carbonyl)-7- methoxyquinolin-4- yl]oxyphenyl]cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   17 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N′-(4-fluorophenyl)-1-N- [4-[7-methoxy-6- (methoxycarbamoyl) quinolin-4- yl]oxyphenyl]cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   20 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N′-(4-fluorophenyl)-1-N- [4-[6-(hydroxycarbamoyl)-7- methoxyquinolin-4- yl]oxyphenyl]cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   21 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N′-(4-fluorophenyl)-1-N- [4-[7-methoxy-6- [[(2R)-pyrrolidin-2- yl]methylcarbamoyl]quinolin- 4-yl]oxyphenyl]cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   22 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N′-(4-fluorophenyl)-1-N- [4-[7-methoxy-6- [[(2S)-pyrrolidin-2- yl]methylcarbamoyl]quinolin- 4-yl]oxyphenyl]cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   26 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N′-(4-fluorophenyl)-1-N- [4-[7-methoxy-6-(oxetan-3- yloxycarbamoyl)quinolin-4- yl]oxyphenyl]cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   27 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N′-(4-fluorophenyl)-1-N- [4-[6- (2-hydroxyethoxycarbamoyl)-7- methoxyquinolin-4- yl]oxyphenyl]cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   30 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N-[4-[6-(2,3- dihydroxypropoxycarbamoyl)-7- methoxyquinolin-4- yl]oxyphenyl]-1-N′-(4- fluorophenyl)cyclopropane- 1,1-dicarboxamide Enantiomer 1 
                 
                     
                 
                   31 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N-[4-[6-(2,3- dihydroxypropoxycarbamoyl)-7- methoxyquinolin-4- yl]oxyphenyl]-1-N′-(4- fluorophenyl)cyclopropane- 1,1-dicarboxamide Enantiomer 2 
                 
                     
                 
                   32 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N′-(4-fluorophenyl)-1-N- [4-[6-(hydrazinecarbonyl)-7- methoxyquinolin-4- yl]oxyphenyl]cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   34 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N-[4-(6-acetyl-7- methoxyquinolin-4- yl)oxyphenyl]-1-N′-(4- fluorophenyl)cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   35 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N′-(4-fluorophenyl)-1-N- [4-[7-methoxy-6-[(E)-N- methoxy-C- methylcarbonimidoyl]quinolin- 4-yl]oxyphenyl]cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   36 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N′-(4-fluorophenyl)-1-N- [4-[7-methoxy-6- [(Z)-N-methoxy-C- methylcarbonimidoyl]quinolin- 4-yl]oxyphenyl]cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   98 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N-[4-[6-carbamoyl-7-(3- morpholin-4- ylpropoxy)quinolin-4- yl]oxyphenyl]-1-N′-(4- fluorophenyl)cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   103 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N-[4-[6-carbamoyl-7-(2- methoxyethoxy)quinolin-4- yl]oxyphenyl]-1-N′-(4- fluorophenyl)cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   106 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N-[4-[6-carbamoyl-7-(2- hydroxyethoxy)quinolin-4- yl]oxyphenyl]-1-N′-(4- fluorophenyl)cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   110 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N′-(4-fluorophenyl)-1-N- [4-[7-(2-hydroxyethoxy)-6- (methylcarbamoyl)quinolin-4- yl]oxyphenyl]cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   115 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N-[4-[6-carbamoyl-7-(2- hydroxypropoxy)quinolin-4- yl]oxyphenyl]-1-N′-(4- fluorophenyl)cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   116 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N′-(4-fluorophenyl)-1-N- [4-[7-(2-hydroxypropoxy)-6- (methylcarbamoyl)quinolin-4- yl]oxyphenyl]cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   128 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   methyl 4-[2-chloro-4-[[1-[(4- fluorophenyl)carbamoyl] cyclopropanecarbonyl] amino]phenoxy]-7- methoxyquinoline-6- carboxylate 
                 
                     
                 
                   129 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   methyl 4-[2-fluoro-4-[[1-[(4- fluorophenyl)carbamoyl] cyclopropanecarbonyl] amino]phenoxy]-7- methoxyquinoline-6- carboxylate 
                 
                     
                 
                   130 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   4-[2-chloro-4-[[1-[(4- fluorophenyl)carbamoyl] cyclopopanecarbonyl] amino]phenoxy]-7- methoxyquinoline-6- carboxylic acid 
                 
                     
                 
                   131 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   4-[2-fluoro-4-[[1-[(4- fluorophenyl)carbamoyl] cyclopropanecarbonyl] amino]phenoxy]-7- methoxyquinoline-6- carboxylic acid 
                 
                     
                 
                   132 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N′-[4-(6-carbamoyl-7- methoxyquinolin-4-yl)oxy-3- chlorophenyl]-1-N-(4- fluorophenyl)cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   133 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N′-[4-(6-carbamoyl-7- methoxyquinolin-4-yl)oxy-3- fluorophenyl]-1-N-(4- fluorophenyl)cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   134 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N′-[3-chloro-4-[7-methoxy-6 (methylcarbamoyl)quinolin-4- yl]oxyphenyl]-1-N-(4- fluorophenyl)cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   135 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N′-[3-fluoro-4-[7-methoxy-6 (methylcarbamoyl)quinolin-4- yl]oxyphenyl]-1-N-(4- fluorophenyl)cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   193 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N′-(4-fluorophenyl)-1-N- [4-[7-methoxy-6-[(E)- methoxyiminomethyl]quinolin- 4-yl]oxyphenyl]cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   264 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N′-(2-chloro-4-fluorophenyl)- 1-N-[3-fluoro-4-[7-methoxy-6- (methylcarbamoyl)quinolin-4- yl]oxyphenyl]cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
                   274 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   1-N-(4-chlorophenyl)-1-N′-[3- fluoro-4-[7-methoxy-6- (methylcarbamoyl)quinolin-4- yl]oxyphenyl]cyclopropane- 1,1-dicarboxamide 
                 
                     
                 
             
                
                
                
                
               
               
                
               
            
             
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
               
            
           
         
       
       or a pharmaceutically acceptable salt thereof. 
     
     
         105 . A compound of formula H: 
       
         
           
           
               
               
           
         
       
       or a pharmaceutically acceptable salt thereof, wherein:
 Y is O; 
 R 1  is selected from the group consisting of —CO—NR 5 R 6  and —CO 2 R 7 , 
 R 2  is optionally substituted C 1 -C 6  alkoxy; 
 R 3  is —H or halo; 
 R 4  is —H or halo; 
 R 5  and R 6  are each independently —H, optionally substituted C 1 -C 6  alkyl, or optionally substituted C 1 -C 6  alkoxy; 
 R 7  is H or optionally substituted C 1 -C 6  alkyl; 
 R 8  and R 9  are each independently H and optionally substituted C 1 -C 6  alkyl. 
 
     
     
         106 . The compound of  claim 105  or a pharmaceutically acceptable salt thereof, wherein R 3  is H. 
     
     
         107 . The compound of  claim 105  or a pharmaceutically acceptable salt thereof, wherein R 4  is halo. 
     
     
         108 . The compound of  claim 105  or a pharmaceutically acceptable salt thereof, wherein R 1  is —CO 2 H, —CO 2 -Me, —CO—NHR 6 , —CO—NH 2 , or —CO—NMeR 6 . 
     
     
         109 . The compound of  claim 105  or a pharmaceutically acceptable salt thereof, wherein R 1  is selected from the group consisting of: 
       
         
           
           
               
               
           
         
       
     
     
         110 . A process for making a compound of Formula H: 
       
         
           
           
               
               
           
         
       
       or a pharmaceutically acceptable salt thereof, comprising:
 reacting a compound of formula IV: 
 
       
         
           
           
               
               
           
         
         with a compound of formula V: 
       
       
         
           
           
               
               
           
         
         R 1  is —CO—NR 5 R 6  or —CO 2 R 7 ; 
         R 2  is optionally substituted C 1 -C 6  alkoxy; 
         R 3  is —H or halo; 
         R 4  is —H or halo; 
         R 5  and R 6  are each independently —H, optionally substituted (C 1 -C 6 ) alkyl, or optionally substituted (C 1 -C 6 ) alkoxy; 
         R 7  is —H or optionally substituted (C 1 -C 6 ) alkyl; 
         R 8  and R 9  are each independently —H and optionally substituted (C 1 -C 6 ) alkyl; and 
         Y is O. 
       
     
     
         111 . The process of  claim 110 , further comprising reacting a compound of Formula VI: 
       
         
           
           
               
               
           
         
       
       with a compound of Formula VII: 
       
         
           
           
               
               
           
         
       
       to form a compound of Formula VIII: 
       
         
           
           
               
               
           
         
       
       and reducing the compound of Formula VIII to provide a compound of Formula V, 
       wherein:
 W is halo. 
 
     
     
         112 . A pharmaceutical composition comprising a compound of  claim 94 , or a pharmaceutically acceptable salt thereof and a pharmaceutically acceptable carrier. 
     
     
         113 . A method of treating a disease, disorder, or syndrome mediated at least in part by modulating in vivo activity of a protein kinase, comprising administering to a subject in need thereof a compound of  claim 94  or a pharmaceutically acceptable salt thereof. 
     
     
         114 . The method of  claim 113 , wherein the disease, disorder, or syndrome mediated at least in part by modulating in vivo activity of a protein kinase is cancer. 
     
     
         115 . A method for inhibiting a protein kinase, the method comprising contacting the protein kinase with a compound of  claim 94  or a pharmaceutically acceptable salt thereof. 
     
     
         116 . The method of  claim 115 , wherein the protein kinase is Axl, Mer, c-Met, KDR, or a combination thereof.

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