US2025002800A1PendingUtilityA1

Marine fuel base comprising a component of renewable origin and method for manufacturing same

Assignee: TOTALENERGIES ONE TECHPriority: Nov 23, 2021Filed: Nov 21, 2022Published: Jan 2, 2025
Est. expiryNov 23, 2041(~15.3 yrs left)· nominal 20-yr term from priority
C10L 2200/0446C10L 10/00C10L 1/02C10G 2400/04C10G 9/007C10L 2270/026C10L 2200/0438C10L 1/19
26
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Claims

Abstract

A marine fuel base comprising an alkyl ester component of renewable origin, derived from fatty acids of plant or animal origin, which improves the viscosity and stability of a petroleum residuum, especially a visbroken residuum.

Claims

exact text as granted — not AI-modified
1 . Use of fatty acid alkyl esters to improve the viscosity of a component of at least one hydrocarbon residue and obtain a marine fuel base, wherein (i) 10 to 70% m/m of a first component consisting of fatty acid alkyl esters of renewable origin is mixed with (ii) 90% to 30% m/m of a second component consisting of at least one hydrocarbon residue coming from a crude oil chosen from an atmospheric residue, a vacuum residue and a visbreaking residue, and the mixture obtained forms a marine fuel base that has a kinematic viscosity at 50° C. 15 to 75% lower than a kinematic viscosity calculated according to the formula: 
       
         
           
             
               
                 
                   
                     
                       ϑ 
                       = 
                       
                         
                           exp 
                           ⁢ 
                              
                           
                             ( 
                             
                               exp 
                               ⁢ 
                                  
                               
                                 ( 
                                 
                                   
                                     
                                       V 
                                       ⁢ 
                                       
                                         B 
                                         mélange 
                                       
                                     
                                     - 
                                     23.097 
                                   
                                   33.469 
                                 
                                 ) 
                               
                             
                             ) 
                           
                         
                         - 
                         0.8 
                       
                     
                     , 
                   
                 
                 
                   
                     ( 
                     4 
                     ) 
                   
                 
               
             
           
         
         where VB mélange  is the weighted average of the viscosity indices of the first component and of the second component, these viscosity indices being calculated via the formula: 
       
       
         
           
             
               
                 
                   
                     
                       
                         V 
                         ⁢ 
                         
                           B 
                           i 
                         
                       
                       = 
                       
                         
                           2 
                           ⁢ 
                           
                             3 
                             . 
                             0 
                           
                           ⁢ 
                           9 
                           ⁢ 
                           7 
                         
                         + 
                         
                           3 
                           ⁢ 
                           
                             3 
                             . 
                             4 
                           
                           ⁢ 
                           69 
                           × 
                           ln 
                           ⁢ 
                           
                             ( 
                             
                               ln 
                               ⁢ 
                               
                                 ( 
                                 
                                   
                                     v 
                                     i 
                                   
                                   + 
                                   
                                     0 
                                     . 
                                     8 
                                   
                                 
                                 ) 
                               
                             
                             ) 
                           
                         
                       
                     
                     , 
                   
                 
                 
                   
                     ( 
                     5 
                     ) 
                   
                 
               
             
           
         
         where v i  is the kinematic viscosity of the component i expressed in stokes. 
       
     
     
         2 . Use according to  claim 1 , wherein the mixture obtained has a kinematic viscosity at 100° C. 5 to 30% lower than the calculated viscosity. 
     
     
         3 . Use according to  claim 1 , wherein the at least one hydrocarbon residue chosen from a vacuum residue and a visbreaking residue. 
     
     
         4 . Use according to  claim 1 , wherein the at least one hydrocarbon residue is a visbreaking residue. 
     
     
         5 . Use according to  claim 3 or 4 , to obtain a mixture having an S-value measured according to the standard ASTM D7157-18 (2018 Revision) greater than a calculated S-value S mélange , defined as being equal to: 
       
         
           
             
               
                 
                   
                     
                       
                         S 
                         mélange 
                       
                       = 
                       
                         
                           So 
                           mélange 
                         
                         
                           1 
                           - 
                           
                             Sa 
                             mélange 
                           
                         
                       
                     
                     , 
                   
                 
                 
                   
                     ( 
                     3 
                     ) 
                   
                 
               
             
           
         
         with, 
       
       
         
           
             
               
                 
                   
                     
                       So 
                       mélange 
                     
                     = 
                     
                       ∑ 
                          
                       
                         
                           x 
                           i 
                         
                         × 
                         S 
                         ⁢ 
                         
                           o 
                           i 
                         
                       
                     
                   
                 
                 
                   
                     ( 
                     1 
                     ) 
                   
                 
               
             
           
         
         
           
             
               
                 
                   
                     
                       
                         or 
                         ⁢ 
                             
                         
                           So 
                           mélange 
                         
                       
                       = 
                       
                         
                           Σ 
                           ⁢ 
                              
                           
                             x 
                             i 
                           
                           × 
                           
                             ( 
                             
                               
                                 1 
                                 ⁢ 
                                 0 
                                 ⁢ 
                                 0 
                               
                               - 
                               
                                 A 
                                 ⁢ 
                                 S 
                                 ⁢ 
                                 
                                   P 
                                   i 
                                 
                               
                             
                             ) 
                           
                           × 
                           S 
                           ⁢ 
                           
                             o 
                             i 
                           
                         
                         
                           Σ 
                           ⁢ 
                              
                           
                             x 
                             i 
                           
                           × 
                           
                             ( 
                             
                               
                                 1 
                                 ⁢ 
                                 0 
                                 ⁢ 
                                 0 
                               
                               - 
                               
                                 A 
                                 ⁢ 
                                 S 
                                 ⁢ 
                                 
                                   P 
                                   i 
                                 
                               
                             
                             ) 
                           
                         
                       
                     
                     , 
                   
                 
                 
                   
                     ( 
                     
                       1 
                       ⁢ 
                       bis 
                     
                     ) 
                   
                 
               
             
           
         
         
           
             
               
                 
                   
                     
                       Sa 
                       mélange 
                     
                     = 
                     
                       
                         Σ 
                         ⁢ 
                            
                         
                           x 
                           i 
                         
                         × 
                         A 
                         ⁢ 
                         S 
                         ⁢ 
                         
                           P 
                           i 
                         
                         × 
                         S 
                         ⁢ 
                         
                           a 
                           i 
                         
                       
                       
                         Σ 
                         ⁢ 
                            
                         
                           x 
                           i 
                         
                         × 
                         A 
                         ⁢ 
                         S 
                         ⁢ 
                         
                           P 
                           i 
                         
                       
                     
                   
                 
                 
                   
                     ( 
                     2 
                     ) 
                   
                 
               
             
           
         
         where: 
         the parameters So and Sa are as defined in the standard ASTM D7157-18 (2018 Revision), and 
         x i  is the mass fraction of the component i, 
         ASP i  is the content of asphaltenes (% m) of the component i, 
         So i  is the solvent power of the component i, 
         Sa i  is the peptizability of the component i, 
         and the solvent power of the first component is estimated from a correlation expressing the solvent power So of said first component according to the kinematic viscosity at 50° C., the kinematic viscosity at 100° C. and the density at 15° C. of said first component. 
       
     
     
         6 . Use according to  claim 1 , wherein the first component comprises methyl esters, ethyl esters, propyl esters and the mixtures thereof. 
     
     
         7 . Marine fuel base comprising:
 (i) 10 to 70% m/m of a first component consisting of fatty acid alkyl esters of renewable origin,   (ii) 90 to 30% m/m of a second component consisting of at least one hydrocarbon residue coming from a crude oil chosen from an atmospheric residue, a vacuum residue and a visbreaking residue,   said base having a kinematic viscosity at 50° C. 15 to 75% lower than a kinematic viscosity calculated according to the formula:   
       
         
           
             
               
                 
                   
                     ϑ 
                     = 
                     
                       
                         exp 
                         ⁢ 
                            
                         
                           ( 
                           
                             exp 
                             ⁢ 
                                
                             
                               ( 
                               
                                 
                                   
                                     V 
                                     ⁢ 
                                     
                                       B 
                                       mélange 
                                     
                                   
                                   - 
                                   23.097 
                                 
                                 33.469 
                               
                               ) 
                             
                           
                           ) 
                         
                       
                       - 
                       0.8 
                     
                   
                 
                 
                   
                     ( 
                     4 
                     ) 
                   
                 
               
             
           
         
         where VB mélange  is the weighted average of the viscosity indices of the first component and of the second component, these viscosity indices being calculated via the formula: 
       
       
         
           
             
               
                 
                   
                     
                       
                         V 
                         ⁢ 
                         
                           B 
                           i 
                         
                       
                       = 
                       
                         
                           2 
                           ⁢ 
                           
                             3 
                             . 
                             0 
                           
                           ⁢ 
                           9 
                           ⁢ 
                           7 
                         
                         + 
                         
                           3 
                           ⁢ 
                           
                             3 
                             . 
                             4 
                           
                           ⁢ 
                           69 
                           × 
                           ln 
                           ⁢ 
                           
                             ( 
                             
                               ln 
                               ⁢ 
                               
                                 ( 
                                 
                                   
                                     v 
                                     i 
                                   
                                   + 
                                   
                                     0 
                                     . 
                                     8 
                                   
                                 
                                 ) 
                               
                             
                             ) 
                           
                         
                       
                     
                     , 
                   
                 
                 
                   
                     ( 
                     5 
                     ) 
                   
                 
               
             
           
         
         where v i  is the kinematic viscosity of the component i expressed in stokes. 
       
     
     
         8 . Base according to  claim 7 , having a kinematic viscosity at 100° C. 5 to 30% lower than the calculated viscosity. 
     
     
         9 . Base according to  claim 7 , wherein the at least one hydrocarbon residue of the second component is chosen from a vacuum residue and a visbreaking residue. 
     
     
         10 . Base according to  claim 7 , wherein the at least one hydrocarbon residue of the second component is a visbreaking residue. 
     
     
         11 . Base according to  claim 9  having an S-value measured according to the standard ASTM D7157-18 (2018 Revision) greater than a calculated S-value S mélange , defined as being equal to: 
       
         
           
             
               
                 
                   
                     
                       
                         S 
                         mélange 
                       
                       = 
                       
                         
                           So 
                           mélange 
                         
                         
                           1 
                           - 
                           
                             Sa 
                             mélange 
                           
                         
                       
                     
                     , 
                   
                 
                 
                   
                     ( 
                     
                       equation 
                       ⁢ 
                           
                       3 
                     
                     ) 
                   
                 
               
             
           
         
         with, 
       
       
         
           
             
               
                 
                   
                     
                       So 
                       mélange 
                     
                     = 
                     
                       ∑ 
                          
                       
                         
                           x 
                           i 
                         
                         × 
                         S 
                         ⁢ 
                         
                           o 
                           i 
                         
                       
                     
                   
                 
                 
                   
                     ( 
                     
                       equation 
                       ⁢ 
                           
                       l 
                     
                     ) 
                   
                 
               
             
           
         
         
           
             
               
                 
                   
                     
                       
                         or 
                         ⁢ 
                             
                         
                           So 
                           mélange 
                         
                       
                       = 
                       
                         
                           Σ 
                           ⁢ 
                              
                           
                             x 
                             i 
                           
                           × 
                           
                             ( 
                             
                               
                                 1 
                                 ⁢ 
                                 0 
                                 ⁢ 
                                 0 
                               
                               - 
                               
                                 A 
                                 ⁢ 
                                 S 
                                 ⁢ 
                                 
                                   P 
                                   i 
                                 
                               
                             
                             ) 
                           
                           × 
                           S 
                           ⁢ 
                           
                             o 
                             i 
                           
                         
                         
                           Σ 
                           ⁢ 
                              
                           
                             x 
                             i 
                           
                           × 
                           
                             ( 
                             
                               
                                 1 
                                 ⁢ 
                                 0 
                                 ⁢ 
                                 0 
                               
                               - 
                               
                                 A 
                                 ⁢ 
                                 S 
                                 ⁢ 
                                 
                                   P 
                                   i 
                                 
                               
                             
                             ) 
                           
                         
                       
                     
                     , 
                   
                 
                 
                   
                     ( 
                     
                       equation 
                       ⁢ 
                           
                       l 
                       ⁢ 
                       bis 
                     
                     ) 
                   
                 
               
             
           
         
         
           
             
               
                 
                   
                     
                       Sa 
                       mélange 
                     
                     = 
                     
                       
                         Σ 
                         ⁢ 
                            
                         
                           x 
                           i 
                         
                         × 
                         A 
                         ⁢ 
                         S 
                         ⁢ 
                         
                           P 
                           i 
                         
                         × 
                         S 
                         ⁢ 
                         
                           a 
                           i 
                         
                       
                       
                         Σ 
                         ⁢ 
                            
                         
                           x 
                           i 
                         
                         × 
                         A 
                         ⁢ 
                         S 
                         ⁢ 
                         
                           P 
                           i 
                         
                       
                     
                   
                 
                 
                   
                     ( 
                     
                       equation 
                       ⁢ 
                           
                       2 
                     
                     ) 
                   
                 
               
             
           
         
       
       where:
 the parameters So and Sa are as defined in the standard ASTM D7157-18 (2018 Revision), and 
 x i  is the mass fraction of the component i, 
 ASP i  is the content of asphaltenes (% m/m) of the component i, 
 So i  is the solvent power of the component i, 
 Sa i  is the peptizability of the component i, 
 and the solvent power of the first component is estimated from a correlation expressing the solvent power So of said first component according to the kinematic viscosity at 50° C., the kinematic viscosity at 100° C. and the density at 15° C. of said first component. 
 
     
     
         12 . Base according to  claim 7 , wherein the component of fatty acid alkyl esters of renewable origin comprises methyl esters, ethyl esters, propyl esters and the mixtures thereof. 
     
     
         13 . Marine fuel comprising a base according to  claim 7 , and optionally at least one fluxant of petroleum origin. 
     
     
         14 . Method for improving the viscosity of a component of at least one hydrocarbon residue for the preparation of a marine fuel base comprising the mixture of (i) 10 to 70% m/m of a first component consisting of fatty acid alkyl esters of renewable origin with (ii) 90% to 30% m/m of a second component consisting of at least one hydrocarbon residue coming from a crude oil chosen from an atmospheric residue, a vacuum residue and a visbreaking residue, and for obtaining a mixture forming a marine fuel base that has a kinematic viscosity at 50° C. 15 to 75% lower than a kinematic viscosity calculated according to the formula: 
       
         
           
             
               
                 
                   
                     
                       ϑ 
                       = 
                       
                         
                           exp 
                           ⁢ 
                              
                           
                             ( 
                             
                               exp 
                               ⁢ 
                                  
                               
                                 ( 
                                 
                                   
                                     
                                       V 
                                       ⁢ 
                                       
                                         B 
                                         mélange 
                                       
                                     
                                     - 
                                     23.097 
                                   
                                   33.469 
                                 
                                 ) 
                               
                             
                             ) 
                           
                         
                         - 
                         0.8 
                       
                     
                     , 
                   
                 
                 
                   
                     ( 
                     4 
                     ) 
                   
                 
               
             
           
         
         where VB mélange  is the weighted average of the viscosity indices of the first component and of the second component, these viscosity indices being calculated via the formula: 
       
       
         
           
             
               
                 
                   
                     
                       
                         V 
                         ⁢ 
                         
                           B 
                           i 
                         
                       
                       = 
                       
                         
                           2 
                           ⁢ 
                           
                             3 
                             . 
                             0 
                           
                           ⁢ 
                           9 
                           ⁢ 
                           7 
                         
                         + 
                         
                           3 
                           ⁢ 
                           
                             3 
                             . 
                             4 
                           
                           ⁢ 
                           69 
                           × 
                           
                             ln 
                             ( 
                             
                               ln 
                               ⁡ 
                               ( 
                               
                                 
                                   v 
                                   i 
                                 
                                 + 
                                 
                                   0 
                                   . 
                                   8 
                                 
                               
                               ) 
                             
                             ) 
                           
                         
                       
                     
                     , 
                   
                 
                 
                   
                     ( 
                     5 
                     ) 
                   
                 
               
             
           
         
         where v i  is the kinematic viscosity of the component i expressed in stokes.

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