P
US7655641B2ExpiredUtilityPatentIndex 60

Sulfonamide derivatives as PPAR modulators

Assignee: LILLY CO ELIPriority: Feb 14, 2003Filed: Feb 10, 2004Granted: Feb 2, 2010
Est. expiryFeb 14, 2023(expired)· nominal 20-yr term from priority
Inventors:CONNER SCOTT EUGENEGOSSETT LYNN STACYGREEN JONATHAN EDWARDJONES JR WINTON DENNISMANTLO NATHAN BRYANMATTHEWS DONALD PAULMAYHUGH DANIEL RAYSMITH DARYL LYNNVANCE JENNIFER ANNWANG XIAODONGWARSHAWSKY ALAN MWINNEROSKI JR LEONARD LARRYXU YANPINGZHU GUOXIN
A61P 3/06A61P 3/10A61P 9/12A61P 9/04C07C 311/19C07C 2601/02C07C 311/29C07D 215/36C07D 263/32C07D 413/04A61K 45/06C07D 333/62C07D 213/74A61P 3/04C07C 2601/14C07C 323/49C07D 319/18C07D 307/79C07C 317/14C07C 2601/08A61K 31/00C07D 209/48C07C 323/52C07D 277/36C07D 307/82C07D 271/12C07D 409/04C07D 209/08C07D 333/34C07D 213/64C07D 213/71C07D 409/12C07D 207/08C07C 311/13C07D 231/18C07D 231/12C07C 311/17
60
PatentIndex Score
5
Cited by
41
References
19
Claims

Abstract

The present invention is directed to a compound of Formula (I): and pharmaceutically acceptable salts, solvates, hydrates or stereoisomers thereof, which are useful in treating or preventing disorders mediated by a peroxisome proliferator activated receptor (PPAR) such as syndrome X, type II diabetes, hyperglycemia, hyperlipidemia, obesity, coagaulopathy, hypertension, arteriosclerosis, and other disorders related to syndrome X and cardiovascular diseases.

Claims

exact text as granted — not AI-modified
1. A compound having a structural Formula I, 
       
         
           
           
               
               
           
         
       
       or pharmaceutically acceptable salts or stereoisomers thereof, 
       wherein: 
       
         
           
           
               
               
           
         
         E is selected from the group consisting of O, S and NR 14 ; 
         W is selected from the group consisting of 
       
       
         
           
           
               
               
           
         
          hydrogen, C 1 -C 6  alkyl, (CH 2 ) n′ C 3 -C 6  cycloalkyl, haloalkyl and acyl; 
         Q is: —C(O)OR 6  or R 6A ; 
         X is selected from the group consisting of a bond, CH 2 , O, S and S[O] p ; 
         Y is selected from the group consisting of a bond, S, CH 2  and O; 
         Z is: benzothiophene;
 wherein the benzothiophene is optionally substituted with one or more groups independently selected from R 15 ; 
 
         m and n′ are each independently selected from the group consisting of 0, 1, 2, 3 and 4; 
         n is selected from the group consisting of 0, 1, 2 and 3; 
         p is: 1 or 2; 
         r is selected from the group consisting of 1, 2, 3 and 4; 
         v is: 1 or 2; 
         R 1  is selected from the group consisting of hydrogen,
 haloalkyl, 
 C 1 -C 6  alkyl, 
 C 1 -C 6  alkyl-C 1 -C 6  alkoxy, 
 C 1 -C 6  alkyl-aryl, 
 C 2 -C 6  alkenyl, 
 C 2 -C 6  alkynyl, 
 (CH 2 ) n′ C 3 -C 6  cycloalkyl, 
 C 1 -C 6  alkoxy, 
 aryl, and 
 R 1  and R 2  together being a 5- to 8-membered heterocyclyl ring; 
 wherein alkyl, aryl, alkenyl, alkynyl, cycloalkyl and alkoxy being optionally substituted with one or more groups independently selected from R 15 ; 
 
         R 1a  and R 1b  are each independently is selected from the group consisting of
 hydrogen, 
 C 1 -C 6  alkyl, and 
 R 1  and R 1a , R 1  and R 1b , R 2  and R 1a , R 2  and R 1b  or R 1a  and R 1b  together being a 3- to 6-membered heterocyclyl or carbocyclyl ring wherein at least one of R 1a  and R 1b  is not hydrogen; 
 
         R 2  is selected from the group consisting of hydrogen,
 haloalkyl, 
 C 1 -C 6  alkyl, 
 C 1 -C 6  alkyl-C 1 -C 6  alkoxy, 
 C 1 -C 6  alkyl-aryl, 
 C 2 -C 6  alkenyl, 
 C 2 -C 6  alkynyl, 
 (CH 2 ) n′ C 3 -C 6  cycloalkyl, 
 C 1 -C 6  alkoxy, 
 aryl, and 
 R 1  and R 2  together being a 5- to 8-membered heterocyclyl ring; 
 wherein alkyl, aryl, alkenyl, alkynyl, cycloalkyl and alkoxy being optionally substituted with one or more groups independently selected from R 15 ; 
 
         R 2a  is selected from the group consisting of hydrogen, halo, C 1 -C 6  alkyl and wherein R 2  and R 2a  together being a 3- to 8-membered ring; wherein alkyl being optionally substituted with one or more groups independently selected from R 15 ; 
         R 3  is selected from the group consisting of hydrogen,
 halo, 
 cyano, 
 haloalkyl, 
 C 1 -C 6  alkyl, 
 (CH 2 ) n′ C 3 -C 6  cycloalkyl, 
 (C 1 -C 4  alkyl)-heterocyclyl, and 
 (C 1 -C 4  alkyl)-NR 7 C(O) p R 9 ; 
 wherein alkyl, cycloalkyl and heterocyclyl being optionally substituted with one or more groups independently selected from R 15 ; 
 
         R 4  and R 5  are each independently selected from the group consisting of
 hydrogen, 
 halo, 
 C 1 -C 6  alkyl 
 C 1 -C 6  alkoxy; 
 aryloxy; 
 N(R 8 ) 2 , 
 SR 8  and 
 R 4  and R 5  together being a 3- to 8-membered ring; 
 
         R 6  is selected from the group consisting of hydrogen, C 1 -C 6  alkyl and aminoalkyl; 
         R 6A  is selected from the group consisting of carboxamide, C 1 -C 3  alkylnitrile, sulfonamide, acylsulfonamide and tetrazole; 
         R 7  is selected from the group consisting of hydrogen and C 1 -C 6  alkyl; 
         R 8  and R 9  are each independently selected from the group consisting of
 hydrogen, C 1 -C 6  alkyl, aryl, heteroaryl, and heterocyclyl; 
 wherein aryl, heteroaryl and heterocyclyl being optionally substituted with one or more substituents selected from the group consisting of hydrogen, nitro, cyano, hydroxyl, halo, haloalkyl, haloalkyloxy, aryloxy, oxo, C 1 -C 6  alkyl and C 1 -C 6  alkoxy; 
 
         R 14  is selected from the group consisting of hydrogen, aryl, C 1 -C 6  alkyl, and C 1 -C 6  alkyl -COOR 6 ,
 wherein aryl and alkyl being optionally substituted with one or more groups independently selected from R 15 ; and 
 
         R 15  is selected from the group consisting of hydrogen, nitro, cyano, hydroxyl, halo, haloalkyl, haloalkyloxy, aryloxy, oxo, C 1 -C 6  alkyl, C 1 -C 6  alkoxy, (CH 2 ) n′ C 3 -C 6  cycloalkyl, N(R 8 ) 2 , NR 8 S(O) 2 R 9 , NR 8 C(O) p R 9 , C(O)NR 8 R 9 , C(O) p R 8 , SR 8 , S(O) p R 8  and S(O) 2 NR 8 R 9 . 
       
     
     
       2. The compound  claim 1 , wherein X and Y are respectively S and O; S and CH 2 ; or CH 2  and O. 
     
     
       3. The compound of  claim 1 , wherein R 1  is C 3 -C 6  alkyl or (CH 2 ) n′ C 3 -C 6  cycloalkyl; R 2  and R 3  are each independently C 1 -C 3  alkyl; and r is 1. 
     
     
       4. The compound  claim 3 , wherein X is positioned para to Y; and R 3  is positioned ortho to Y. 
     
     
       5. A compound having a structural Formula II, 
       
         
           
           
               
               
           
         
       
       or pharmaceutically acceptable salts or stereoisomers thereof, 
       wherein:
 Q is: —C(O)OR 6  or R 6A ; 
 X is selected from the group consisting of a bond, CH 2 , O, S and S[O] p ; 
 Y is selected from the group consisting of a bond, S, CH 2  and O; 
 Z is benzothiopene;
 wherein the benzothiophene is optionally substituted with one or more groups independently selected from R 15 ; 
 
 m and n′ are each independently selected from the group consisting of 0, 1, 2, 3 and 4; 
 n is selected from the group consisting of 0, 1, 2 and 3; 
 p is: 1 or 2; 
 r is selected from the group consisting of 1, 2, 3 and 4; 
 R 1  is selected from the group consisting of aryl,
 haloalkyl, 
 C 1 -C 6  alkyl, 
 C 1 -C 6  alkyl-C 1 -C 6  alkoxy, 
 C 1 -C 6  alkyl-aryl, 
 C 2 -C 6  alkenyl, 
 C 2 -C 6  alkynyl, 
 (CH 2 ) n′ C 3 -C 6  cycloalkyl, 
 C 1 -C 6  alkoxy and 
 R 1  and R 2  together being a 5- to 8-membered heterocyclyl ring; 
 wherein alkyl, aryl, alkenyl, alkynyl, cycloalkyl and alkoxy being optionally substituted with one or more groups independently selected from R 15 ; 
 
 R 1a  and R 1b  are each independently selected from the group consisting of
 hydrogen, 
 C 1 -C 6  alkyl, and, 
 R 1  and R 1a , R 1  and R 1b , R 2  and R 1a , R 2  and R 1b  or R 1a  and R 1b  together being a 3- to 6-membered heterocyclyl or carbocyclyl ring where at least one of R 1a  and R 1b  is not hydrogen; 
 
 R 2  is selected from the group consisting of hydrogen,
 haloalkyl, 
 C 1 -C 6  alkyl, 
 C 1 -C 6  alkyl-C 1 -C 6  alkoxy, 
 C 1 -C 6  alkyl-aryl, 
 C 2 -C 6  alkenyl, 
 C 2 -C 6  alkynyl, 
 (CH 2 ) n′ C 3 -C 6  cycloalkyl, 
 C 1 -C 6  alkoxy, 
 aryl, and 
 R 1  and R 2  together being a 5- to 8-membered heterocyclyl ring; 
 wherein alkyl, aryl, alkenyl, alkynyl, cycloalkyl and alkoxy being optionally substituted with one or more groups independently selected from R 15 ; 
 
 R 2a  is selected from the group consisting of hydrogen, halo or C 1 -C 6  alkyl and wherein R 2  and R 2a  together being a 3- to 8-membered ring; wherein alkyl being optionally substituted with one or more groups independently selected from R 15 ; 
 R 3  is selected from the group consisting of hydrogen,
 halo, 
 cyano, 
 haloalkyl, 
 C 1 -C 6  alkyl, 
 (CH 2 ) n′ C 3 -C 6  cycloalkyl, 
 (C 1 -C 4  alkyl)-heterocyclyl, and 
 (C 1 -C 4  alkyl)-NR 7 C(O) p R 9 ; 
 wherein alkyl, cycloalkyl and heterocyclyl being optionally substituted with one or more groups independently selected from R 15 ; 
 
 R 4  and R 5  are each independently selected from the group consisting of hydrogen,
 halo, 
 C 1 -C 6  alkyl 
 C 1 -C 6  alkoxy; 
 aryloxy; 
 N(R 8 ) 2 , 
 SR 8  and 
 R 4  and R 5  together being a 3- to 8-membered ring; 
 
 R 6  is selected from the group consisting of hydrogen, C 1 -C 6  alkyl and aminoalkyl; 
 R 6A  is selected from the group consisting of carboxamide, C 1 -C 3  alkylnitrile, sulfonamide, acylsulfonamide and tetrazole; 
 R 7  is selected from the group consisting of hydrogen and C 1 -C 6  alkyl; 
 R 8  and R 9  are each independently selected from the group consisting of
 hydrogen, C 1 -C 6  alkyl, aryl, heteroaryl, and heterocyclyl; 
 wherein aryl, heteroaryl and heterocyclyl being optionally substituted with one or more substituents selected from the group consisting of hydrogen, nitro, cyano, hydroxyl, halo, haloalkyl, haloalkyloxy, aryloxy, oxo, C 1 -C 6  alkyl and C 1 -C 6  alkoxy; 
 
 R 15  is selected from the group consisting of hydrogen, nitro, cyano, hydroxyl, halo, haloalkyl, haloalkyloxy, aryloxy, oxo, C 1 -C 6  alkyl, C 1 -C 6  alkoxy, (CH 2 ) n′ C 3 -C 6  cycloalkyl, N(R 8 ) 2 , NR 8 S(O) 2 R 9 , NR 8 C(O) p R 9 , C(O)NR 8 R 9 , C(O) p R 8 , SR 8 , S(O) p R 8  and S(O) 2 NR 8 R 9 . 
 
     
     
       6. The compound of  claim 5 , wherein X and Y are respectively S and O; S and CH 2 ; or CH 2  and O. 
     
     
       7. The compound of  claim 6 , wherein R 1  is C 3 -C 6  alkyl or (CH 2 ) n′ C 3 -C 6  cycloalkyl; R 2  and R 3  are each independently C 1 -C 3  alkyl; and r is 1. 
     
     
       8. The compound  claim 7 , wherein X is positioned para to Y; and R 3  is positioned ortho to Y. 
     
     
       9. The compound of  claim 5 , wherein the compound having a structural Formula III, 
       
         
           
           
               
               
           
         
       
       or pharmaceutically acceptable salts or stereoisomers thereof, wherein:
 n is: 1 or 2; 
 r is: 1, 2, 3, or 4; 
 X is: S or CH 2 ; 
 Y is: CH 2  or O; 
 Z is: benzothiophene; 
 wherein the benzothiophene is optionally substituted with one or more groups independently selected from R 15 ; 
 R 1  and R 2  are each independently selected from the group consisting of C 1 -C 6  alkyl and (CH 2 ) n′ C 3 -C 6  cycloalkyl; and 
 R 1a  and R 1b , R 3 , R 4  and R 5  are each independently selected from the group consisting of hydrogen and C 1 -C 6  alkyl. 
 
     
     
       10. A compound having a structural Formula VI, 
       
         
           
           
               
               
           
         
       
       or pharmaceutically acceptable salts or stereoisomers thereof, wherein:
 X is selected from the group consisting of a bond, CH 2 , O, S and S[O] p ; 
 Y is selected from the group consisting of a bond, S, CH 2  and O; 
 Z is benzothiophene; wherein the benzotihophene is optionally substituted with one or more groups selected from R 15 ; 
 n is: 0, 1, 2 or 3; 
 n′ is: 0, 1, 2, 3 or 4; 
 p is: 1 or 2; 
 r is: 1, 2, 3 or 4; 
 R 1  is selected from the group consisting of hydrogen,
 haloalkyl, 
 C 1 -C 6  alkyl, 
 C 1 -C 6  alkyl-C 1 -C 6  alkoxy, 
 C 1 -C 6  alkyl-aryl, 
 C 2 -C 6  alkenyl, 
 C 2 -C 6  alkynyl, 
 (CH 2 ) n′ C 3 -C 6  cycloalkyl, 
 C 1 -C 6  alkoxy, 
 aryl, and 
 R 1  and R 2  together being a 5- to 8-membered heterocyclyl ring; 
 wherein alkyl, aryl, alkenyl, alkynyl, cycloalkyl and alkoxy being optionally substituted with one or more groups independently selected from R 15 ; 
 
 R 1a  and R 1b  are each independently selected from the group consisting of
 hydrogen, 
 C 1 -C 6  alkyl, and 
 R 1  and R 1a , R 1  and R 1b , R 2  and R 1a , R 2  and R 1b  or R 1a  and R 1b  together being a 3- to 6-membered heterocyclyl or carbocyclyl ring; wherein at least one of R 1a  and R 1b  is not hydrogen; 
 
 R 2  is selected from the group consisting of hydrogen,
 haloalkyl, 
 C 1 -C 6  alkyl, 
 C 1 -C 6  alkyl-C 1 -C 6  alkoxy, 
 C 1 -C 6  alkyl-aryl, 
 C 2 -C 6  alkenyl, 
 C 2 -C 6  alkynyl, 
 (CH 2 ) n′ C 3 -C 6  cycloalkyl, 
 C 1 -C 6  alkoxy, 
 aryl, and 
 R 1  and R 2  together being a 5- to 8-membered heterocyclyl ring; 
 wherein alkyl, aryl, alkenyl, alkynyl, cycloalkyl and alkoxy being optionally substituted with one or more groups independently selected from R 15 ; 
 
 R 2a  is selected from the group consisting of hydrogen, halo and C 1 -C 6  alkyl; wherein R 2  and R 2a  together being a 3- to 8-membered ring; wherein alkyl being optionally substituted with one or more groups independently selected from R 15 ; 
 R 3  is selected from the group consisting of hydrogen,
 halo, 
 cyano, 
 haloalkyl, 
 C 1 -C 6  alkyl, 
 (CH 2 ) n′ C 3 -C 6  cycloalkyl, 
 (C 1 -C 4  alkyl)-heterocyclyl, and 
 (C 1 -C 4  alkyl)-NR 7 C(O) p R 9 , 
 wherein alkyl, cycloalkyl and heterocyclyl being optionally substituted with one or more groups independently selected from R 15 ; 
 
 R 6  is selected from the group consisting of hydrogen, C 1 -C 6  alkyl and aminoalkyl; 
 R 7  is selected from the group consisting of hydrogen and C 1 -C 6 alkyl; 
 R 8  and R 9  are each independently selected from the group consisting of hydrogen, C 1 -C 6  alkyl, aryl, heteroaryl, and heterocyclyl;
 wherein aryl, heteroaryl and heterocyclyl being optionally substituted with one or more substituents selected from the group consisting of hydrogen, nitro, cyano, hydroxyl, halo, haloalkyl, haloalkyloxy, aryloxy, oxo, C 1 -C 6  alkyl and C 1 -C 6  alkoxy; and 
 
 R 15  is selected from the group consisting of hydrogen, nitro, cyano, hydroxyl, halo, haloalkyl, haloalkyloxy, aryloxy, oxo, C 1 -C 6  alkyl, C 1 -C 6  alkoxy, N(R 8 ) 2 , NR 8 S(O) 2 R 9 , NR 8 C(O) p R 9 , C(O)NR 8 R 9 , C(O) p R 8 , SR 8 , S(O) p R 8  and S(O) 2 NR 8 R 9 . 
 
     
     
       11. The compound of  claim 10 , wherein the compound having a structural Formula VII, 
       
         
           
           
               
               
           
         
       
       or pharmaceutically acceptable salts or stereoisomers thereof, 
       wherein:
 q is: 1, 2, 3, or 4; 
 T is S; 
 R 10  and R 11  are each independently selected from the group consisting of hydrogen, nitro, cyano, hydroxyl, halo, haloalkyl, haloalkyloxy, aryloxy, C 1 -C 6  alkyl and C 1 -C 6  alkoxy;
 wherein alkyl, aryloxy, and alkoxy being optionally substituted with one or more groups independently selected from R 15 . 
 
 
     
     
       12. The compound of  claim 11 , wherein the compound having a structural Formula VIII, 
       
         
           
           
               
               
           
         
       
       or pharmaceutically acceptable salts or stereoisomers thereof, 
       wherein:
 q is: 1 or 2; 
 R 1  is selected from the group consisting of C 3 -C 5  alky and (CH 2 ) n′ C 3 -C 6  cycloalkyl; 
 R 2  and R 3  are each independently: C 1 -C 3  alkyl; 
 R 10  is selected from the group consisting of halo, haloalkyl and C 1 -C 3  alkyl; wherein R 10  being substituted at a position 5, or 6, or both 5 and 6 of benzothiophenyl ring; and 
 R 11  is selected from the group consisting of hydrogen and C 1 -C 6  alkyl. 
 
     
     
       13. The compound of  claim 12 , wherein R 10  is Cl, F, Br, CH 3  or CF 3  being substituted at a position 5 of benzothiophenyl ring. 
     
     
       14. A compound having a structural Formula IX, 
       
         
           
           
               
               
           
         
       
       or pharmaceutically acceptable salts or stereoisomers thereof, wherein:
 E is selected from the group consisting of O, S and NR 14 ; 
 W is selected from the group consisting of 
 
       
         
           
           
               
               
           
         
          hydrogen, C 1 -C 6  alkyl, (CH 2 ) n′ C 3 -C 6  cycloalkyl, haloalkyl and acyl; 
         Q is selected from the group consisting of —C(O)OR 6  and R 6A ; 
         X is selected from the group consisting of a bond, C, O, S and S[O] p ; 
         Y is selected from the group consisting of a bond, S, CH 2  and O; 
         Z is benzothiopene: and:
 wherein the benzothiophene is optionally substituted with one or more groups independently selected from R 15 ; 
 
         m and n′ are each independently: 0, 1, 2, 3 or 4; 
         n is: 0, 1, 2 or 3; 
         p is: 1 or 2; 
         r is: 1, 2, 3 or 4; 
         v is: 1 or 2; 
         R 1  is selected from the group consisting of hydrogen,
 haloalkyl, 
 C 1 -C 6  alkyl, 
 C 1 -C 6  alkyl-C 1 -C 6  alkoxy, 
 C 1 -C 6  alkyl-aryl, 
 C 2 -C 6  alkenyl, 
 C 2 -C 6  alkynyl, 
 (CH 2 ) n′ C 3 -C 6  cycloalkyl, 
 C 1 -C 6  alkoxy, 
 aryl, and 
 R 1  and R 2  together being a 5- to 8-membered heterocyclyl ring: 
 wherein alkyl, aryl, alkenyl, alkynyl, cycloalkyl and alkoxy being optionally substituted with one or more groups independently selected from R 15 ; 
 
         R 1a  and R 1b  are each independently selected from the group consisting of
 hydrogen, 
 C 1 -C 6  alkyl, and 
 R 1  and R 1a , R 1  and R 1b , R 2  and R 1a , R 2  and R 1b  or R 1a  and R 1b  together being a 3- to 6-membered heterocyclyl or carbocyclyl ring wherein at least one of R 1a  and R 1b  is not hydrogen; 
 
         R 2  is selected from the group consisting of hydrogen,
 haloalkyl, 
 C 1 -C 6  alkyl, 
 C 1 -C 6  alkyl-C 1 -C 6  alkoxy, 
 C 1 -C 6  alkyl-aryl, 
 C 2 -C 6  alkenyl, 
 C 2 -C 6  alkynyl, 
 (CH 2 ) n′ C 3 -C 6  cycloalkyl, 
 C 1 -C 6  alkoxy, 
 aryl, and 
 R 1  and R 2  together being a 5- to 8-membered heterocyclyl ring; 
 wherein alkyl, aryl, alkenyl, alkynyl, cycloalkyl and alkoxy being optionally substituted with one or more groups independently selected from R 15 ; 
 
         R 2a  is selected from the group consisting of hydrogen, halo and C 1 -C 6  alkyl and wherein R 2  and R 2a  together being a 3- to 8-membered ring; wherein alkyl being optionally substituted with one or more groups independently selected from R 15 ; 
         R 3  is selected from the group consisting of hydrogen,
 halo, 
 cyano, 
 haloalkyl, 
 C 1 -C 6  alkyl, 
 (CH 2 ) n′ C 3 -C 6  cycloalkyl, 
 (C 1 -C 4  alkyl)-heterocyclyl, and 
 (C 1 -C 4  alkyl)-NR 7 C(O) p R 9 : 
 wherein alkyl, cycloalkyl and heterocyclyl being optionally substituted with one or more groups independently selected from R 15 ; 
 
         R 4  and R 5  are each independently selected from the group consisting of
 hydrogen, 
 halo, 
 C 1 -C 6  alkyl 
 C 1 -C 6  alkoxy; 
 aryloxy; 
 N(R 8 ) 2 , 
 SR 8  and 
 R 4  and R 5  together being a 3- to 8-membered ring; 
 
         R 6  is selected from the group consisting of hydrogen, C 1 -C 6  alkyl and aminoalkyl; 
         R 6A  is selected from the group consisting of carboxamide, C 1 -C 3  alkylnitrile, sulfonamide, acylsulfonamide and tetrazole; 
         R 7  is selected from the group consisting of hydrogen and C 1 -C 6 alkyl; 
         R 8  and R 9  are each independently selected from the group consisting of
 hydrogen, C 1 -C 6  alkyl, aryl, heteroaryl, and heterocyclyl; 
 wherein aryl, heteroaryl and heterocyclyl being optionally substituted with one or more substituents selected from the group consisting of hydrogen, nitro, cyano, hydroxyl, halo, haloalkyl, haloalkyloxy, aryloxy, oxo, C 1 -C 6  alkyl and C 1 -C 6  alkoxy; 
 
         R 14  is selected from the group consisting of hydrogen, aryl, C 1 -C 6  alkyl, and C 1 -C 6  alkyl -COOR 6 ;
 wherein aryl and alkyl being optionally substituted with one or more groups independently selected from R 15 ; and 
 
         R 15  is selected from the group consisting of hydrogen, nitro, cyano, hydroxyl, halo, haloalkyl, haloalkyloxy, aryloxy, oxo, C 1 -C 6  alkyl, C 1 -C 6  alkoxy, (CH 2 ) n′ C 3 -C 6  cycloalkyl, N(R 8 ) 2 , NR 8 S(O) 2 R 9 , NR 8 C(O) p R 9 , C(O)NR 8 R 9 , C(O) p R 8 , SR 8 , S(O) p R 8  and S(O) 2 NR 8 R 9 . 
       
     
     
       15. The compound of  claim 14 , wherein the compound having a structural Formula X: 
       
         
           
           
               
               
           
         
       
       and pharmaceutically acceptable salts, solvates, hydrates or stereoisomers thereof, 
       wherein:
 n and q are each independently: 1, 2, 3 or 4; 
 T is S; 
 X is selected from the group consisting of CH 2 , O and S; 
 R 1  is selected from the group consisting of hydrogen, C 1 -C 6  alkyl and (CH 2 ) n′ C 3 -C 6  cycloalkyl; 
 R 1a , R 1b , R 1c  and R 2  are each independently selected from the group consisting of hydrogen and C 1 -C 6  alkyl; and 
 R 10  and R 11  are each independently selected from the group consisting of hydrogen, nitro, cyano, hydroxyl, halo, haloalkyl, haloalkyloxy, aryloxy, C 1 -C 6  alkyl and C 1 -C 6  alkoxy; wherein alkyl, alkoxy and aryloxy being optionally substituted with one or more groups selected from R 15 . 
 
     
     
       16. The compound of  claim 15 , wherein the compound having a structural Formula XI: 
       
         
           
           
               
               
           
         
       
       or pharmaceutically acceptable salts or stereoisomers thereof, wherein:
 q is 1 or 2; 
 E is selected from the group consisting of O, S and NR 14 ; 
 R 1 , R 2  and R 11  are each independently selected from the group consisting of C 1 -C 4  alkyl; 
 R 10  is selected from the group consisting of Cl, F, Br, CH 3  and CF 3 ; wherein R 10  being substituted at a position 5, or 6, or both 5 and 6 of benzothiophenyl ring; and 
 R 14  is selected from the group consisting of hydrogen, C 1 -C 6  alkyl and aryl. 
 
     
     
       17. A compound selected from the group consisting of 
       
         
           
                 
                 
                 
               
                     
                 
                   No. 
                   Structure 
                   Name 
                 
                     
                 
                     
                 
                 
                 
                 
               
                   1 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   3-(4-{2-[(5-Fluoro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-ethylsulfanyl}- 2-methyl-phenyl)- propionic acid 
                 
                     
                 
                   2 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   3-(4-{2-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-ethylsulfanyl}- 2-methyl-phenyl)- propionic acid 
                 
                     
                 
                   5 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   3-(4-{2-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-1-methyl-ethylsulfanyl}-2- methyl-phenyl)-propionic acid 
                 
                     
                 
                   6 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{2-[(5-Chloro-3- ethyl-benzo[b]thiophene-2- sulfonyl)-propyl amino]-1-methyl- ethylsulfanyl}-2- methyl-phenoxy)-acetic acid 
                 
                     
                 
                   7 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   4-{2-[(6-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-ethylsulfanyl}- 2-methyl-phenoxy)-acetic acid 
                 
                     
                 
                   8 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   4-{2-[(7-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-ethylsulfanyl}- 2-methyl-phenoxy)-acetic acid 
                 
                     
                 
                   9 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{2-[(4-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-ethylsulfanyl}- 2-methyl-phenoxy)-acetic acid 
                 
                     
                 
                   10 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{2-[(5-Chloro-3- trifluoromethyl- benzo[b]thiophene-2- sulfonyl)-propyl- amino]-ethylsulfanyl}- 2-methyl-phenoxy)-acetic acid 
                 
                     
                 
                   11 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{2-[(5-Chloro-3- trifluoromethyl- benzo[b]thiophene-2- sulfonyl)-propyl- amino]-1-methyl- ethoxy}-2-methyl- phenoxy)-acetic acid 
                 
                     
                 
                   13 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   2-(4-{2-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propy]- amino]-ethyl}- phenoxy)-2-methyl- propionic acid 
                 
                     
                 
                   14 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   2-(4-{3-[(3,5-Dimethyl- benzo[b]thiophene-2- sulfonyl)-propyl- amino]-propyl}- phenoxy)-2-methyl- propionic acid 
                 
                     
                 
                   15 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   2-(4-{3-[(5-Fluoro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-propyl}- phenoxy)-2-methyl- propionic acid 
                 
                     
                 
                   16 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   2-(4-{3-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-(2,2,2- trifluoro-ethyl)-amino]- propyl}-phenoxy)-2- methyl-propionic acid 
                 
                     
                 
                   17 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   2-(4-{2-[(3-Ethyl- benzo[b]thiophene-2- sulfonyl)-propyl- amino]-ethoxy}-3- propyl-phenoxy)-2- methyl-propionic acid 
                 
                     
                 
                   18 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   2-[4-(1-{[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-methyl}- propoxy)-2-methyl- phenoxy]-2-methyl- propionic acid 
                 
                     
                 
                   19 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   3-[4-(1-{[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-methyl}- propoxy)-2-methyl- phenyl]-propionic acid 
                 
                     
                 
                   20 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   [4-(1-{[(5-Fluoro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-methyl}- propylsulfanyl)-2- methyl-phenoxy]-acetic acid 
                 
                     
                 
                   21 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   [4-(1-{[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-methyl}- propylsulfanyl)-2- methyl-phenoxy]-acetic acid 
                 
                     
                 
                   22 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   [4-(1-{[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-methyl}- propylsulfanyl)-2- methyl-phenoxy]-acetic acid 
                 
                     
                 
                   34 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (R)-(2-Methyl-4-{1- methyl-2-[(3-methyl-5- trifluoromethyl- benzo[b]thiophene-2- sulfonyl)-propyl- amino]-ethylsulfanyl}- phenoxy)-acetic acid 
                 
                     
                 
                   35 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (R)-3-(4-{2-[(6-Chloro- 5-fluoro-3-methyl- benzo[b]thiophene-2- sulfonyl)-propyl- amino]-1-methyl- ethylsulfanyl}-2- methyl-phenyl)-propionic acid 
                 
                     
                 
                   36 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (R)-(4-{2-[(6-Chloro-5- fluoro-3-methyl- benzo[b]thiophene-2- sulfony])-propyl- amino]-1-methyl- ethylsulfanyl}-2- methyl-phenoxy)-acetic acid 
                 
                     
                 
                   79 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{2-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-ethylsulfanyl}- 2-propyl-phenoxy)-acetic acid 
                 
                     
                 
                   80 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{2-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-ethylsulfanyl}- phenoxy)-acetic acid 
                 
                     
                 
                   81 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{2-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-ethylsulfanyl}- 2-trifluoromethyl- phenoxy)-acetic acid 
                 
                     
                 
                   83 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{2-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propy]- amino]-1-methyl- ethylsulfanyl}-2- methyl-phenoxy)-acetic acid 
                 
                     
                 
                   84 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{2-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-1-methyl- ethylsulfanyl}-2- methyl-phenoxy)-acetic acid 
                 
                     
                 
                   85 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (2-Methyl-4-{2-[(3- methyl-5-trifluoromethyl- benzo[b]thiophene-2- sulfonyl)-propyl- amino]-ethylsulfanyl}- phenoxy)-acetic acid 
                 
                     
                 
                   90 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{2-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-ethylsulfanyl}- 2-methyl-phenoxy)-acetic acid 
                 
                     
                 
                   91 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{2-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-(3-methyl- butyl)-amino]- ethylsulfanyl}-2- methyl-phenoxy)-acetic acid 
                 
                     
                 
                   92 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{2-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-cyclopropyl- amino]-ethylsulfanyl}- 2-methyl-phenoxy)-acetic acid 
                 
                     
                 
                   93 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{2-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-cyclobutyl- amino]-ethylsulfanyl}- 2-methyl-phenoxy)-acetic acid 
                 
                     
                 
                   94 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{2-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-cyclopropylmethyl- amino]-ethylsulfanyl}- 2-methyl-phenoxy)-acetic acid 
                 
                     
                 
                   95 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{2-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-pentyl-amino]- ethylsulfanyl}-2- methyl-phenoxy)-acetic acid 
                 
                     
                 
                   96 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{2-[Butyl-(5-chloro- 3-methyl-benzo[b]thiophene-2- sulfonyl)-amino]- ethylsulfanyl}-2- methyl-phenoxy)-acetic acid 
                 
                     
                 
                   98 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{2-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-ethoxy}-2- methyl-phenylsulfanyl)- acetic acid 
                 
                     
                 
                   99 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{3-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-propyl}-2- methyl-phenoxy)-acetic acid 
                 
                     
                 
                   100 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{2-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-1-methyl- ethoxy}-2-methyl- phenoxy)-acetic acid 
                 
                     
                 
                   101 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   3-(4-{2-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl-amino]-1- methyl-ethoxy}-2-methyl- phenyl)-propionic acid 
                 
                     
                 
                   102 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   2-(4-{2-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-1-methyl- ethoxy}-2-methyl- phenoxy)-2-methyl- propionic acid 
                 
                     
                 
                   103 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   3-(4-{2-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-1-methyl- ethoxy}-2-methoxy- phenyl)-propionic acid 
                 
                     
                 
                   104 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{2-[(5-Fluoro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-1-methyl- ethylsulfanyl}-2- methyl-phenoxy)-acetic acid 
                 
                     
                 
                   105 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   3-(4-{2-[(5-Fluoro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-1-methyl- ethoxy}-2-methyl- phenyl)-propionic acid 
                 
                     
                 
                   106 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{2-[(5-Fluoro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-1-methyl- ethoxy}-2-methyl- phenoxy)-acetic acid 
                 
                     
                 
                   107 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (2-Chloro-4-{2-[(5- chloro-3-methyl- benzo[b]thiophene-2- sulfonyl)-propyl- amino]-ethylsulfanyl}- phenoxy)-acetic acid 
                 
                     
                 
                   108 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{2-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-ethylsulfanyl)- 2-ethyl-phenoxy)-acetic acid 
                 
                     
                 
                   112 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (R)-(3-Chloro-4-{2-[(5- chloro-3-methyl- benzo[b]thiophene-2- sulfonyl)-propyl-amino]-1- methyl-ethylsulfanyl}-phenyl)- acetic acid 
                 
                     
                 
                   113 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (3-Chloro-4-{2-[(5- chloro-3-methyl- benzo[b]thiophene-2- sulfonyl)-propyl- amino]-ethylsulfanyl}- phenyl)-acetic acid 
                 
                     
                 
                   114 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   [4-(1-{[(5-Fluoro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-methyl}- propoxy)-2-methyl- phenoxy]-acetic acid 
                 
                     
                 
                   115 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   3-[4-(1-{[(5-Fluoro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-methyl}- propoxy)-2-methyl- phenyl]-propionic acid 
                 
                     
                 
                   116 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   3-(4-{2-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-butoxy}-2- methyl-phenyl)-propionic acid 
                 
                     
                 
                   117 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   [4-(1-{[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-methyl}- propoxy)-2-methyl- phenoxy]-acetic acid 
                 
                     
                 
                   118 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   [4-(1-{[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-methyl}- propoxy)-2-methoxy- phenoxy]-acetic acid 
                 
                     
                 
                   119 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{2-[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-phenethyl- amino]-ethylsulfanyl}- 2-methyl-phenoxy)- acetic acid 
                 
                     
                 
                   120 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   (4-{2-[Benzyl-(5- chloro-3-methyl- benzo[b]thiophene-2- sulfonyl)-amino]- ethylsulfanyl}-2- methyl-phenoxy)-acetic acid 
                 
                     
                 
                   121 
                   
                     
                       
                       
                           
                           
                       
                     
                   
                   [4-(1-{[(5-Chloro-3- methyl-benzo[b]thiophene-2- sulfonyl)-propyl- amino]-methyl}- propylsulfanyl)-2- methyl-phenoxy]-acetic acid. 
                 
                     
                 
             
                
                
                
               
               
                
               
            
             
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
                
               
            
           
         
       
     
     
       18. A pharmaceutical composition comprising a pharmaceutically acceptable carrier and at least one compound of  claim 1  or pharmaceutically acceptable salts thereof. 
     
     
       19. A method for lowering blood-glucose in a mammal comprising the step of administering an effective amount of at least one compound of  claim 1 .

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