US8969363B2ActiveUtilityA1

Heterocyclic compounds and uses thereof

96
Assignee: CASTRO ALFREDO CPriority: Jul 19, 2011Filed: Jul 18, 2012Granted: Mar 3, 2015
Est. expiryJul 19, 2031(~5 yrs left)· nominal 20-yr term from priority
A61P 37/00A61P 37/06A61P 43/00A61P 35/00C07D 487/04C07D 471/04C07D 513/04C07D 473/34C07D 495/04C07D 519/00C07D 401/12A61P 29/00
96
PatentIndex Score
44
Cited by
905
References
56
Claims

Abstract

Compounds and pharmaceutical compositions that modulate kinase activity, including PI3 kinase activity, and compounds, pharmaceutical compositions, and methods of treatment of diseases and conditions associated with kinase activity, including PI3 kinase activity, are described herein.

Claims

exact text as granted — not AI-modified
What is claimed is: 
     
       1. A compound of Formula (I): 
       
         
           
           
               
               
           
         
       
       or an enantiomer, a mixture of enantiomers, or a mixture of two or more diastereomers thereof, or its pharmaceutically acceptable forms thereof, wherein
 Cy is aryl or heteroaryl substituted by 0-1 occurrences of R 3  and 0-3 occurrences of R 5 ; 
 W b   5  is CR 8 or CHR 8 ; 
 R 8  is hydrogen, alkyl, alkenyl, alkynyl, cycloalkyl, heteroalkyl, alkoxy, amido, amino, acyl, acyloxy, sulfonamido, halo, cyano, hydroxyl, or nitro; 
 B is hydrogen, alkyl, amino, heteroalkyl, cycloalkyl, heterocyclyl, heterocyclylalkyl, aryl or heteroaryl, each of which is substituted with 0-4 occurrences of R 2 ; 
 each R 2  is independently alkyl, heteroalkyl, alkenyl, alkynyl, cycloalkyl, heterocyclyl, aryl, arylalkyl, heteroaryl, heteroarylalkyl, alkoxy, amido, amino, acyl, acyloxy, alkoxycarbonyl, sulfonamido, halo, cyano, hydroxyl, nitro, phosphate, urea or carbonate; 
 X is absent or —(CH(R 9 )) z —; 
 Y is absent, —O—, —S—, —S(═O)—, —S(═O) 2 —, —N(R 9 )—, —C(═O)—(CHR 9 ) z —, —C(═O)—, —N(R 9 )—C(═O)NH—, or —N(R 9 )C(R 9 ) 2 —; 
 each z is independently an integer of 1, 2, 3, or 4; 
 R 3  is unsubstituted alkyl, or 
 R 3  is alkenyl, alkynyl, cycloalkyl, heterocyclyl, heteroalkyl, alkoxy, amido, amino, acyl, acyloxy, sulfinyl, sulfonyl, sulfoxide, sulfone, sulfonamido, halo, cyano, heteroaryl, aryl, hydroxyl, or nitro; wherein each of the above substituents can be substituted with 0, 1, 2, or 3 R 17 ; 
 each R 5  is independently unsubstituted alkyl, or 
 each R 5  is independently alkenyl, alkynyl, cycloalkyl, heteroalkyl, alkoxy, amido, amino, acyl, acyloxy, sulfonamido, halo, cyano, hydroxyl, or nitro; 
 each R 9  is independently hydrogen, alkyl, cycloalkyl, or heteroalkyl; an 
 
       
         
           
           
               
               
           
         
         W d  is 
         wherein X 1  is N or CR 14 ; 
         wherein R 10 , R 11  R 12 , R 13 , R 14 , and R 17  are independently hydrogen, alkyl, heteroalkyl, alkenyl, alkynyl, cycloalkyl, heterocyclyl, aryl, arylalkyl, heteroaryl, heteroarylalkyl, alkoxy, heterocyclyloxy, amido, amino, acyl, acyloxy, alkoxycarbonyl, sulfonamido, halo, cyano, hydroxyl, nitro, phosphate, urea, carbonate, oxo, or NR′R″ wherein R′ and R″ are taken together with nitrogen to form a cyclic moiety. 
       
     
     
       2. The compound of  claim 1 , wherein Cy is aryl substituted with 0-1 occurrences of R 3  and 0-3 occurrences of R 5 . 
     
     
       3. The compound of  claim 2 , wherein Cy is phenyl substituted with 1 occurrence of R 3  and 0 occurrences of R 5 . 
     
     
       4. The compound of  claim 3 , wherein the compound of Formula (I) has a structure of Formula (IIa) or (IIb): 
       
         
           
           
               
               
           
         
       
     
     
       5. The compound of  claim 4 , wherein the compound of Formula (I) has a structure of Formula (IIIa) or (IIIb): 
       
         
           
           
               
               
           
         
       
     
     
       6. The compound of  claim 5 , wherein the compound of Formula (I) has a structure of Formula (IIIb-1): 
       
         
           
           
               
               
           
         
       
     
     
       7. The compound of  claim 1 , wherein Cy is heteroaryl substituted with 0-1 occurrences of R 3  and 0-3 occurrences of R 5 . 
     
     
       8. The compound of  claim 7 , wherein Cy is 5-membered heteroaryl substituted with 0-1 occurrences of R 3  and 0-3 occurrences of R 5 . 
     
     
       9. The compound of  claim 8 , wherein Cy is isothiazolyl substituted with 0-1 occurrences of R 3  and 0 occurrence of R 5 . 
     
     
       10. The compound of  claim 9 , wherein the compound of Formula (I) has the structure of Formula (IVa) or Formula (IVb): 
       
         
           
           
               
               
           
         
       
     
     
       11. The compound of  claim 10 , wherein the compound of Formula (IVa) or Formula (IVb) has the structure of Formula (Va) or Formula (Vb): 
       
         
           
           
               
               
           
         
       
     
     
       12. The compound of  claim 11 , wherein the compound of Formula (I) has a structure of Formula (Va-1): 
       
         
           
           
               
               
           
         
       
     
     
       13. The compound of  claim 8 , wherein Cy is thiophenyl substituted with 0-1 occurrences of R 3  and 0 occurrence of R 5 . 
     
     
       14. The compound of  claim 13 , wherein the compound of Formula (I) has the structure of Formula (VIa) or Formula (VIb): 
       
         
           
           
               
               
           
         
       
     
     
       15. The compound of  claim 14 , wherein the compound of Formula (VIa) or Formula (VIb) has the structure of Formula (VIIa) or (VIIb): 
       
         
           
           
               
               
           
         
       
     
     
       16. The compound of  claim 14 , wherein the compound of Formula (VIa) or Formula (VIb) has the structure of Formula (VIIIa) or Formula (VIIIb): 
       
         
           
           
               
               
           
         
       
     
     
       17. The compound of  claim 16 , wherein the compound of Formula (VIIa) or Formula (VIIb) has the structure of Formula (IXa) or Formula (IXb): 
       
         
           
           
               
               
           
         
       
     
     
       18. The compound of  claim 17 , wherein the compound of Formula (I) has a structure of Formula (IXa-1): 
       
         
           
           
               
               
           
         
       
     
     
       19. The compound of  claim 1 , wherein each R 5  is independently selected from CH 3 , OCH 3 , and halo. 
     
     
       20. The compound of  claim 1 . wherein R 3  is unsubstituted alkyl or R 3  is selected from cycloalkyl, halo, aryl, and heteroaryl. 
     
     
       21. The compound of  claim 20 , wherein R 3  is selected from methyl, chloro, and pyrazolo. 
     
     
       22. The compound of  claim 1 , wherein B is aryl substituted with 0-3 occurrences of R 2 . 
     
     
       23. The compound of  claim 22 , wherein B is phenyl substituted with 0-3 occurrences of R 2 . 
     
     
       24. The compound of  claim 23 , wherein B is unsubstituted phenyl. 
     
     
       25. The compound of  claim 23 , wherein B is phenyl substituted with 1 occurrence of R 2 . 
     
     
       26. The compound of  claim 1 , wherein R 2  is halo or alkyl. 
     
     
       27. The compound of  claim 1 , wherein B is cycloalkyl. 
     
     
       28. The compound of  claim 1 , wherein B is heterocyclyl. 
     
     
       29. The compound of  claim 1 , wherein Y is absent, —O—, —N(R 9 )—, or —S(═O) 2 —. 
     
     
       30. The compound of  claim 1 , wherein X-Y is —CH 2 —N(CH 3 )—. 
     
     
       31. The compound of  claim 1 , wherein X-Y is (S)—CH(CH 3 )—NH—. 
     
     
       32. The compound of  claim 1 , wherein X-Y is (R)—CH(CH 3 )—NH—. 
     
     
       33. The compound of  claim 1 , wherein X 1  is N. 
     
     
       34. The compound of  claim 1 , wherein R 10 , R 11 , R 12 , R 13  are independently selected from hydrogen, alkyl, heteroalkyl, alkenyl, alkynyl, alkoxy, amido, amino, acyl, acyloxy, alkoxycarbonyl, sulfonamido, halo, cyano, and hydroxyl. 
     
     
       35. The compound of  claim 34 , wherein R 10 , R 11 , R 12 , and R 13  are independently selected from hydrogen, amino, and chloro. 
     
     
       36. The compound of  claim 35 , wherein R 10  is selected from amino and chloro. 
     
     
       37. The compound of  claim 1 . wherein R 8  is hydrogen. 
     
     
       38. The compound of  claim 1 , wherein the compound is 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
       
       or a pharmaceutically acceptable form thereof. 
     
     
       39. The compound of  claim 1 , wherein the compounds is 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
       
       or a pharmaceutically acceptable form thereof. 
     
     
       40. The compound of  claim 1 , wherein the compounds is 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
       
       or a pharmaceutically acceptable form thereof. 
     
     
       41. The compound of  claim 1 , wherein the compounds is 
       
         
           
           
               
               
           
         
       
       or a pharmaceutically acceptable form thereof. 
     
     
       42. The compound of  claim 1 , wherein the compounds is 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
       
       or a pharmaceutically acceptable form thereof. 
     
     
       43. The compound of  claim 1 , wherein the compounds is 
       
         
           
           
               
               
           
         
       
       or a pharmaceutically acceptable form thereof. 
     
     
       44. A compound selected from 
       
         
           
           
               
               
           
         
       
       or a pharmaceutically acceptable form thereof. 
     
     
       45. A compound selected from 
       
         
           
           
               
               
           
         
       
       or a pharmaceutically acceptable form thereof. 
     
     
       46. The compound of  claim 45 , wherein the compound is 
       
         
           
           
               
               
           
         
       
       or a pharmaceutically acceptable form thereof. 
     
     
       47. The compound of  claim 39 , wherein the compound is 
       
         
           
           
               
               
           
         
       
       or a pharmaceutically acceptable form thereof. 
     
     
       48. The compound of  claim 39 , wherein the compound is 
       
         
           
           
               
               
           
         
       
       or a pharmaceutically acceptable form thereof. 
     
     
       49. A pharmaceutical composition comprising a compound according to  claim 1  and one or more pharmaceutically acceptable excipients. 
     
     
       50. A pharmaceutical composition comprising a compound according to  claim 38  and one or more pharmaceutically acceptable excipients. 
     
     
       51. A pharmaceutical composition comprising a compound according to  claim 39  and one or more pharmaceutically acceptable excipients. 
     
     
       52. A pharmaceutical composition comprising a compound according to  claim 44  and one or more pharmaceutically acceptable excipients. 
     
     
       53. A pharmaceutical composition comprising a compound according to  claim 45  and one or more pharmaceutically acceptable excipients. 
     
     
       54. A pharmaceutical composition comprising a compound according to  claim 46  and one or more pharmaceutically acceptable excipients. 
     
     
       55. A pharmaceutical composition comprising a compound according to  claim 47  and one or more pharmaceutically acceptable excipients. 
     
     
       56. A pharmaceutical composition comprising a compound according to  claim 48  and one or more pharmaceutically acceptable excipients.

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