P
US9850236B2ActiveUtilityPatentIndex 71

Trifluoromethyl alcohols as modulators of RORγt

Assignee: JANSSEN PHARMACEUTICA NVPriority: Oct 30, 2014Filed: Oct 30, 2015Granted: Dec 26, 2017
Est. expiryOct 30, 2034(~8.3 yrs left)· nominal 20-yr term from priority
Inventors:GOLDBERG STEVENVENKATESAN HARIHARANTANIS VIRGINIAKINZEL OLAFGEGE CHRISTIANSTEENECK CHRISTOPHKLEYMANN GERALDHOFFMANN THOMASFOURIE ANNE MXUE XIAOHUA
A61P 37/02A61P 43/00A61P 37/00A61P 3/10A61P 37/06A61P 3/00A61P 29/00A61P 11/06A61P 17/06A61P 19/00A61P 1/04A61P 1/12A61P 11/00A61P 17/00A61P 25/00A61P 11/02A61P 19/02A61K 31/4439A61K 31/426A61K 31/454A61K 45/06C07D 495/10A61K 31/4709A61K 31/541C07D 487/08A61K 31/427C07D 417/14C07D 277/56C07D 417/06
71
PatentIndex Score
2
Cited by
79
References
43
Claims

Abstract

The present invention comprises compounds of Formula I. wherein: X, A 1 , A 2 , A 3 , A 4 , R 1 , R 2 , and R 3 are defined in the specification. The invention also comprises a method of treating or ameliorating a syndrome, disorder or disease, wherein said syndrome, disorder or disease is rheumatoid arthritis or psoriasis. The invention also comprises a method of modulating RORγt activity in a mammal by administration of a therapeutically effective amount of at least one compound of claim 1.

Claims

exact text as granted — not AI-modified
What is claimed is: 
     
       1. A compound of Formula I: 
       
         
           
           
               
               
           
         
         wherein 
         X is CH, CR 1 , or N; 
         A 1  is C (1-2) alkyl; 
         A 2  is cyclobutyl, or C (1-4) alkyl, wherein said C (1-4) alkyl is optionally substituted with OCH 3  or up to three fluorine atoms;
 or A 1  and A 2  are taken together with their attached nitrogen to form a ring selected the group consisting of azetidinyl, piperidinyl, pyrrolidinyl, 
 
       
       
         
           
           
               
               
           
         
       
       wherein said ring is optionally substituted with up to three substituents independently selected from the group consisting of F, CF 3 , CH 3 , —CN, and CH 2 OH;
 R 1  is Cl, C(CH 3 ) 3 , CH 2 CH 3 , OCF 3 , CF 3 , OCH(CH 3 ) 2 , CHF 2 , OCHF 2 , OCH 3 , F, CH 3 , or —CN; 
 R 2  is H, F, or Cl;
 or R 1  and R 2  may be taken together with their attached phenyl to form a naphthalenyl, or quinolinyl group; 
 
 R 3  is CF 3 , or CH 2 CH 3 ; 
 A 3  is H 
 A 4  is H, C (1-5) alkyl, 
 
       
         
           
           
               
               
           
         
         wherein said C (1-5) alkyl is optionally substituted with one to two substituents independently selected from COOH, CONH 2 , —CN, and OH;
 or A 3  and A 4  may be taken together with their attached nitrogen to make a ring selected from the group consisting of 
 
       
       
         
           
           
               
               
           
         
         and pharmaceutically acceptable salts thereof. 
       
     
     
       2. The compound of  claim 1  wherein:
 R 1  is Cl, C(CH 3 ) 3 , CH 2 CH 3 , OCF 3 , CF 3 , OCH(CH 3 ) 2 , CHF 2 , OCHF 2 , OCH 3 , F, or CH 3 ; 
 A 4  is H, C (1-5) alkyl, 
 
       
         
           
           
               
               
           
         
       
       wherein said C (1-5) alkyl is optionally substituted with one to two substituents independently selected from CONH 2 , —CN, and OH;
 and pharmaceutically acceptable salts thereof. 
 
     
     
       3. The compound of  claim 2 , of Formula II: 
       
         
           
           
               
               
           
         
         and pharmaceutically acceptable salts thereof. 
       
     
     
       4. The compound of  claim 2  selected from the group consisting of: 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         and pharmaceutically acceptable salts thereof. 
       
     
     
       5. The compound of  claim 3  selected from the group consisting of: 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         and pharmaceutically acceptable salts thereof. 
       
     
     
       6. The compound of  claim 1  selected from the group consisting of: 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         
           
           
               
               
           
         
         and pharmaceutically acceptable salts thereof. 
       
     
     
       7. A pharmaceutical composition, comprising a compound of  claim 1  and a pharmaceutically acceptable carrier. 
     
     
       8. A pharmaceutical composition made by mixing a compound of  claim 1  and a pharmaceutically acceptable carrier. 
     
     
       9. A process for making a pharmaceutical composition comprising mixing a compound of  claim 1  and a pharmaceutically acceptable carrier. 
     
     
       10. A method for treating or ameliorating a RORγt mediated inflammatory syndrome, disorder or disease selected from the group consisting of: inflammatory bowel diseases, rheumatoid arthritis, psoriasis, chronic obstructive pulmonary disorder, psoriatic arthritis, ankylosing spondylitis, neutrophilic asthma, steroid resistant asthma, multiple sclerosis, and systemic lupus erythematosus, comprising administering to a subject in need thereof an effective amount of a compound of  claim 1 . 
     
     
       11. The method of  claim 10 , wherein the disease is psoriasis. 
     
     
       12. The method of  claim 10 , wherein the disease is rheumatoid arthritis. 
     
     
       13. The method of  claim 10 , wherein the inflammatory bowel disease is ulcerative colitis. 
     
     
       14. The method of  claim 10 , wherein the inflammatory bowel disease is Crohn's disease. 
     
     
       15. The method of  claim 10 , wherein the disease is multiple sclerosis. 
     
     
       16. The method of  claim 10 , wherein the disease is neutrophilic asthma. 
     
     
       17. The method of  claim 10 , wherein the disease is steroid resistant asthma. 
     
     
       18. The method of  claim 10 , wherein the disease is psoriatic arthritis. 
     
     
       19. The method of  claim 10 , wherein the disease is ankylosing spondylitis. 
     
     
       20. The method of  claim 10 , wherein the disease is systemic lupus erythematosus. 
     
     
       21. The method of  claim 10 , wherein the disease is chronic obstructive pulmonary disorder. 
     
     
       22. The compound of  claim 5  selected from the group consisting of: 
       
         
           
           
               
               
           
         
         
           
           
               
               
           
         
       
       and pharmaceutically acceptable salts thereof. 
     
     
       23. The compound of  claim 22  that is: 
       
         
           
           
               
               
           
         
       
       and pharmaceutically acceptable salts thereof. 
     
     
       24. The compound of  claim 22  that is: 
       
         
           
           
               
               
           
         
       
       and pharmaceutically acceptable salts thereof. 
     
     
       25. The compound of  claim 22  that is: 
       
         
           
           
               
               
           
         
       
       and pharmaceutically acceptable salts thereof. 
     
     
       26. The compound of  claim 22  that is: 
       
         
           
           
               
               
           
         
       
       and pharmaceutically acceptable salts thereof. 
     
     
       27. The compound of  claim 22  that is: 
       
         
           
           
               
               
           
         
       
       and pharmaceutically acceptable salts thereof. 
     
     
       28. The compound of  claim 22  that is: 
       
         
           
           
               
               
           
         
       
       and pharmaceutically acceptable salts thereof. 
     
     
       29. A pharmaceutical composition, comprising a compound of  claim 22  and a pharmaceutically acceptable carrier. 
     
     
       30. A pharmaceutical composition made by mixing a compound of  claim 22  and a pharmaceutically acceptable carrier. 
     
     
       31. A process for making a pharmaceutical composition comprising mixing a compound of  claim 22  and a pharmaceutically acceptable carrier. 
     
     
       32. A method for treating or ameliorating a RORγt mediated inflammatory syndrome, disorder or disease selected from the group consisting of: inflammatory bowel diseases, rheumatoid arthritis, psoriasis, chronic obstructive pulmonary disorder, psoriatic arthritis, ankylosing spondylitis, neutrophilic asthma, steroid resistant asthma, multiple sclerosis, and systemic lupus erythematosus, comprising administering to a subject in need thereof an effective amount of a compound of  claim 22 . 
     
     
       33. The method of  claim 32 , wherein the disease is psoriasis. 
     
     
       34. The method of  claim 32 , wherein the disease is rheumatoid arthritis. 
     
     
       35. The method of  claim 32 , wherein the inflammatory bowel disease is ulcerative colitis. 
     
     
       36. The method of  claim 32 , wherein the inflammatory bowel disease is Crohn's disease. 
     
     
       37. The method of  claim 32 , wherein the disease is multiple sclerosis. 
     
     
       38. The method of  claim 32 , wherein the disease is neutrophilic asthma. 
     
     
       39. The method of  claim 32 , wherein the disease is steroid resistant asthma. 
     
     
       40. The method of  claim 32 , wherein the disease is psoriatic arthritis. 
     
     
       41. The method of  claim 32 , wherein the disease is ankylosing spondylitis. 
     
     
       42. The method of  claim 32 , wherein the disease is systemic lupus erythematosus. 
     
     
       43. The method of  claim 32 , wherein the disease is chronic obstructive pulmonary disorder.

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